Advanced Search

Citation: Ruimei Fang, Yajuan Cui, Zhonghua Shi, Maochu Gong, Yaoqiang Chen. Promotion of a Pd/Al2O3 close-coupled catalyst by Ni[J]. Chinese Journal of Catalysis, ;2015, 36(7): 994-1000. doi: 10.1016/S1872-2067(15)60850-6 shu

Promotion of a Pd/Al2O3 close-coupled catalyst by Ni

  • 1.

    a College of Chemical Engineering, Sichuan University, Chengdu 610064, Sichuan, China;

  • Corresponding author: Zhonghua Shi,  Yaoqiang Chen, 
  • Received Date: 5 February 2015
    Available Online: 26 March 2015

    Fund Project: 国家自然科学基金(21173153) (21173153) 四川省科技厅科技支撑项目(2014SZ0143). (2014SZ0143)

  • The influence of a nickel promoter on the catalytic behavior of a modified alumina supported Pd close-coupled catalyst was investigated. Doping with nickel improved the catalytic activity for the reactions of C3H8, especially over the aged catalyst. T50 and T90 of the aged Pd catalyst were decreased by 31 and 30 ℃, respectively. The single reaction results revealed that doping with Ni promoted the catalytic activity for the C3H8 + NO reaction. The fresh and aged catalysts were characterized by H2-temperature-programmed reduction, CO chemisorption, high resolution transmission electron microscopy, and X-ray photoelectron spectroscopy, which revealed that the doping with Ni inhibited the sintering of active PdOx species and the formation of undesired metallic Pd0, and led to improved reducibility of active PdOx and increased the surface area of PdOx species.
  • 加载中
    1. [1]

      [1] Gandhi H S, Graham G W, McCabe R W. J Catal, 2003, 216: 433

    2. [2]

      [2] Kašpar J, Fornasiero P, Hickey N. Catal Today, 2003, 77: 419

    3. [3]

      [3] Li M, Wu X D, Wan J, Liu S, Ran R, Weng D. Catal Today, 2015, 242: 322

    4. [4]

      [4] Lan L, Chen S H, Zhao M, Gong M C, Chen Y Q. J Mol Catal A, 2014, 394: 10

    5. [5]

      [5] Yao Y L, Fang R M, Shi Z H, Gong M C, Chen Y Q. Chin J Catal (姚艳玲, 方瑞梅, 史忠华, 龚茂初, 陈耀强. 催化学报), 2011, 32: 589

    6. [6]

      [6] Wang G, You R, Meng M. Fuel, 2013, 103: 799

    7. [7]

      [7] Neyertz C, Volpe M, Gigola C. Appl Catal A, 2004, 277: 137

    8. [8]

      [8] Spinicci R, Tofanari A. Appl Catal A, 2002, 227: 159

    9. [9]

      [9] Dong L. Chin J Catal (董林. 催化学报), 2009, 30: 1150

    10. [10]

      [10] Hungría A B, Calvino J J, Anderson J A, Martínez-Arias A. Appl Catal B, 2006, 62: 359

    11. [11]

      [11] Pan X Q, Zhang Y B, Zhang B, Miao Z Z, Wu T X, Yang X G. Chem Res Chin Univ, 2013, 29: 952

    12. [12]

      [12] Fernández-García M, Martínez-Arias A, Belver C, Anderson J A, Conesa J C, Soria J. J Catal, 2000, 190: 387

    13. [13]

      [13] Trillat J F, Massardier J, Moraweck B, Praliaud H, Renouprez A J. Stud Surf Sci Catal, 1998, 116: 103

    14. [14]

      [14] Elhamdaoui A, Bergeret G, Massardier J, Primet M, Renouprez A. J Catal, 1994, 148: 47

    15. [15]

      [15] Hungría A B, Iglesias-Juez A, Martínez-Arias A, Fernández-García M, Anderson J A, Conesa J C, Soria J. J Catal, 2002, 206: 281

