玉米酒糟衍生硬碳：一种可持续的高倍率、长寿命钠离子电池负极材料

引用本文: 张雪, 何子涵, 吴英琪, 余维来, 刘涛. 玉米酒糟衍生硬碳：一种可持续的高倍率、长寿命钠离子电池负极材料[J]. 物理化学学报, 2026, 42(5): 100199. doi: 10.1016/j.actphy.2025.100199 shu

Citation: Xue Zhang, Zihan He, Yingqi Wu, Weilai Yu, Tao Liu. Corn-distillers-derived hard carbon: a sustainable high-rate, long-life anode for sodium-ion batteries[J]. Acta Physico-Chimica Sinica, 2026, 42(5): 100199. doi: 10.1016/j.actphy.2025.100199 shu

玉米酒糟衍生硬碳：一种可持续的高倍率、长寿命钠离子电池负极材料

张雪 ^1, ,
何子涵 ^1, ,
吴英琪 ^1, ,
余维来 ^{2,
,} ,
刘涛 ^{1,
,}

1.
中国地质大学(武汉)材料科学与化学学院, 太阳燃料实验室, 湖北武汉 430078
2.
Department of Chemical Engineering and Applied Chemistry, University of Toronto, Toronto ON, M5S3E5, Canada

通讯作者: Email: weilai.yu@utoronto.ca (余维来); liutao54@cug.edu.cn (刘涛)

摘要: 以玉米酒糟为原料制备的硬碳(HC)是一种可持续、低成本钠离子电池(SIBs)负极候选材料，但其实际应用一直受限于其不足的可逆容量。本研究报道一种温度梯度处理法，该方法可精确调控玉米酒糟衍生硬碳的层间距、孔隙率和石墨化程度，从而获得卓越的电化学性能。优化后的材料具有0.378 nm层间距和1.68 nm主孔径，展现出优异的高倍率性能：在1.0和2.0 A g^-1电流密度下分别实现289与198 mAh g^-1的比容量，且在2.0 A g^-1下循环700次后容量保持率达83%。通过原位X射线衍射与非原位拉曼光谱联用，揭示出“吸附-插层协同孔隙填充”的独特储钠机制，该机制有助于解释其快速动力学特性和长循环稳定性。这些结果表明，通过精准调控生物质衍生硬碳的结构策略，可实现实用化SIB负极所需的容量、倍率性能和循环寿命——使这种储量丰富、源自废弃物的材料大幅迈向商业化。

关键词:

English

Corn-distillers-derived hard carbon: a sustainable high-rate, long-life anode for sodium-ion batteries

Xue Zhang ^1, ,
Zihan He ^1, ,
Yingqi Wu ^1, ,
Weilai Yu ^{2,
,} ,
Tao Liu ^{1,
,}

1.
Laboratory of Solar Fuel, Faculty of Materials Science and Chemistry, China University of Geosciences, Wuhan 430078, Hubei Proivince, China
2.
Department of Chemical Engineering and Applied Chemistry, University of Toronto, Toronto ON, M5S3E5, Canada

Corresponding author: Email: weilai.yu@utoronto.ca (Weilai Yu); liutao54@cug.edu.cn (Tao Liu)

Received Date: 29 August 2025
Accepted Date: 29 September 2025
Revised Date: 28 September 2025
Available Online: 15 May 2026

Abstract: Hard carbon (HC) derived from corn-distillers is a sustainable, affordable anode candidate for sodium-ion batteries (SIBs), yet its practical deployment has been limited by insufficient reversible capacity. Here we report a temperature-gradient treatment that precisely tailors interlayer spacing, porosity, and graphitization in corn-distillers-derived hard carbon, unlocking exceptional electrochemical performance. The optimized material exhibits an interlayer spacing of 0.378 nm and a dominant pore size of 1.68 nm. It demonstrates outstanding high-rate behavior, achieving 289 and 198 mAh g^-1 at 1.0 and 2.0 A g^-1, respectively. Additionally, it retains 83% of its capacity after 700 cycles at 2.0 A g^-1. Integrating in situ X-ray diffraction with ex situ Raman spectroscopy demonstrates a unique sodium-storage mechanism characterized by both "adsorption–intercalation and pore-filling". This approach helps elucidate the rapid kinetics and long-lasting performance. These results demonstrate that controlled structural tactics of biomass-derived HC can achieve the desired capacity, rate capability, and longevity required for practical SIB anodes—bringing an abundant, waste-derived feedstock dramatically closer to commercialization.

Key words:

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沈阳化工大学材料科学与工程学院沈阳 110142

玉米酒糟衍生硬碳：一种可持续的高倍率、长寿命钠离子电池负极材料

通讯作者: Email: weilai.yu@utoronto.ca (余维来); liutao54@cug.edu.cn (刘涛)

English

Corn-distillers-derived hard carbon: a sustainable high-rate, long-life anode for sodium-ion batteries

Corresponding author: Email: weilai.yu@utoronto.ca (Weilai Yu); liutao54@cug.edu.cn (Tao Liu)

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玉米酒糟衍生硬碳：一种可持续的高倍率、长寿命钠离子电池负极材料

通讯作者: Email: weilai.yu@utoronto.ca (余维来); liutao54@cug.edu.cn (刘涛)

English

Corn-distillers-derived hard carbon: a sustainable high-rate, long-life anode for sodium-ion batteries

Corresponding author: Email: weilai.yu@utoronto.ca (Weilai Yu); liutao54@cug.edu.cn (Tao Liu)

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CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs