二氧化锰@氮掺杂碳@镍铁氧体杂化材料的一锅法绿色合成及吸波性能研究

戴鑫鑫 兰笛 陈星亮 王行伟 姬广斌

引用本文: 戴鑫鑫, 兰笛, 陈星亮, 王行伟, 姬广斌. 二氧化锰@氮掺杂碳@镍铁氧体杂化材料的一锅法绿色合成及吸波性能研究[J]. 物理化学学报, 2026, 42(8): 100302. doi: 10.1016/j.actphy.2026.100302 shu
Citation:  Xinxin Dai, Di Lan, Xingliang Chen, Xingwei Wang, Guangbin Ji. One pot green synthesis and electromagnetic wave absorption performance of manganese dioxide@nitrogen-doped carbon@NiFe2O4 hybrids[J]. Acta Physico-Chimica Sinica, 2026, 42(8): 100302. doi: 10.1016/j.actphy.2026.100302 shu

二氧化锰@氮掺杂碳@镍铁氧体杂化材料的一锅法绿色合成及吸波性能研究

    通讯作者: Email: chenxlmoon@163.com (陈星亮); wangxingwei@licp.cas.cn (王行伟); gbji@nuaa.edu.cn (姬广斌)
摘要: 技术革新与工业化的加速推进使电磁辐射的防护及重金属污染的治理成为当前的研究热点。本研究采用原创的一锅法绿色合成工艺,制备出了二氧化锰@氮掺杂碳@镍铁氧体复合杂化材料。通过系统性的表征,深入分析了合成产物的微观结构形貌、晶相组成、化学元素分布、电磁参数及吸波性能。反射损耗曲线结果表明:通过调控吡咯单体用量制备的优化样品表现出了理想的电磁波吸收性能,在3.2 mm匹配厚度下的最低反射损耗值可达到−48 dB,这主要可以归因于界面极化引发的共振效应、良好的阻抗匹配及其他协同因素。该一锅法合成策略所体现的绿色理念,对推动绿色合成技术的发展具有积极意义。

English

    1. [1]

      X. Ren, Z. Jia, Z. Gao, S. Zhang, Y. Zhang, D. Lan, G. Wu, Adv. Funct. Mater. (2025) e24264, https://doi.org/10.1002/adfm.202524264. doi: 10.1002/adfm.202524264

    2. [2]

      M. Shi, Z. Jia, D. Lan, Z. Gao, S. Zhang, G. Wu, Adv. Funct. Mater. (2025) e28665, https://doi.org/10.1002/adfm.202528665. doi: 10.1002/adfm.202528665

    3. [3]

      P. Yin, D. Lan, Z. Yuan, R. Wang, Y. Zhang, X. Sun, J. Alloys Compd. 1037 (2025) 182260, https://doi.org/10.1016/j.jallcom.2025.182260. doi: 10.1016/j.jallcom.2025.182260

    4. [4]

      X. Chen, F. Zhang, D. Lan, S. Zhang, S. Du, Z. Zhao, G. Ji, G. Wu, Adv. Compos. Hybrid Mater. 6 (6) (2023) 220, https://doi.org/10.1007/s42114-023-00792-4. doi: 10.1007/s42114-023-00792-4

    5. [5]

      Y. Shen, C. Zhao, X. Wang, Q. Yu, F. Zhou, Tribol. Int. 214 (2026) 111229, https://doi.org/10.1016/j.triboint.2025.111229. doi: 10.1016/j.triboint.2025.111229

    6. [6]

      Z. Jia, J. Li, D. Lan, S. Zhang, Z. Gao, X. Shi, G. Wu, J. Mater. Sci. Technol. 256 (2026) 246, https://doi.org/10.1016/j.jmst.2025.08.044. doi: 10.1016/j.jmst.2025.08.044

    7. [7]

      S.-X. Xiong, L.-J. Cai, Y. Zhang, Y. Ma, D. Lan, G. Chen, C.-J. Dong, H.-T. Guan, Rare Metals 44 (10) (2025) 7720, https://doi.org/10.1007/s12598-025-03439-z. doi: 10.1007/s12598-025-03439-z