    16. [16]

      [16] Hungría A B, Browning N D, Erni R P, Fernández-García M, Conesa J C, Pérez-Omil J A, Martínez-Arias A. J Catal, 2005, 235: 251

    17. [17]

      [17] Zhang S J, Li L D, Zhang F X, Xue B, Guan N J. Chin J Catal (张淑娟, 李兰冬, 章福祥, 薛斌, 关乃佳. 催化学报), 2005, 26: 929

    18. [18]

      [18] Hungría A B, Fernández-García M, Anderson J A, Martínez-Arias A. J Catal, 2005, 235: 262

    19. [19]

      [19] Martínez-Arias A, Fernández-García M, Hungría A B, Iglesias-Juez A, Anderson J A. Catal Today, 2007, 126: 90

    20. [20]

      [20] Fang R M, Cui Y J, Chen S J, Shang H Y, Shi Z H, Gong M C, Chen Y Q. Chin J Catal (方瑞梅, 崔亚娟, 陈思洁, 尚鸿燕, 史忠华, 龚茂初, 陈耀强. 催化学报), 2015, 36: 229

    21. [21]

      [21] Zhao B, Wang Q Y, Li G F, Zhou R X. J Environ Chem Eng, 2013, 1: 534

    22. [22]

      [22] Narui K, Furuta K, Yata H, Nishida A, Kohtoku Y, Matsuzaki T. Catal Today, 1998, 45: 173

    23. [23]

      [23] Bonarowska M, Pielaszek J, Juszczyk W, Karpiński Z. J Catal, 2000, 195: 304

    24. [24]

      [24] Simplício L M T, Brandão S T, Sales E A, Lietti L, Bozon-Verduraz F. Appl Catal B, 2006, 63: 9

    25. [25]

      [25] Bourane A, Derrouiche S, Bianchi D. J Catal, 2004, 228: 288

    26. [26]

      [26] Usami Y, Kagawa K, Kawazoe M, Matsumura Y, Sakurai H, Haruta M. Appl Catal A, 1998, 171: 123

    27. [27]

      [27] Xiao L H, Sun K P, Xu X L, Li X N. Catal Commun, 2005, 6: 796

    28. [28]

      [28] Liu J Y, Zhao M, Xu C H, Liu S Y, Zhang X Q, Chen Y Q. Chin J Catal (刘建英, 赵明, 徐成华, 刘盛余, 张雪乔, 陈耀强. 催化学报), 2013, 34: 751

    29. [29]

      [29] Kobayashi T, Yamada T, Kayano K. Appl Catal B, 2001, 30: 287

    30. [30]

      [30] Zhao M, Zhang H L, Li X, Chen Y Q. J Energy Chem, 2014, 23: 755

    31. [31]

      [31] Talo A, Lahtinen J, Hautojärvi P. Appl Catal B, 1995, 5: 221

    32. [32]

      [32] Yang L Y, Lin S Y, Yang X, Fang W M, Zhou R X. J Hazard Mater, 2014, 279: 226

    33. [33]

      [33] Shinjoh H, Muraki H, Fujitani Y. Appl Catal, 1989, 49: 195

    34. [34]

      [34] Li Y, Wang X X, Xie C, Song C S. Appl Catal A, 2009, 357: 213

    35. [35]

      [35] Tanabe T, Nagai Y, Dohmae K, Takagi N, Takahashi N, Matsumoto S, Shinjoh H. Appl Catal B, 2011, 105: 41

  • 加载中
    1. [1]

      Qingqing SHEN , Xiangbowen DU , Kaicheng QIAN , Zhikang JIN , Zheng FANG , Tong WEI , Renhong LI . Self-supporting Cu/α-FeOOH/foam nickel composite catalyst for efficient hydrogen production by coupling methanol oxidation and water electrolysis. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1953-1964. doi: 10.11862/CJIC.20240028

