Citation: Yihan Xue, Xue Han, Jie Zhang, Xiaoru Wen. Efficient capacitive desalination over NCQDs decorated FeOOH composite[J]. Acta Physico-Chimica Sinica, ;2025, 41(7): 100072. doi: 10.1016/j.actphy.2025.100072 shu

Efficient capacitive desalination over NCQDs decorated FeOOH composite

College of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, Inner Mongolia Autonomous Region, China

Received Date: 12 December 2024
Revised Date: 26 January 2025
Accepted Date: 24 February 2025

Fund Project: The project was supported by the Natural Science Foundation of Inner Mongolia Autonomous Region of China (2023MS02010) and the Program for Young Talents of Science and Technology in Universities of Inner Mongolia Autonomous Region (NJYT23032).

Capacitive deionization (CDI) is emerging as a novel technology for seawater purification, with the electrode material playing a crucial role in desalination performance. In this study, we designed a nitrogen-doped carbon quantum dots decorated iron oxide hydroxide (NCQDs/FeOOH) composite by a facile hydrothermal strategy and investigated as the CDI cathode for desalination application. Microstructural analyses reveal that the composite features a relatively uniform nanoparticle-assembled network, hierarchical pore alignment, and abundant porosity. Electrochemical tests confirm its outstanding capacitance property and conductivity. In an initial NaCl aqueous solution of 2000 mg·L^-1 at an applied potential of 1.4 V, the GAC_NaCl of NCQDs/FeOOH hybrid electrode reaches 56.52 mg·g^-1, along with remarkable cycling durability. Furthermore, the CV (cyclic voltammetry) and ex situ XPS (X-ray photoelectron spectroscopy) characterizations indicate the predominantly pseudocapacitive desalination mechanism.
- Carbon quantum dots,
- FeOOH,
- Composite material,
- CDI desalination,
- Durability
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