Citation: Yajuan Ma, Zemei Wang, Xiaofeng Xu, Jingyu Wang. Review on porous nanomaterials for adsorption and photocatalytic conversion of CO₂[J]. Chinese Journal of Catalysis, ;2017, 38(12): 1956-1969. doi: 10.1016/S1872-2067(17)62955-3 shu

Review on porous nanomaterials for adsorption and photocatalytic conversion of CO₂

Key Laboratory of Material Chemistry for Energy Conversion and Storage(Ministry of Education), School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei, China

Received Date: 11 October 2017
Revised Date: 31 October 2017

Fund Project: This work was supported by the National Natural Science Foundation of China (21771070, 21571071).

Photocatalytic conversion of "greenhouse gas" CO₂ is considered to be one of the most effective ways to alleviate current energy and environmental problems without additional energy consumption and pollutant emission. The performance of many traditional semiconductor photocatalysts is not efficient enough to satisfy the requirements of practical applications because of their limited specific surface area and low CO₂ adsorption capacity. Therefore, the exploration of photocatalysts with high CO₂ uptake is significant in the field of CO₂ conversion. Recently the porous materials appeared to be a kind of superior candidate for enriching the CO₂ molecules on the surface of photocatalysts for catalytic conversion. This paper first summarizes the advances in the development of nanoporous adsorbents for CO₂ capture. Three main classes of porous materials are considered:inorganic porous materials, metal organic frameworks, and microporous organic polymers. Based on systematic research on CO₂ uptake, we then highlight the recent progress in these porous-material-based photocatalysts for CO₂ conversion. Benefiting from the improved CO₂ uptake capacity, the porous-material-based photocatalysts exhibited remarkably enhanced efficiency in the reduction of CO₂ to chemical fuels, such as CO, CH₄, and CH₃OH. Based on reported recent achievements, we predict a trend of development in multifunctional materials with both high adsorption capability and photocatalytic performance for CO₂ utilization.
- Porous material,
- Composite nanostructure,
- CO₂ adsorption,
- Photocatalysis,
- CO₂ conversion
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通讯作者: 陈斌, bchen63@163.com

Review on porous nanomaterials for adsorption and photocatalytic conversion of CO₂