微波辅助构筑Ta2CTx MXene/CuInS2异质结构增强介电损耗和宽频电磁波吸收性能

引用本文: 张帅, 李海丰, 张世杰, 王顺, 杜苏轩, 赵志伟, 赵小苗, 梁笑微. 微波辅助构筑Ta₂CT_x MXene/CuInS₂异质结构增强介电损耗和宽频电磁波吸收性能[J]. 物理化学学报, 2026, 42(8): 100305. doi: 10.1016/j.actphy.2026.100305 shu

Citation: Shuai Zhang, Haifeng Li, Shijie Zhang, Shun Wang, Suxuan Du, Zhiwei Zhao, Xiaomiao Zhao, Xiaowei Liang. Microwave assisted construction of Ta₂CT_x MXene/CuInS₂ heterostructures toward enhanced dielectric loss and broadband electromagnetic wave absorption[J]. Acta Physico-Chimica Sinica, 2026, 42(8): 100305. doi: 10.1016/j.actphy.2026.100305 shu

微波辅助构筑Ta₂CT_x MXene/CuInS₂异质结构增强介电损耗和宽频电磁波吸收性能

张帅 ^1, ,
李海丰 ^2, ,
张世杰 ^{1,
,} ,
王顺 ^{1,
,} ,
杜苏轩 ^1, ,
赵志伟 ^{1,
,} ,
赵小苗 ^1, ,
梁笑微 ^1,

1.
河南工业大学材料科学与工程学院, 河南郑州 450001
2.
湖北汽车工业学院汽车材料学院, 湖北十堰 442002

通讯作者: Email: zsj562389@sina.com (张世杰); shun_wang@haut.edu.cn (王顺); zzw3217@163.com (赵志伟)

摘要: MXene在电磁波吸收领域的应用日益广泛。为挖掘更多MXene类型的潜力，本研究通过HF蚀刻成功合成了Ta₂CT_x MXene，并利用微波辅助化学合成系统制备了一系列Ta₂CT_x MXene/CuInS₂复合材料。实验表明：在2.9 mm厚度、50 wt%填料负载量的条件下，Ta₂CT_x样品的最小反射损耗达到−27.61 dB，有效吸收带宽为0.08 GHz；而同等填料负载下，Ta₂CT_x MXene/CuInS₂-50复合材料在更薄的1.5 mm厚度处表现出显著更优的4.48 GHz有效吸收带宽。这种性能提升归因于CuInS₂的引入改善了阻抗匹配并增强了介电损耗。此外，两组分形成的多层片状结构构建了连续导电网络，通过多重反射和导电损耗有效耗散了电磁能量。本研究为开发基于Ta₂CT_x MXene的高效吸波材料提供了可行策略。

关键词:

English

Microwave assisted construction of Ta₂CT_x MXene/CuInS₂ heterostructures toward enhanced dielectric loss and broadband electromagnetic wave absorption

Shuai Zhang ^1, ,
Haifeng Li ^2, ,
Shijie Zhang ^{1,
,} ,
Shun Wang ^{1,
,} ,
Suxuan Du ^1, ,
Zhiwei Zhao ^{1,
,} ,
Xiaomiao Zhao ^1, ,
Xiaowei Liang ^1,

1.
School of Material Science and Engineering, Henan University of Technology, Zhengzhou 450001, Henan Province, China
2.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China

Corresponding author: Email: zsj562389@sina.com (Shijie Zhang); shun_wang@haut.edu.cn (Shun Wang); zzw3217@163.com (Zhiwei Zhao)

Received Date: 08 March 2026
Accepted Date: 16 April 2026
Revised Date: 12 April 2026
Available Online: 15 August 2026

Abstract: The application of MXene in the electromagnetic wave absorption (EWA) field has been increasingly extensive. To explore the potential of more MXene types, this study has successfully synthesized Ta₂CT_x MXene via HF etching and subsequently prepared a series of Ta₂CT_x MXene/CuInS₂ composites using a microwave-assisted chemical synthesis system. The Ta₂CT_x sample has demonstrated an optimal minimum reflection loss (RL_min) of −27.61 dB with an effective absorption bandwidth (EAB) of 0.8 GHz at a thin thickness of 2.9 mm and a 50 wt% filler loading. In contrast, the Ta₂CT_x MXene/CuInS₂-50 composite has exhibited a significantly superior EAB of 4.48 GHz at a thinner thickness of 1.5 mm under the same filler loading condition. This enhanced performance has been attributed to the improved impedance matching and increased dielectric loss contributed by the incorporation of CuInS₂. Furthermore, the multilayered sheet-like structure formed by the two components has established a continuous conductive network, which has effectively dissipated electromagnetic energy through multiple reflections and conductive loss. Ultimately, this work has provided a viable strategy for developing high-efficiency absorbers based on Ta₂CT_x MXene materials.

Key words:

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沈阳化工大学材料科学与工程学院沈阳 110142

微波辅助构筑Ta₂CT_x MXene/CuInS₂异质结构增强介电损耗和宽频电磁波吸收性能

通讯作者: Email: zsj562389@sina.com (张世杰); shun_wang@haut.edu.cn (王顺); zzw3217@163.com (赵志伟)

English

Microwave assisted construction of Ta₂CT_x MXene/CuInS₂ heterostructures toward enhanced dielectric loss and broadband electromagnetic wave absorption

Corresponding author: Email: zsj562389@sina.com (Shijie Zhang); shun_wang@haut.edu.cn (Shun Wang); zzw3217@163.com (Zhiwei Zhao)

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