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Citation: Yan Li, Bing Li, Ting Chen, Zhicheng Zhou, Jun Wang, Jun Huang. Direct hydroxylation of arenes with O2 catalyzed by V@CN catalyst[J]. Chinese Journal of Catalysis, ;2015, 36(7): 1086-1092. doi: 10.1016/S1872-2067(14)60319-3 shu

Direct hydroxylation of arenes with O2 catalyzed by V@CN catalyst

  • 1.

    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemistry and Chemical Engineering, Nanjing Tech University, Nanjing 210009, Jiangsu, China

  • Corresponding author: Jun Huang, 
  • Received Date: 15 January 2015
    Available Online: 16 February 2015

    Fund Project: 国家自然科学基金(21136005) (21136005) 国家高技术研究发展计划(863计划, 2012AA03A606) (863计划, 2012AA03A606) 江苏高校优势学科建设工程(PAPD, 38701001). (PAPD, 38701001)

  • A vanadium doped graphitic carbon nitride catalyst has been prepared and used for the direct hydroxylation of arenes with O2. Substituted arenes with electron-withdrawing groups such as CN, NO2, COOH, CF3, and COCH3 were oxygenated to the corresponding phenols in moderate yields. The catalyst also proved applicable for the hydroxylation of aromatic halides (F, Cl, and Br) with O2.
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