Citation: Rengui Li. Latest progress in hydrogen production from solar water splitting via photocatalysis, photoelectrochemical, and photovoltaic-photoelectrochemical solutions[J]. Chinese Journal of Catalysis, ;2017, 38(1): 5-12. doi: 10.1016/S1872-2067(16)62552-4 shu

Latest progress in hydrogen production from solar water splitting via photocatalysis, photoelectrochemical, and photovoltaic-photoelectrochemical solutions

Rengui Li ^a,b,

a Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;
b State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China

Received Date: 30 August 2016
Revised Date: 25 September 2016

Fund Project: This work was supported by the National Basic Research Program of the Ministry of Science and Technology (973 Program, 2014CB239400), the National Natural Science Foundation of China (21501236, 21673230), and Youth Innovation Promotion Association of Chinese Academy of Sciences (2016167).

Hydrogen production via solar water splitting is regarded as one of the most promising ways to utilize solar energy and has attracted more and more attention. Great progress has been made on photocatalytic water splitting for hydrogen production in the past few years. This review summa-rizes the very recent progress (mainly in the last 2-3 years) on three major types of solar hydrogen production systems:particulate photocatalysis (PC) systems, photoelectrochemical (PEC) systems, and photovoltaic-photoelectrochemical (PV-PEC) hybrid systems. The solar-to-hydrogen (STH) conversion efficiency of PC systems has recently exceeded 1.0% using a SrTiO₃:La,Rh/Au/BiVO₄:Mo photocatalyst, 2.5% for PEC water splitting on a tantalum nitride photoanode, and reached 22.4% for PV-PEC water splitting using a multi-junction GaInP/GaAs/Ge cell and Ni electrode hybrid sys-tem. The advantages and disadvantages of these systems for hydrogen production via solar water splitting, especially for their potential demonstration and application in the future, are briefly de-scribed and discussed. Finally, the challenges and opportunities for solar water splitting solutions are also forecasted.
- Solar energy utilization,
- Photocatalysis,
- Water splitting for hydrogen production,
- Charge separation
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