Citation:
Yuan An, Tan Long, Liu Li, Ying Jin, Tang Hao, Sun Runguang. Research Progress of Li2S-P2S5 Electrolytes and Their Application in Solid-State Lithium-Ion Batteries[J]. Chemistry,
;2019, 82(8): 706-716.
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All-solid-state lithium-ion batteries have been widely used in portable electronic devices due to their advantages of good safety performance, high energy density, wide working-temperature range, etc. The solid electrolytes are the key material of all-solid-state lithium-ion batteries. Among various electrolytes, the sulfide-based materials have the characteristics of high ionic conductivity, wide electrochemical window, low grain boundary resistance and easy film formation, and is considered to be the most promising electrolyte in all-solid-state batteries. In this paper, we focused on the recent progress in the solid electrolytes with respect to the preparation, characterization and modification of Li2S-P2S5 electrolytes, and stability/compatibility of the interface between the solid electrolyte and the electrode. Moreover, the performance of these solid electrolyte related all-solid-state lithium-ion batteries are also reviewed.
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