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钠离子电池正极材料中离子迁移与电子转移的协同优化

王双 ,  傅小奇 ,  姚山山

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引用本文: 王双, 傅小奇, 姚山山. 钠离子电池正极材料中离子迁移与电子转移的协同优化[J]. 物理化学学报, 2026, 42(5): 100206. doi: 10.1016/j.actphy.2025.100206 shu
Citation:  Shuang Wang, Xiaoqi Fu, Shanshan Yao. Synergistic optimization of ion migration and electron transfer in sodium-ion battery cathode materials[J]. Acta Physico-Chimica Sinica, 2026, 42(5): 100206. doi: 10.1016/j.actphy.2025.100206 shu

钠离子电池正极材料中离子迁移与电子转移的协同优化

  • 1.

    江苏大学材料科学与工程学院, 江苏 镇江 212013

  • 2.

    江苏大学化学化工学院, 江苏 镇江 212013

    • 通讯作者: Email: xfu@ujs.edu.cn (傅小奇); yaosshan@hotmail.com (姚山山)
摘要: 钠离子电池(SIBs)凭借钠资源丰富、成本低廉及环境友好等优势，在大规模储能系统中展现出巨大应用潜力。正极材料的离子迁移与电子转移速率是决定电池倍率性能、循环寿命及容量保持率的关键因素，二者的协同提升对突破性能瓶颈至关重要。本文以钠离子电池三大主流正极材料——层状过渡金属氧化物(LTMOs)、聚阴离子化合物(PACs)和普鲁士蓝类似物(PBAs)为研究对象，系统梳理了不同材料体系中离子迁移通道与电子转移路径的结构基础，深入解析了二者的协同调控机制。结合最新研究成果，从元素优化、结构设计与复合改性三个维度，阐释了协同提升离子通道通畅性与电子通路连续性的具体路径与作用机理，提炼出高性能SIBs正极材料的普适性设计策略，为进一步开发兼具高容量、高倍率性能与稳定的SIBs正极材料提供了有益参考。

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