Citation: Qiang Cheng, Jingping Li, Zhendong Ke, Jiaming Li, Kai Wang. Advanced oxidation technology synergistic photothermal degradation of antibiotics over inorganic/organic S-scheme heterojunction[J]. Acta Physico-Chimica Sinica, ;2026, 42(5): 100187. doi: 10.1016/j.actphy.2025.100187 shu

Advanced oxidation technology synergistic photothermal degradation of antibiotics over inorganic/organic S-scheme heterojunction

Qiang Cheng ¹ ,
Jingping Li ¹ ,
Zhendong Ke ^2,, ,
Jiaming Li ¹ ,
Kai Wang ^1,,

1.
College of Urban and Environmental Sciences, Huangshi Key Laboratory of Prevention and Control of Soil Pollution, Hubei Normal University, Huangshi 435002, Hubei Province, China
2.
Huangshi Ecological Environment Monitoring Center, Department of Ecology and Environment of Hubei Province, Huangshi 435000, Hubei Province, China

Corresponding author: Zhendong Ke, 13807231662@163.com Kai Wang, wangkai@hbnu.edu.cn
Received Date: 21 August 2025
Revised Date: 14 September 2025
Accepted Date: 14 September 2025

The rational engineering of inorganic/organic catalysts capable of concomitant utilization of solar energy and advanced oxidation processes (AOPs) holds significant promise for the degradation of antibiotic contaminants. The study developed MoO_2-x/g-C₃N₄ (MOCN) S-scheme heterojunctions with oxygen vacancies using an ultrasonic-assisted integration technique, employing them as solar-driven peroxymonosulfate (PMS) catalysts for the degradation of antibiotics. The formation of an internal electric field between MoO_2-x and g-C₃N₄, along with the charge transfer pathway in the S-scheme heterojunction, was confirmed using density functional theory, femtosecond transient absorption spectroscopy, and in-situ XPS analysis. Meanwhile, the oxygen vacancy and photothermal effect of the MOCN heterojunction further accelerate the electron migration rate. The optimized MOCN-2 catalyst achieved 90.9 % tetracycline (TC) removal within 20 min compared to pristine MoO_2-x and g-C₃N₄. Continuous flow experiments and bactericidal activity experiments together validated the practical feasibility of this catalyst for water treatment applications. The analysis above led to the proposal of a possible mechanism for TC degradation. This research brings forward new strategies for the synthesis of S-scheme heterojunctions to improve wastewater treatment.
- Advanced oxidation technology,
- Inorganic/organic heterojunction,
- S-scheme mechanism,
- Antibiotics degradation,
- Photothermal effect
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沈阳化工大学材料科学与工程学院沈阳 110142