金属@碳纳米片异质界面的协同工程用于双功能电磁波吸收与电化学储能

引用本文: 魏祺, 仇亚茹, 杨腾飞, 蒋艺玲, 朱韶涵, 周杰, 刘聪聪, 侯文杰, 王越, 刘冬. 金属@碳纳米片异质界面的协同工程用于双功能电磁波吸收与电化学储能[J]. 物理化学学报, 2026, 42(9): 100320. doi: 10.1016/j.actphy.2026.100320 shu

Citation: Qi Wei, Yaru Qiu, Tengfei Yang, Yiling Jiang, Shaohan Zhu, Jie Zhou, Congcong Liu, Wenjie Hou, Yue Wang, Dong Liu. Synergistic engineering of heterointerfaces in metal@carbon nanosheets for bifunctional electromagnetic wave absorption and electrochemical energy storage[J]. Acta Physico-Chimica Sinica, 2026, 42(9): 100320. doi: 10.1016/j.actphy.2026.100320 shu

金属@碳纳米片异质界面的协同工程用于双功能电磁波吸收与电化学储能

魏祺 ^{1, †,} ,
仇亚茹 ^{2, †,} ,
杨腾飞 ^{1, †,} ,
蒋艺玲 ^1, ,
朱韶涵 ^1, ,
周杰 ^{1,
,} ,
刘聪聪 ^3, ,
侯文杰 ^{4,
,} ,
王越 ^5, ,
刘冬 ^{1,
,}

1.
山东理工大学化学化工学院, 山东淄博 255049
2.
菏泽医学专科学校药学与检验系, 山东菏泽 274000
3.
淄博市检验检测计量研究总院, 山东淄博 255000
4.
电子科技大学基础与前沿研究院, 四川成都 610054
5.
湖北汽车工业学院汽车材料学院, 湖北十堰 442002

通讯作者: Email: tjuzhoujie@163.com (周杰); byhhwj@163.com (侯文杰); liu_dong@sdut.edu.cn (刘冬)

摘要: 无线通信与电子设备的普及加剧了电磁波污染与高性能储能需求的双重挑战。为解决这些问题，我们开发了一种简易策略制备金属(铜或钴)修饰的软碳多孔纳米片复合材料，该材料具有原位分散金属纳米颗粒的多级孔纳米片结构。系统表征证实了晶态铜相和钴相在碳基体中的成功复合。其中SC-N/Co复合材料展现出卓越的多功能性能：作为电磁波吸收体时，在1.5 mm的薄层厚度下可实现-39.10 dB的强反射损耗与6.16 GHz的宽频带吸收；作为锂离子电池负极时，则表现出高可逆容量、优异倍率性能及在1.0 A g^-1电流密度下循环1000次后仍保持~325 mA h g^-1的长周期稳定性。这种卓越性能源于界面极化增强、阻抗匹配优化及电荷传输动力学改善等多重协同效应。本研究为设计兼具电磁波调控与高效储能双功能的碳-金属复合材料提供了新思路。

关键词:

English

Synergistic engineering of heterointerfaces in metal@carbon nanosheets for bifunctional electromagnetic wave absorption and electrochemical energy storage

Qi Wei ^{1, †,} ,
Yaru Qiu ^{2, †,} ,
Tengfei Yang ^{1, †,} ,
Yiling Jiang ^1, ,
Shaohan Zhu ^1, ,
Jie Zhou ^{1,
,} ,
Congcong Liu ^3, ,
Wenjie Hou ^{4,
,} ,
Yue Wang ^5, ,
Dong Liu ^{1,
,}

1.
School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo 255049, Shandong Province, China
2.
Department of Pharmacy and Laboratory Medicine, Heze Medical College, Heze 274000, Shandong Province, China
3.
Zibo Municipal General Institute of Inspection and Metrology, Zibo 255000, Shandong Province, China
4.
Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, Sichuan Province, China
5.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China

Corresponding author: Email: tjuzhoujie@163.com (Jie Zhou); byhhwj@163.com (Wenjie Hou); liu_dong@sdut.edu.cn (Dong Liu)

Received Date: 01 April 2026
Accepted Date: 08 May 2026
Revised Date: 04 May 2026
Available Online: 15 September 2026

Abstract: The proliferation of wireless communication and electronic devices has intensified the dual challenges of electromagnetic (EM) wave pollution and the demand for high-performance energy storage. To address these issues, we develop a facile strategy to fabricate metal (Cu or Co)-decorated soft carbon porous nanosheet composites, which exhibit a hierarchical porous nanosheet structure with in situ dispersed metallic nanoparticles. Systematic characterization confirms the successful integration of crystalline Cu and Co phases within the carbon matrix. The SC-N/Co composite exhibits exceptional multifunctional performance. As an electromagnetic wave absorber, it achieves a strong reflection loss of -39.10 dB and a broad bandwidth of 6.16 GHz at a thin matching thickness of 1.5 mm. Concurrently, as a lithium-ion battery anode, it delivers high reversible capacity, rate capability, and outstanding long-term cycling stability of ~325 mA h g^-1 after 1000 cycles at 1.0 A g^-1. The superior performance is attributed to synergistic effects, including enhanced interfacial polarization, optimized impedance matching, and improved charge transport kinetics. This study provides a promising pathway for designing carbon-metal composites for dual-functional applications in EM wave management and efficient energy storage.

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1.
沈阳化工大学材料科学与工程学院沈阳 110142

金属@碳纳米片异质界面的协同工程用于双功能电磁波吸收与电化学储能

通讯作者: Email: tjuzhoujie@163.com (周杰); byhhwj@163.com (侯文杰); liu_dong@sdut.edu.cn (刘冬)

English

Synergistic engineering of heterointerfaces in metal@carbon nanosheets for bifunctional electromagnetic wave absorption and electrochemical energy storage

Corresponding author: Email: tjuzhoujie@163.com (Jie Zhou); byhhwj@163.com (Wenjie Hou); liu_dong@sdut.edu.cn (Dong Liu)

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通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

金属@碳纳米片异质界面的协同工程用于双功能电磁波吸收与电化学储能

通讯作者: Email: tjuzhoujie@163.com (周杰); byhhwj@163.com (侯文杰); liu_dong@sdut.edu.cn (刘冬)

English

Synergistic engineering of heterointerfaces in metal@carbon nanosheets for bifunctional electromagnetic wave absorption and electrochemical energy storage

Corresponding author: Email: tjuzhoujie@163.com (Jie Zhou); byhhwj@163.com (Wenjie Hou); liu_dong@sdut.edu.cn (Dong Liu)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

计量

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通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs