Citation: Kun Rong, Cuilian Wen, Jiansen Wen, Xiong Li, Qiugang Liao, Siqing Yan, Chao Xu, Xiaoliang Zhang, Baisheng Sa, Zhimei Sun. Hierarchical MoS₂/Ti₃C₂T_x heterostructure with excellent photothermal conversion performance for solar-driven vapor generation[J]. Acta Physico-Chimica Sinica, ;2025, 41(6): 100053. doi: 10.1016/j.actphy.2025.100053 shu

Hierarchical MoS₂/Ti₃C₂T_x heterostructure with excellent photothermal conversion performance for solar-driven vapor generation

1.
Materials Genome Institute, School of Materials Science and Engineering, Fuzhou University, Fuzhou 350100, Fujian Province, China;
2.
School of Materials Science and Engineering, Beihang University, Beijing 100191, China;
3.
Xiamen Talentmats New Materials Science & Technology Co., Ltd., Xiamen 361015, Fujian Province, China

Received Date: 26 November 2024
Revised Date: 7 January 2025
Accepted Date: 21 January 2025

Fund Project: The project was supported by the National Key Research and Development Program of China (2022YFB3807200), the National Natural Science Foundation of China (52332005), and the Natural Science Foundation of Fujian Province (2024J01262).

Metallic 1T Molybdenum disulfide (1T-MoS₂) exhibits enhanced full spectral light absorption and prominent electrical conductivity, making it ideal for photothermal applications in conjunction with Ti₃C₂T_x MXene. Despite the challenges in increasing the 1T-MoS₂ proportion within MoS₂/Ti₃C₂T_x heterostructures and the incomplete understanding of the mechanisms governing their formation and properties, herein, a combined theoretical and experimental framework has been established, suggesting that the metallic characteristics of Ti₃C₂T_x and 1T-MoS₂ could significantly improve photothermal performance through strong interlayer interactions and efficient electron transport. The hierarchical MoS₂/Ti₃C₂T_x heterostructure has been fabricated through a one-step hydrothermal synthesis method with enhanced 1T-MoS₂ proportion, which achieves multilayered wrinkled architecture resulting from the in-situ growth of MoS₂ on Ti₃C₂T_x nanosheets. Notably, a remarkable peak photoheating temperature of 107 °C under an 808 nm laser with an intensity of 0.5 W·cm^-2 is realized, demonstrating its exceptional photothermal conversion capability. By incorporated into a polyvinylidene difluoride membrane, the MoS₂/Ti₃C₂T_x heterostructure functions as an efficient self-floating solar-driven steam generator, reaching an evaporation rate of 1.79 kg·m^-2·h^-1 and an evaporation efficiency of 96.4% under one solar irradiance. This study proposes a versatile strategy for the MoS₂/Ti₃C₂T_x heterostructure, offering the potential for sustainable solar-driven vapor generation technologies.
- MXene,
- Molybdenum disulfide,
- Heterostructure,
- Photothermal conversion,
- Solar-driven vapor generation
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Hierarchical MoS2/Ti3C2Tx heterostructure with excellent photothermal conversion performance for solar-driven vapor generation

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通讯作者: 陈斌, bchen63@163.com

Hierarchical MoS₂/Ti₃C₂T_x heterostructure with excellent photothermal conversion performance for solar-driven vapor generation