锚定策略诱导Ni-MOF@膨胀石墨复合材料的导电损耗以实现宽带微波吸收

引用本文: 冯仁威, 范聪敏, 兰笛, 刘澜翔, 何秦川, 王益群. 锚定策略诱导Ni-MOF@膨胀石墨复合材料的导电损耗以实现宽带微波吸收[J]. 物理化学学报, 2026, 42(8): 100301. doi: 10.1016/j.actphy.2026.100301 shu

Citation: Renwei Feng, Congmin Fan, Di Lan, Lanxiang Liu, Qinchuan He, Yiqun Wang. Anchoring strategy-induced conductive loss in Ni-MOF@expanded graphite composites to achieve broadband microwave absorption[J]. Acta Physico-Chimica Sinica, 2026, 42(8): 100301. doi: 10.1016/j.actphy.2026.100301 shu

锚定策略诱导Ni-MOF@膨胀石墨复合材料的导电损耗以实现宽带微波吸收

冯仁威 ^1, ,
范聪敏 ^{1,
,} ,
兰笛 ^2, ,
刘澜翔 ^1, ,
何秦川 ^1, ,
王益群 ^{1, 3,
,}

1.
成都理工大学材料与化学化工学院, 四川成都 610059
2.
湖北汽车工业学院材料科学与工程学院, 湖北十堰 442002
3.
西北工业大学化学与化工学院, 陕西西安 710072

通讯作者: congmin@mail.ustc.edu.cn (范聪敏); Email: wangyiqun17@cdut.edu.cn (王益群)

摘要: 金属有机框架(MOF)衍生物因其大比表面积和结构可调性，已成为电磁波吸收材料的候选者。然而，磁性MOF衍生物导电损耗不足及团聚问题严重制约了其应用。本文提出了一种新型导电网络构建工程与锚定策略，通过镍催化自组装及热处理工艺，设计出具有层状网格结构的Ni-MOF@碳纤维/膨胀石墨(EG)复合材料。具体而言，通过精确调控碳源与网格状EG，诱导游离碳构建了既可连接EG又能锚定MOF衍生物的导电网络。扫描电镜分析证实碳纤维连接EG层形成了更丰富的微导电网络。同时，碳纤维的锚定作用调控了阻抗匹配并激活界面诱导极化，电磁参数测试验证了该现象。因此，S-4样品的最小反射损耗(RL_min)达到−41.73 dB，最大有效吸收带宽(EAB_max)为5.12 GHz，匹配厚度仅1.48 mm，雷达散射截面显著降低39.58 dB m²。该工作为高性能电磁波吸收材料的导电网络构建工程与锚定技术应用提供了重要启示。

关键词:

English

Anchoring strategy-induced conductive loss in Ni-MOF@expanded graphite composites to achieve broadband microwave absorption

1.
College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu 610059, Sichuan Province, China
2.
School of Materials Science and Engineering, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China
3.
School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710072, Shaanxi Province, China

Corresponding author: congmin@mail.ustc.edu.cn (Congmin Fan); Email: wangyiqun17@cdut.edu.cn (Yiqun Wang)

Received Date: 03 March 2026
Accepted Date: 08 April 2026
Revised Date: 07 April 2026
Available Online: 15 August 2026

Abstract: Metal-organic framework (MOF) derivatives have become candidates for electromagnetic wave absorption materials due to their large specific surface area and structural tunability. However, the insufficient conductivity loss and agglomeration of magnetic MOF derivatives seriously hinder their application. Herein, a novel conductive network construction engineering and anchoring strategy is proposed to design Ni-MOF@carbon fibers/Expanded graphite (EG) composites with a layered grid structure using Ni-catalyzed self-assembly and heat treatment processes. Specifically, free carbon is promoted to form a conductive network connecting EG and anchoring MOF derivatives by meticulously controlling the carbon source and grid-like EG. SEM analysis confirmed that the carbon fibers connected the EG layers to form a richer conductive micronetwork. Simultaneously, the anchoring of the carbon fibers regulated the impedance matching and activated the interface-induced polarization, which was confirmed by electromagnetic parameters. Therefore, the RL_min of S-4 reached −41.73 dB, the EAB_max was 5.12 GHz, the matching thickness was only 1.48 mm, and the radar cross section value was greatly reduced 39.58 dB·m². This work provides meaningful insights into the potential applications of conductive network construction engineering and anchoring technology for high-performance electromagnetic wave absorbing materials.

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沈阳化工大学材料科学与工程学院沈阳 110142

锚定策略诱导Ni-MOF@膨胀石墨复合材料的导电损耗以实现宽带微波吸收

通讯作者: congmin@mail.ustc.edu.cn (范聪敏); Email: wangyiqun17@cdut.edu.cn (王益群)

English

Anchoring strategy-induced conductive loss in Ni-MOF@expanded graphite composites to achieve broadband microwave absorption

Corresponding author: congmin@mail.ustc.edu.cn (Congmin Fan); Email: wangyiqun17@cdut.edu.cn (Yiqun Wang)

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中国化学会秘书处

锚定策略诱导Ni-MOF@膨胀石墨复合材料的导电损耗以实现宽带微波吸收

通讯作者: congmin@mail.ustc.edu.cn (范聪敏); Email: wangyiqun17@cdut.edu.cn (王益群)

English

Anchoring strategy-induced conductive loss in Ni-MOF@expanded graphite composites to achieve broadband microwave absorption

Corresponding author: congmin@mail.ustc.edu.cn (Congmin Fan); Email: wangyiqun17@cdut.edu.cn (Yiqun Wang)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

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CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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