    8. [8]

      W. Gu, Z. Luo, J. Wang, X. Tan, Z. Tao, P. Zhou, H. Zhang, D. Lan, A. Xia, J. Mater. Sci. Technol. 243 (2026) 102, https://doi.org/10.1016/j.jmst.2025.04.024. doi: 10.1016/j.jmst.2025.04.024

    9. [9]

      Y. Y. Wang, F. Zhang, N. Li, J. F. Shi, L. C. Jia, D. X. Yan, Z. M. Li, Carbon 205 (2023) 10, https://doi.org/10.1016/j.carbon.2023.01.007. doi: 10.1016/j.carbon.2023.01.007

    10. [10]

      J. Xu, Y. Zhao, Y. Chen, Y. Chen, Z.-H. Xie, P. R. Munroe, ACS Appl. Mater. Interfaces 14 (37) (2022) 42468, https://doi.org/10.1021/acsami.2c11642. doi: 10.1021/acsami.2c11642

    11. [11]

      W. Zhao, Z. Guo, D. Lan, Z. Jia, S. Zhang, G. Wu, Small 21 (45) (2025) e09339, https://doi.org/10.1002/smll.202509339. doi: 10.1002/smll.202509339

    12. [12]

      S. Sharma, S. R. Parne, S. S. S. Panda, S. Gandi, Adv. Colloid Interface Sci. 327 (2024) 103143, https://doi.org/10.1016/j.cis.2024.103143. doi: 10.1016/j.cis.2024.103143

    13. [13]

      Z.-h. Liu, R. Tao, P. Luo, X. Shu, G.-d. Ban, RSC Advances 7 (73) (2017) 46060, https://doi.org/10.1039/C7RA07666E. doi: 10.1039/C7RA07666E

    14. [14]

      Y. Liu, Z. Zhang, S. Xiao, C. Qiang, L. Tian, J. Xu, Appl. Surf. Sci. 257 (17) (2011) 7678, https://doi.org/10.1016/j.apsusc.2011.04.007. doi: 10.1016/j.apsusc.2011.04.007

    15. [15]

      G. Xie, Z. Zhang, R. Wu, Journal of Wuhan University of Technology-Mater. Sci. Ed. 20 (4) (2005) 55, https://doi.org/10.1007/BF02841283. doi: 10.1007/BF02841283

    16. [16]

      Y. Zhang, D. Lan, Z. Wang, G. Xu, Z. Gao, G. Bu, X. Zhong, P. Yin, Adv. Compos. Hybrid Mater. 8 (5) (2025) 387, https://doi.org/10.1007/s42114-025-01444-5. doi: 10.1007/s42114-025-01444-5

    17. [17]

      W. Wang, H. Cheng, J. Wang, S. Wang, X. Liu, Mater. Res. Bull. 179 (2024) 112954, https://doi.org/10.1016/j.materresbull.2024.112954. doi: 10.1016/j.materresbull.2024.112954

    18. [18]

      Q. Wang, Y. Liu, E. Su, X. Su, Mater. Today Nano 29 (2025) 100603, https://doi.org/10.1016/j.mtnano.2025.100603. doi: 10.1016/j.mtnano.2025.100603

    19. [19]

      X. Chen, D. Lan, L. Zhou, Z. Zeng, Y. Liu, S. Du, Z. Zou, G. Wu, Ceram. Int. 50 (13, Part B) (2024) 24549, https://doi.org/10.1016/j.ceramint.2024.04.190. doi: 10.1016/j.ceramint.2024.04.190

    20. [20]

      X. Chen, Y. Wang, H. Liu, S. Jin, G. Wu, J. Colloid Interface Sci. 606 (2022) 526, https://doi.org/10.1016/j.jcis.2021.07.094. doi: 10.1016/j.jcis.2021.07.094

    21. [21]

