双内建电场驱动的D-A COFs/ZnIn2S4 S型异质结加速电荷分离实现纯水中高效光合成H2O2

引用本文: 郭杰, 薛丽君, 宋发辉, 李程鹏, 陈卓, 温丽丽. 双内建电场驱动的D-A COFs/ZnIn₂S₄ S型异质结加速电荷分离实现纯水中高效光合成H₂O₂[J]. 物理化学学报, 2026, 42(4): 100177. doi: 10.1016/j.actphy.2025.100177 shu

Citation: Jie Guo, Lijun Xue, Fahui Song, Chengpeng Li, Zhuo Chen, Lili Wen. Dual built-in electric field-driven S-scheme heterojunction of D-A COFs/ZnIn₂S₄ for accelerated charge separation toward high-efficiency H₂O₂ photosynthesis in pure water[J]. Acta Physico-Chimica Sinica, 2026, 42(4): 100177. doi: 10.1016/j.actphy.2025.100177 shu

双内建电场驱动的D-A COFs/ZnIn₂S₄ S型异质结加速电荷分离实现纯水中高效光合成H₂O₂

华中师范大学化学学院, 光能利用与减污降碳教育部工程研究中心, 湖北武汉 430079

通讯作者: Email: czdwd@mails.ccnu.edu.cn (陈卓); wenlili@ccnu.edu.cn (温丽丽)

摘要: 构建双内建电场(IEF)驱动的S型异质结为光催化H₂O₂生产中的高效电荷分离与利用提供了一种极具前景的策略。本文报道了一种基于供体-受体共价有机框架(D-A COFs) TpAQ (由三醛基间苯三酚(Tp)和2, 6-二氨基蒽醌(AQ)合成)与ZnIn₂S₄ (ZIS)构筑的双IEF驱动的S型异质结，其中双内建电场分别源自异质结界面和D-A COFs中的D-A界面。值得注意的是，通过同时利用氧还原反应和水氧化反应路径，优化后的TpAQ/ZIS-10在纯水中的可见光驱动产H₂O₂速率达到2362 μmol g⁻¹ h⁻¹，显著高于单一组分TpAQ和ZIS。此外，实验结果与理论计算共同表明，TpAQ/ZIS异质结中双IEF的协同效应显著促进了载流子的传输与分离。本研究为构建具有双IEF的高效S型异质结提供了宝贵见解。

关键词:

English

Dual built-in electric field-driven S-scheme heterojunction of D-A COFs/ZnIn₂S₄ for accelerated charge separation toward high-efficiency H₂O₂ photosynthesis in pure water

Engineering Research Center of Photoenergy Utilization for Pollution Control and Carbon Reduction, Ministry of Education; College of Chemistry, Central China Normal University, Wuhan 430079, Hubei Province, China

Corresponding author: Email: czdwd@mails.ccnu.edu.cn (Chen Zhuo); wenlili@ccnu.edu.cn (Wen Lili)

Received Date: 29 July 2025
Accepted Date: 31 August 2025
Revised Date: 28 August 2025
Available Online: 15 April 2026

Abstract: The construction of dual built-in electric field (IEF)-driven S-scheme heterojunctions presents a promising strategy to accelerate efficient charge separation and improve charge utilization in photocatalytic H₂O₂ production. Herein, we report, the construction of a heterojunction based on donor-acceptor covalent organic frameworks (D-A COFs) TpAQ (synthesized from two monomers: 1, 3, 5-triformylphloroglucinol (Tp) and 2, 6-diaminoanthraquinone (AQ)) and ZnIn₂S₄ (ZIS), realizing a dual IEF-driven S-scheme heterojunction—one from the heterojunction interface and another from D-A interface within D-A COFs. In particular, the optimized TpAQ/ZIS-10 exhibits a significantly higher visible-light driven photocatalytic H₂O₂ production rate of 2362 μmol g⁻¹ h⁻¹ in pure water than TpAQ and ZIS by utilizing both the oxygen reduction reaction and water oxidation reaction pathways. Furthermore, the experimental results and theoretical calculations revealed that the synergistic effect of dual IEF in TpAQ/ZIS heterojunction significantly facilitates efficient charge carrier transfer and separation. This work provides valuable insight for constructing highly efficient S-scheme heterojunctions with dual IEF.

Key words:

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1.
沈阳化工大学材料科学与工程学院沈阳 110142

双内建电场驱动的D-A COFs/ZnIn₂S₄ S型异质结加速电荷分离实现纯水中高效光合成H₂O₂

通讯作者: Email: czdwd@mails.ccnu.edu.cn (陈卓); wenlili@ccnu.edu.cn (温丽丽)

English

Dual built-in electric field-driven S-scheme heterojunction of D-A COFs/ZnIn₂S₄ for accelerated charge separation toward high-efficiency H₂O₂ photosynthesis in pure water

Corresponding author: Email: czdwd@mails.ccnu.edu.cn (Chen Zhuo); wenlili@ccnu.edu.cn (Wen Lili)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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