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Citation: Mu-yao LIU, Jian-yun WANG, Lian DUAN, Xian LIU, Lei ZHANG. Nickel oxide modified C3N5 photocatalyst for enhanced hydrogen evolution performance[J]. Journal of Fuel Chemistry and Technology, ;2022, 50(2): 243-249. doi: 10.1016/S1872-5813(21)60166-4 shu

Nickel oxide modified C3N5 photocatalyst for enhanced hydrogen evolution performance

  • 1.

    School of Chemistry and Chemical Engineering, Taiyuan University of Technology, Taiyuan 030024, China

  • 2.

    Department of Chemistry, Taiyuan Normal University, Jinzhong 030619, China

  • 3.

    Shenzhen Huace International Certification Co., Ltd, Shenzhen 518101, China

Figures(8)

  • Recently, a new carbon nitride (C3N5) photocatalyst has attracted much attention due to its excellent light harvesting and unique 2D structure. However, high recombination rates of electron-hole pairs of bulk C3N5 serious affect the photocatalytic performance. Herein, nickel oxide (NiO) modified C3N5 p-n junctions photocatalyst was synthesized by a facile hydrothermal method. Results indicated that the 9-Ni/C3N5 nanosheet photocatalyst showed excellent hydrogen production efficiency under visible light. The hydrogen production rate reached 357 μmol/(g·h), which was 107-fold higher than that of pristine C3N5. The high catalytic performace was attributed to the 9-Ni/C3N5 p-n junctions which could efficiently promote photogenerated electron-hole pair separation and thus promote the hydrogen evolution reaction.
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