      J. Ge, S. Liu, L. Liu, Y. Cui, F. Meng, Y. Li, X. Zhang, F. Wang, J. Mater. Sci. Technol. 81 (2021) 190, https://doi.org/10.1016/j.jmst.2020.10.082. doi: 10.1016/j.jmst.2020.10.082

    22. [22]

      H. Zhang, Z. Jia, B. Wang, X. Wu, T. Sun, X. Liu, L. Bi, G. Wu, Chem. Eng. J. 421 (2021) 129960, https://doi.org/10.1016/j.cej.2021.129960. doi: 10.1016/j.cej.2021.129960

    23. [23]

      F. T. Thema, E. Manikandan, A. Gurib-Fakim, M. Maaza, J. Alloys Compd. 657 (2016) 655, https://doi.org/10.1016/j.jallcom.2015.09.227. doi: 10.1016/j.jallcom.2015.09.227

    24. [24]

      N. Matinise, X. G. Fuku, K. Kaviyarasu, N. Mayedwa, M. Maaza, Appl. Surf. Sci. 406 (2017) 339, https://doi.org/10.1016/j.apsusc.2017.01.219. doi: 10.1016/j.apsusc.2017.01.219

    25. [25]

      X. Chen, W. Wang, T. Shi, G. Wu, Y. Lu, Carbon 163 (2020) 202, https://doi.org/10.1016/j.carbon.2020.03.005. doi: 10.1016/j.carbon.2020.03.005

    26. [26]

      S. Luo, S. Dong, C. Lu, C. Yu, Y. Ou, L. Luo, J. Sun, J. Sun, J. Colloid Interface Sci. 513 (2018) 389, https://doi.org/10.1016/j.jcis.2017.11.044. doi: 10.1016/j.jcis.2017.11.044

    27. [27]

      A. G. M. da Silva, T. S. Rodrigues, E. G. Candido, I. C. de Freitas, A. H. M. da Silva, H. V. Fajardo, R. Balzer, J. F. Gomes, J. M. Assaf, D. C. de Oliveira, N. Oger, S. Paul, R. Wojcieszak, P. H. C. Camargo, J. Colloid Interface Sci. 530 (2018) 282, https://doi.org/10.1016/j.jcis.2018.06.089. doi: 10.1016/j.jcis.2018.06.089

    28. [28]

      Y. Jin, C. Fan, Q. Zhang, Q. He, Y. Wang, Inorg. Chem. Front. 12 (23) (2025) 7590, https://doi.org/10.1039/D5QI01376C. doi: 10.1039/D5QI01376C

    29. [29]

      Y. Zhao, H. Zhang, X. Yang, H. Huang, G. Zhao, T. Cong, X. Zuo, Z. fan, S. Yang, L. Pan, Carbon 171 (2021) 395, https://doi.org/10.1016/j.carbon.2020.09.036. doi: 10.1016/j.carbon.2020.09.036

    30. [30]

      Y. Lei, Q. He, Y. Wang, C. Fan, X. Yin, C. Wang, L. Liu, ACS Sustain. Chem. Eng. 13 (39) (2025) 16679, https://doi.org/10.1021/acssuschemeng.5c07718. doi: 10.1021/acssuschemeng.5c07718

    31. [31]

      Z. Ye, K. Wang, X. Li, J. Yang, J. Alloys Compd. 893 (2022) 162396, https://doi.org/10.1016/j.jallcom.2021.162396. doi: 10.1016/j.jallcom.2021.162396

    32. [32]

      J. Wen, D. Lan, Y. Wang, L. Ren, A. Feng, Z. Jia, G. Wu, Int. J. Miner. Metall. Mater. 31 (7) (2024) 1701, https://doi.org/10.1007/s12613-024-2881-0. doi: 10.1007/s12613-024-2881-0

    33. [33]

      L. Wang, X. Yu, X. Li, J. Zhang, M. Wang, R. Che, Chem. Eng. J. 383 (2020) 123099, https://doi.org/10.1016/j.cej.2019.123099. doi: 10.1016/j.cej.2019.123099

    34. [34]

