迈向实用的圆偏振发光：基于碳点的圆偏振激光器

引用本文: 历婷, 曾孝, 杨玉卓, 温新懿, 丁树荣, 石林林, 张永强, 卢思宇. 迈向实用的圆偏振发光：基于碳点的圆偏振激光器[J]. 物理化学学报, 2026, 42(4): 100191. doi: 10.1016/j.actphy.2025.100191 shu

Citation: Ting Li, Xiao Zeng, Yuzhuo Yang, Xinyi Wen, Shurong Ding, Linlin Shi, Yongqiang Zhang, Siyu Lu. Towards practical circularly polarized luminescence: carbon dots-based circularly polarized lasers[J]. Acta Physico-Chimica Sinica, 2026, 42(4): 100191. doi: 10.1016/j.actphy.2025.100191 shu

迈向实用的圆偏振发光：基于碳点的圆偏振激光器

郑州大学化学学院, 平原实验室, 河南郑州 450001

通讯作者: Email: linlinshi@zzu.edu.cn (石林林); zhangyongqiang@zzu.edu.cn (张永强); sylu2013@zzu.edu.cn (卢思宇)

摘要: 圆偏振发光(CPL)在量子计算、3D显示和生物成像等领域具有重要应用价值，但其实际应用面临不对称因子低、发光亮度低、方向性差和发射谱宽等挑战。为解决这些问题，圆偏振激光技术通过受激辐射放大和谐振腔模式选择，可显著提升CPL性能，实现高g值(接近理论极限2)、高亮度、窄线宽和强方向性的圆偏振光输出。目前，有机微晶、钙钛矿等材料虽能实现高g值圆偏振激光，但仍存在制备复杂、生物相容性差等问题。相比之下，碳点(CDs)因其制备简单、成本低、毒性小、易修饰和生物相容性好等优势，成为极具潜力的新型圆偏振增益介质。本文系统综述了圆偏振激光的材料体系、器件类型及应用进展，重点探讨了CDs作为增益介质的优势及其在3D显示、光学通信、信息加密和生物传感等领域的潜力，并展望了CDs圆偏振激光的未来发展方向和挑战，为推动高性能圆偏振激光器件的实用化进程提供了参考。

关键词:

English

Towards practical circularly polarized luminescence: carbon dots-based circularly polarized lasers

School of Chemistry, Pingyuan Laboratory, Zhengzhou University, Zhengzhou 450001, Henan Province, China

Corresponding author: Email: linlinshi@zzu.edu.cn (Linlin Shi); zhangyongqiang@zzu.edu.cn (Yongqiang Zhang); sylu2013@zzu.edu.cn (Siyu Lu)

Received Date: 31 July 2025
Accepted Date: 23 September 2025
Revised Date: 15 September 2025
Available Online: 15 April 2026

Abstract: Circularly polarized luminescence (CPL) has significant application value in fields such as quantum computing, three-dimensional (3D) display, and bioimaging. However, its practical application faces challenges including low dissymmetry factor (g), insufficient quantum yield, poor directionality, and broad emission spectrum. To address these issues, circularly polarized laser technology can significantly enhance CPL performance through stimulated emission amplification and resonant cavity mode selection, achieving circularly polarized light output with high g (close to the theoretical limit of 2), high brightness, narrow linewidth, and strong directionality. Currently, although materials like organic microcrystals and perovskites can realize circularly polarized laser with high g, they still have problems such as complex preparation and poor biocompatibility. In contrast, carbon dots (CDs) have emerged as a highly promising new type of circularly polarized gain medium due to their advantages of simple preparation, low cost, low toxicity, easy modification, and good biocompatibility. This paper systematically reviews the material systems, device types, and application progress of circularly polarized laser, focusing on the advantages of CDs as gain media and their potential in fields such as 3D display, optical communication, information encryption, and biosensing. It also prospects the future development directions and challenges of CDs-based circularly polarized lasers, providing a reference for promoting the practical application process of high-performance circularly polarized laser devices.

Key words:

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沈阳化工大学材料科学与工程学院沈阳 110142

迈向实用的圆偏振发光：基于碳点的圆偏振激光器

通讯作者: Email: linlinshi@zzu.edu.cn (石林林); zhangyongqiang@zzu.edu.cn (张永强); sylu2013@zzu.edu.cn (卢思宇)

English

Towards practical circularly polarized luminescence: carbon dots-based circularly polarized lasers

Corresponding author: Email: linlinshi@zzu.edu.cn (Linlin Shi); zhangyongqiang@zzu.edu.cn (Yongqiang Zhang); sylu2013@zzu.edu.cn (Siyu Lu)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

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CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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中国化学会秘书处

迈向实用的圆偏振发光：基于碳点的圆偏振激光器

通讯作者: Email: linlinshi@zzu.edu.cn (石林林); zhangyongqiang@zzu.edu.cn (张永强); sylu2013@zzu.edu.cn (卢思宇)

English

Towards practical circularly polarized luminescence: carbon dots-based circularly polarized lasers

Corresponding author: Email: linlinshi@zzu.edu.cn (Linlin Shi); zhangyongqiang@zzu.edu.cn (Yongqiang Zhang); sylu2013@zzu.edu.cn (Siyu Lu)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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