    2. [2]

      Hailang JIA , Pengcheng JI , Hongcheng LI . Preparation and performance of nickel doped ruthenium dioxide electrocatalyst for oxygen evolution. Chinese Journal of Inorganic Chemistry, 2025, 41(8): 1632-1640. doi: 10.11862/CJIC.20240398

    3. [3]

      Wang Wang , Yucheng Liu , Shengli Chen . Use of NiFe Layered Double Hydroxide as Electrocatalyst in Oxygen Evolution Reaction: Catalytic Mechanisms, Electrode Design, and Durability. Acta Physico-Chimica Sinica, 2024, 40(2): 2303059-0. doi: 10.3866/PKU.WHXB202303059

    4. [4]

      Pei Li , Yuenan Zheng , Zhankai Liu , An-Hui Lu . Boron-Containing MFI Zeolite: Microstructure Control and Its Performance of Propane Oxidative Dehydrogenation. Acta Physico-Chimica Sinica, 2025, 41(4): 2406012-0. doi: 10.3866/PKU.WHXB202406012

    5. [5]

      Haoyu Sun , Dun Li , Yuanyuan Min , Yingying Wang , Yanyun Ma , Yiqun Zheng , Hongwen Huang . Hierarchical Palladium-Copper-Silver Porous Nanoflowers as Efficient Electrocatalysts for CO2 Reduction to C2+ Products. Acta Physico-Chimica Sinica, 2024, 40(6): 2307007-0. doi: 10.3866/PKU.WHXB202307007

    6. [6]

      Wen YANG , Didi WANG , Ziyi HUANG , Yaping ZHOU , Yanyan FENG . La promoted hydrotalcite derived Ni-based catalysts: In situ preparation and CO2 methanation performance. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 561-570. doi: 10.11862/CJIC.20230276

    7. [7]

      Bo YANG , Gongxuan LÜ , Jiantai MA . Nickel phosphide modified phosphorus doped gallium oxide for visible light photocatalytic water splitting to hydrogen. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 736-750. doi: 10.11862/CJIC.20230346

    8. [8]

      Meiran Li , Yingjie Song , Xin Wan , Yang Li , Yiqi Luo , Yeheng He , Bowen Xia , Hua Zhou , Mingfei Shao . Nickel-Vanadium Layered Double Hydroxides for Efficient and Scalable Electrooxidation of 5-Hydroxymethylfurfural Coupled with Hydrogen Generation. Acta Physico-Chimica Sinica, 2024, 40(9): 2306007-0. doi: 10.3866/PKU.WHXB202306007

    9. [9]

      Qiangqiang SUN , Pengcheng ZHAO , Ruoyu WU , Baoyue CAO . Multistage microporous bifunctional catalyst constructed by P-doped nickel-based sulfide ultra-thin nanosheets for energy-efficient hydrogen production from water electrolysis. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1151-1161. doi: 10.11862/CJIC.20230454

    10. [10]

      Bizhu Shao , Huijun Dong , Yunnan Gong , Jianhua Mei , Fengshi Cai , Jinbiao Liu , Dichang Zhong , Tongbu Lu . Metal-Organic Framework-Derived Nickel Nanoparticles for Efficient CO2 Electroreduction in Wide Potential Windows. Acta Physico-Chimica Sinica, 2024, 40(4): 2305026-0. doi: 10.3866/PKU.WHXB202305026

    11. [11]

      Renxiao Liang ,  Zhe Zhong ,  Zhangling Jin ,  Lijuan Shi ,  Yixia Jia . A Palladium/Chiral Phosphoric Acid Relay Catalysis for the One-Pot Three-Step Synthesis of Chiral Tetrahydroquinoline. University Chemistry, 2024, 39(5): 209-217. doi: 10.3866/PKU.DXHX202311024

    12. [12]