      S. Zhang, Z. Jia, Y. Zhang, G. Wu, Nano Res. 16 (2) (2023) 3395, https://doi.org/10.1007/s12274-022-5368-1. doi: 10.1007/s12274-022-5368-1

    35. [35]

      L. Chai, Y. Wang, Z. Jia, Z. Liu, S. Zhou, Q. He, H. Du, G. Wu, Chem. Eng. J. 429 (2022) 132547, https://doi.org/10.1016/j.cej.2021.132547. doi: 10.1016/j.cej.2021.132547

    36. [36]

      S. Deng, X. Xu, C. Fan, Q. He, Y. Wang, Colloid Surf. A-Physicochem. Eng. Asp. 727 (2025) 138430, https://doi.org/10.1016/j.colsurfa.2025.138430. doi: 10.1016/j.colsurfa.2025.138430

    37. [37]

      P. Li, D. Xiang, Q. He, C. Fan, Y. Wang, X. Yin, J. Colloid Interface Sci. 702 (2026) 138997, https://doi.org/10.1016/j.jcis.2025.138997. doi: 10.1016/j.jcis.2025.138997

    38. [38]

      S. J. Cheon, J. R. Choi, S.-b. Lee, J. I. Lee, H. Lee, J. Alloys Compd. 976 (2024) 173019, https://doi.org/10.1016/j.jallcom.2023.173019. doi: 10.1016/j.jallcom.2023.173019

    39. [39]

      H. Zhang, C. Shi, Z. Jia, X. Liu, B. Xu, D. Zhang, G. Wu, J. Colloid Interface Sci. 584 (2021) 382, https://doi.org/10.1016/j.jcis.2020.09.122. doi: 10.1016/j.jcis.2020.09.122

    40. [40]

      X. Chen, D. Lan, L. Zhou, H. Liu, X. Song, S. Wang, Z. Zou, G. Wu, Int. J. Miner., Metall. Mater. 32 (3) (2025) 591, https://doi.org/10.1007/s12613-024-3063-9. doi: 10.1007/s12613-024-3063-9

    41. [41]

      J. Tang, K. Wang, Y. Lu, N. Liang, X. Qin, G. Tian, D. Zhang, S. Feng, H. Yue, J. Magn. Magn. Mater. 514 (2020) 167268, https://doi.org/10.1016/j.jmmm.2020.167268. doi: 10.1016/j.jmmm.2020.167268

    42. [42]

      S. Golchinvafa, S. M. Masoudpanah, J. Alloys Compd. 787 (2019) 390, https://doi.org/10.1016/j.jallcom.2019.02.039. doi: 10.1016/j.jallcom.2019.02.039

    43. [43]

      M. Qin, L. Zhang, X. Zhao, H. Wu, Adv. Funct. Mater 31 (30) (2021) 2103436, https://doi.org/10.1002/adfm.202103436. doi: 10.1002/adfm.202103436

    44. [44]

      Y. Zhang, X. Wang, T. Dong, S. Yang, Q. Yu, B. Yu, M. Cai, F. Zhou, J. Colloid Interface Sci. 686 (2025) 829, https://doi.org/10.1016/j.jcis.2025.02.009. doi: 10.1016/j.jcis.2025.02.009

    45. [45]

      Y. Zhang, X. Wang, S. Yang, C. Li, T. Dong, Q. Yu, Ceram. Int. 50 (14) (2024) 25216, https://doi.org/10.1016/j.ceramint.2024.04.252. doi: 10.1016/j.ceramint.2024.04.252

    46. [46]

      T. Hou, Z. Jia, B. Wang, H. Li, X. Liu, L. Bi, G. Wu, Chem. Eng. J. 414 (2021) 128875, https://doi.org/10.1016/j.cej.2021.128875. doi: 10.1016/j.cej.2021.128875

    47. [47]

      S. Zhang, Z. Gao, Z. Sun, B. Cheng, Z. Zhao, Y. Jia, G. Wu, Appl. Surf. Sci. 611 (2023) 155707, https://doi.org/10.1016/j.apsusc.2022.155707. doi: 10.1016/j.apsusc.2022.155707

