Citation: Yingtong Shi, Guotong Xu, Guizeng Liang, Di Lan, Siyuan Zhang, Yanru Wang, Daohao Li, Guanglei Wu. PEG-VN modified PP separator for high-stability and high-efficiency lithium-sulfur batteries[J]. Acta Physico-Chimica Sinica, ;2025, 41(7): 100082. doi: 10.1016/j.actphy.2025.100082 shu

PEG-VN modified PP separator for high-stability and high-efficiency lithium-sulfur batteries

1.
State Key Laboratory of Bio-fibers and Eco-textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, Shandong Province, China;
2.
Qingdao Engineering Research Center for New Metallic Functional Materials, Characteristic Laboratory of Advanced Metal Functional Materials and Processing in Universities of Shandong, Qingdao Binhai University, Qingdao 266555, Shandong Province, China;
3.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China;
4.
School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710072, Shaanxi Province, China

Received Date: 17 January 2025
Revised Date: 14 March 2025
Accepted Date: 18 March 2025

Fund Project: The project was supported by the National Natural Science Foundation of China (52302272, 52377026), Taishan Scholars and Young Experts Program of Shandong Province (tsqn202211124, tsqn202103057), the Natural Science Foundation of Shandong Province (ZR2022QB023, ZR2024ME046), the Qingchuang Talents Induction Program of Shandong Higher Education Institution (Research and Innovation Team of Marine Polysaccharides Fibers-based Energy Materials), the State Key Laboratory of Bio-Fibers and Eco-Textiles, Qingdao University (ZKT10, GZRC202006).

Lithium-sulfur (Li-S) batteries are regarded as one of the most promising candidates for next generation energy storage systems due to their high theoretical energy density. However, the practical application of Li-S batteries is limited by the low lithium ion (Li⁺) transport efficiency and the rapid capacity decay caused by the shuttle effect. Herein, we report a composite comprising Polyethylene glycol (PEG) and vanadium nitride (VN) nanosheets coated onto a commercial polypropylene (PP) separator, called PEG-VN@PP separator. The supercatalytic effect and adsorption properties exhibited by the VN nanosheets significantly enhance the conversion of polysulfides, thereby improving both the capacity and stability of Li-S batteries. Due to the coating of PEG, lithium ions are attracted to the polar functional groups, enabling selective transport, which improves the transport efficiency of Li⁺ and the rate capability of Li-S batteries. The Li-S battery assembled with PEG-VN@PP exhibits a high specific capacity of 782.0 mAh·g^-1 and an average capacity decay of 0.048% per cycle at 1C (1675 mA·g^-1) for 700 cycles, using the carbon nanotubes/sulfur cathode with a sulfur mass loading of 1.2 mg·cm^-2.
- Vanadium nitride,
- Polyethylene glycol,
- Separator modification,
- Shuttle effect,
- Lithium-sulfur batteries
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沈阳化工大学材料科学与工程学院沈阳 110142

PEG-VN modified PP separator for high-stability and high-efficiency lithium-sulfur batteries

南开大学师唯/华北电力大学（保定）刘景维：二维配位聚合物中有序的亲锂冠醚位点用于无枝晶锂沉积

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