Citation: Jing Liu, Ping Song, Mingbo Ruan, Weilin Xu. Catalytic properties of graphitic and pyridinic nitrogen doped on carbon black for oxygen reduction reaction[J]. Chinese Journal of Catalysis, ;2016, 37(7): 1119-1126. doi: 10.1016/S1872-2067(16)62456-7 shu

Catalytic properties of graphitic and pyridinic nitrogen doped on carbon black for oxygen reduction reaction

Jing Liu ^a,b, ,
Ping Song ^a ,
Mingbo Ruan ^a ,
Weilin Xu ^a

a. State Key Laboratory of Electroanalytical Chemistry, Jilin Province Key Laboratory of Low Carbon Chemical Power, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, Jilin, China;
b. University of Chinese Academy of Sciences, Beijing 100049, China

Received Date: 20 March 2016
Revised Date: 11 May 2016

Fund Project: This work was supported by the National Basic Research Program of China (973 Program, 2012CB932800, 2014CB932700), the National Natural Science Foundation of China (21422307, 21303180, 21433003, 21503212, 21503211), and the "Recruitment Program of Global Youth Experts" of China.

Pure graphitic nitrogen (G-N) was doped on carbon black by Hummers method and a following heat treatment was used to transform the G-N to pyridinic (P)-N. An oxygen reduction reaction (ORR) study showed that the G-N site doped on carbon gave a two-electron ORR with H₂O₂ as the main product, while the P-N site gave the four-electron process of ORR and decreased the production of H₂O₂. The results help the understanding and design of doped N-based ORR electrocatalysts.
- Carbon black,
- Heat-treatment,
- Oxygen reduction reaction,
- Nitrogen doping,
- Carbon-based catalysts
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