    48. [48]

      O. C. Compton, S. T. Nguyen, Small 6 (2010) 711, https://doi.org/10.1002/smll.200901934. doi: 10.1002/smll.200901934

    49. [49]

      X. Wang, S. Yang, C. Li, C. Zhao, Y. Liu, S. Sun, X. Chen, B. Yu, M. Cai, Q. Yu, F. Zhou, W. Liu, Prog. Org. Coat. 192 (2024) 108500, https://doi.org/10.1016/j.porgcoat.2024.108500. doi: 10.1016/j.porgcoat.2024.108500

    50. [50]

      S. Zhang, J. Li, X. Jin, G. Wu, Int. J. Miner., Metall. Mater. 30 (3) (2023) 428, https://doi.org/10.1007/s12613-022-2546-9. doi: 10.1007/s12613-022-2546-9

    51. [51]

      Y. Guo, J. Hao, T. Wang, S. Su, S. Yang, X. Wang, Q. Yu, J. Mater. Sci.-Mater. Electron. 36 (31) (2025) 1972, https://doi.org/10.1007/s10854-025-16014-0. doi: 10.1007/s10854-025-16014-0

    52. [52]

      P. Liu, Y. Huang, X. Zhang, Compos. Sci. Technol. 107 (2015) 54, https://doi.org/10.1016/j.compscitech.2014.11.021. doi: 10.1016/j.compscitech.2014.11.021

    53. [53]

      H. Liu, Y. Li, M. Yuan, G. Sun, H. Li, S. Ma, Q. Liao, Y. Zhang, ACS Appl. Mater. Interfaces 10 (26) (2018) 22591, https://doi.org/10.1021/acsami.8b05211. doi: 10.1021/acsami.8b05211

    54. [54]

      X. Chen, K. Zhong, T. Shi, X. Meng, G. Wu, Y. Lu, Synth. Met. 248 (2019) 59, https://doi.org/10.1016/j.synthmet.2019.01.006. doi: 10.1016/j.synthmet.2019.01.006

    55. [55]

      X. Chen, Z. Jia, A. Feng, B. Wang, X. Tong, C. Zhang, G. Wu, J. Colloid Interface Sci. 553 (2019) 465, https://doi.org/10.1016/j.jcis.2019.06.058. doi: 10.1016/j.jcis.2019.06.058

    56. [56]

      J. Feng, Y. Wang, Y. Hou, J. Li, L. Li, Ceram. Int. 42 (15) (2016) 17814, https://doi.org/10.1016/j.ceramint.2016.08.110. doi: 10.1016/j.ceramint.2016.08.110

    57. [57]

      J. Fang, Z. Chen, W. Wei, Y. Li, T. Liu, Z. Liu, X. Yue, Z. Jiang, RSC Advances 5 (62) (2015) 50024, https://doi.org/10.1039/C5RA07192E. doi: 10.1039/C5RA07192E

    58. [58]

      T. Cheng, Y. Guo, Y. Xie, L. Zhao, T. Wang, A. Meng, Z. Li, M. Zhang, Carbon 206 (2023) 181, https://doi.org/10.1016/j.carbon.2023.02.052. doi: 10.1016/j.carbon.2023.02.052

    59. [59]

      X. Zhang, H. Jiang, L. Xu, K. Zuraiqi, T. Daeneke, J. Zhou, G. K. Li, A. Zavabeti, Ceram. Int. 48 (7) (2022) 10066, https://doi.org/10.1016/j.ceramint.2021.12.216. doi: 10.1016/j.ceramint.2021.12.216

    60. [60]

      X. Sun, Z. Wang, S. Wang, Y. Ning, M. Yang, S. Yang, L. Zhou, Q. He, Y. Li, Chem. Eng. J. 422 (2021) 130142, https://doi.org/10.1016/j.cej.2021.130142. doi: 10.1016/j.cej.2021.130142

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  • 发布日期:  2026-08-15
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