      Zhanggui DUAN , Yi PEI , Shanshan ZHENG , Zhaoyang WANG , Yongguang WANG , Junjie WANG , Yang HU , Chunxin LÜ , Wei ZHONG . Preparation of UiO-66-NH2 supported copper catalyst and its catalytic activity on alcohol oxidation. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 496-506. doi: 10.11862/CJIC.20230317

    13. [13]

      Zhuo Han , Danfeng Zhang , Haixian Wang , Guorui Zheng , Ming Liu , Yanbing He . Research Progress and Prospect on Electrolyte Additives for Interface Reconstruction of Long-Life Ni-Rich Lithium Batteries. Acta Physico-Chimica Sinica, 2024, 40(9): 2307034-0. doi: 10.3866/PKU.WHXB202307034

    14. [14]

      Zhiquan Zhang , Baker Rhimi , Zheyang Liu , Min Zhou , Guowei Deng , Wei Wei , Liang Mao , Huaming Li , Zhifeng Jiang . Insights into the Development of Copper-Based Photocatalysts for CO2 Conversion. Acta Physico-Chimica Sinica, 2024, 40(12): 2406029-0. doi: 10.3866/PKU.WHXB202406029

    15. [15]

      Qing Li , Guangxun Zhang , Yuxia Xu , Yangyang Sun , Huan Pang . P-Regulated Hierarchical Structure Ni2P Assemblies toward Efficient Electrochemical Urea Oxidation. Acta Physico-Chimica Sinica, 2024, 40(9): 2308045-0. doi: 10.3866/PKU.WHXB202308045

    16. [16]

      Yan LIU , Jiaxin GUO , Song YANG , Shixian XU , Yanyan YANG , Zhongliang YU , Xiaogang HAO . Exclusionary recovery of phosphate anions with low concentration from wastewater using a CoNi-layered double hydroxide/graphene electronically controlled separation film. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1775-1783. doi: 10.11862/CJIC.20240043

    17. [17]

      Peng YUE , Liyao SHI , Jinglei CUI , Huirong ZHANG , Yanxia GUO . Effects of Ce and Mn promoters on the selective oxidation of ammonia over V2O5/TiO2 catalyst. Chinese Journal of Inorganic Chemistry, 2025, 41(2): 293-307. doi: 10.11862/CJIC.20240210

    18. [18]

      Bing WEI , Jianfan ZHANG , Zhe CHEN . Research progress in fine tuning of bimetallic nanocatalysts for electrocatalytic carbon dioxide reduction. Chinese Journal of Inorganic Chemistry, 2025, 41(3): 425-439. doi: 10.11862/CJIC.20240201

    19. [19]

      Jingping Li , Suding Yan , Jiaxi Wu , Qiang Cheng , Kai Wang . Improving hydrogen peroxide photosynthesis over inorganic/organic S-scheme photocatalyst with LiFePO4. Acta Physico-Chimica Sinica, 2025, 41(9): 100104-0. doi: 10.1016/j.actphy.2025.100104

    20. [20]

      Shijie Ren , Mingze Gao , Rui-Ting Gao , Lei Wang . Bimetallic Oxyhydroxide Cocatalyst Derived from CoFe MOF for Stable Solar Water Splitting. Acta Physico-Chimica Sinica, 2024, 40(7): 2307040-0. doi: 10.3866/PKU.WHXB202307040

Get Citation
PDF
XML
Metrics
  • PDF Downloads(0)
  • Abstract views(429)
  • HTML views(8)

通讯作者: 陈斌, bchen63@163.com
  • 1. 

    沈阳化工大学材料科学与工程学院 沈阳 110142

  1. 本站搜索
  2. 百度学术搜索
  3. 万方数据库搜索
  4. CNKI搜索
Address：Zhongguancun North First Street 2,100190 Beijing, PR China Tel: +86-010-82449177-888
Powered By info@rhhz.net

/

DownLoad:  Full-Size Img  PowerPoint
Return