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Citation: Ruimei Fang, Yajuan Cui, Zhonghua Shi, Maochu Gong, Yaoqiang Chen. Promotion of a Pd/Al2O3 close-coupled catalyst by Ni[J]. Chinese Journal of Catalysis, ;2015, 36(7): 994-1000. doi: 10.1016/S1872-2067(15)60850-6 shu

Promotion of a Pd/Al2O3 close-coupled catalyst by Ni

  • 1.

    a College of Chemical Engineering, Sichuan University, Chengdu 610064, Sichuan, China;

  • Corresponding author: Zhonghua Shi,  Yaoqiang Chen, 
  • Received Date: 5 February 2015
    Available Online: 26 March 2015

    Fund Project: 国家自然科学基金(21173153) (21173153) 四川省科技厅科技支撑项目(2014SZ0143). (2014SZ0143)

  • The influence of a nickel promoter on the catalytic behavior of a modified alumina supported Pd close-coupled catalyst was investigated. Doping with nickel improved the catalytic activity for the reactions of C3H8, especially over the aged catalyst. T50 and T90 of the aged Pd catalyst were decreased by 31 and 30 ℃, respectively. The single reaction results revealed that doping with Ni promoted the catalytic activity for the C3H8 + NO reaction. The fresh and aged catalysts were characterized by H2-temperature-programmed reduction, CO chemisorption, high resolution transmission electron microscopy, and X-ray photoelectron spectroscopy, which revealed that the doping with Ni inhibited the sintering of active PdOx species and the formation of undesired metallic Pd0, and led to improved reducibility of active PdOx and increased the surface area of PdOx species.
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