Citation: Xue Liu, Lipeng Wang, Luling Li, Kai Wang, Wenju Liu, Biao Hu, Daofan Cao, Fenghao Jiang, Junguo Li, Ke Liu. Cu基和Pt基甲醇水蒸气重整制氢催化剂研究进展[J]. Acta Physico-Chimica Sinica, ;2025, 41(5): 100049. doi: 10.1016/j.actphy.2025.100049 shu

Cu基和Pt基甲醇水蒸气重整制氢催化剂研究进展

Xue Liu ¹ ,
Lipeng Wang ¹ ,
Luling Li ² ,
Kai Wang ³ ,
Wenju Liu ¹ ,
Biao Hu ¹ ,
Daofan Cao ¹ ,
Fenghao Jiang ¹ ,
Junguo Li ¹ ,
Ke Liu ^1,4

1.
Department of Chemistry, College of Science, Southern University of Science and Technology, Shenzhen 518055, Guangdong Province, China;
2.
Shenzhen Gas Group Co Ltd. Shenzhen 518000, Guangdong Province, China;
3.
Anyang Institute of Technology, Anyang 455099, Henan Province, China;
4.
College of Innovation and Entrepreneurship, Southern University of Science and Technology, Shenzhen 518055, Guangdong Province, China

Received Date: 18 November 2024
Revised Date: 13 December 2024
Accepted Date: 20 December 2024

Fund Project: The project was supported by Shenzhen Science and Technology Program, Shenzhen Science and Technology Innovation Committee (KQTD20180411143418361), Shenzhen Gas & SUSTech Joint Energy Lab, Southern University of Science and Technology, Guangdong Provincial Key Laboratory of Catalysis (2020B121201002), Key Scientific Research Project of Colleges and Universities in Henan Province (24B530001) and National Natural Science Foundation of China (U22B20149).

甲醇水蒸气重整(methanol steam reforming, MSR)反应是实现甲醇在线制氢的重要途径，在清洁能源应用中具有重要作用。MSR反应中的催化性能直接影响氢气产量和副产物组成，其中Cu基和Pt基催化剂被广泛研究。其催化机制主要涉及甲醇和水分子中C―H和O―H键的断裂。Cu基催化剂的活性依赖于Cu⁰和Cu⁺位点的比例及协同作用，Pt基催化剂则通过Pt⁰、Pt^δ⁺或Pt²⁺活性位点与氧空位的相互作用发挥作用。然而，活性金属与载体之间的电子转移及相互作用机制仍存争议，影响金属价态、吸附位点及反应路径选择，特别是在甲醇脱氢生成中间产物(如甲醛、甲酸和甲酸甲酯)的反应路径上，尚未形成统一认识。本文总结了Cu⁰与Cu⁺的单位点与协同位点机制，探讨了Pt基催化剂的直接路径与协同路径，分析In₂O₃等对Pt位点调控及氧空位生成的促进作用。通过催化性能评估与机理研究，提出了优化催化剂活性和稳定性的策略。本综述不仅深化了对MSR反应机理的理解，还为高效催化剂的设计提供了理论基础和研究方向。
- Hydrogen production of methanol steam reforming,
- Cu-based and Pt-Based catalysts,
- Active sites,
- Synergies,
- Reaction pathways
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