Citation: Bai Jingru, Zhang Benxi, Zhang Wei, Yue Mingbo. The Carbon Deposition Characteristics of Propylene in Oil Shale Retorting Gas on Different Heat-Resistant Alloys[J]. Chemistry, ;2016, 79(5): 438-442. shu

The Carbon Deposition Characteristics of Propylene in Oil Shale Retorting Gas on Different Heat-Resistant Alloys

1.
School of Energy and Power Engineering, Northeast Dianli University, Jilin city 132012

Corresponding author: Zhang Benxi,
Received Date: 3 September 2015
Available Online: 16 November 2015
Fund Project:

An experimental research for the carbon deposition characteristics of propylene in oil shale retorting gas was carried out under different conditions including temperatures (700, 750 and 800℃), gas flow (20, 30 and 40 mL/min) and constant time (20min) by a home-made continuous flow reactor system. Different reactors made by 2520 and 316L stainless steel tubes were used. The results showed that the initial carbon deposition temperature range was 630~650℃ and 670~690℃ for 2520 and 316L, respectively. The carbon deposition morphology observed by SEM indicated that no matter 2520 or 316L there were two species of carbon, i.e. filamentous carbon and amorphous carbon. The amount analysis of carbon deposition under different conditions by TPO methods showed that 316L had a characteristic of metal powder resistance. The results of the TG/DSC analyses for carbons stripped proved that the carbon deposition activity of 316L stainless steel is higher than that of 2520 stainless steel.
- Heat-resisting alloy,
- Oil shale,
- Propylene,
- Carbon deposition,
- Metal-catalyzed
1. [1]
  [1] 曹东方. 石油和化工设备, 2013, 16(10): 23~27.
2. [2]
  [2] 李处森, 于力. 中国腐蚀与防护学报, 2001, 21(3): 158~166.
3. [3]
  [3] A Niaei, D Salari, N Daneshvar et al. World Acad. Sci. Eng. Technol., 2007, 29(1): 15~17.
4. [4]
  [4] D Melo, D Sigüenza, O Salas et al. Surf. Coat. Technol., 2009, 204(6): 788~792.
5. [5]
  [5] S Esconjauregui, C M Whelan, K Maex. Carbon, 2009, 47(3): 659~669.
6. [6]
  [6] 谢文杰, 方文军, 李丹等. 化学学报, 2009, 67(15): 1759~1764.
7. [7]
  [7] 路遥, 金晶, 陈磊等. 煤炭学报, 2012, 37(2): 328~331.
8. [8]
  [8] 袁翠峪, 魏迎旭, 李金哲等. 催化学报, 2012, 33(2)，376~374.
9. [9]
  [9] 卢翠英, 成来飞, 张立同等. 复合材料学报, 2008, 25(6): 152~155.
10. [10]
  [10] 孙佰仲, 孙世鹏, 王擎等. 煤炭学报, 2015, 39(S2): 538~543.
11. [11]
  [11] 李处森, 杨院生. 中国腐蚀与防护学报, 2004, 24(3): 188~192.
12. [12]
  [12] H O Pierson. Handbook of chemical vapor deposition: principles, technology and applications, William Andrew, 1999.
13. [13]
  [13] 张伟刚. 化学气相沉积: 从烃类气体到固体碳, 科学出版社, 2007.
14. [14]
  [14] 刘红梅, 申文杰, 包信和等. 催化学报, 2004, 25(6): 495~500.
15. [15]
  [15] A Becker, K J Hüttinger. Carbon, 1998, 36(3): 177~199.
16. [16]
  [16] A Becker, K J Hüttinger. Carbon, 1998, 36(3): 201~211.
17. [17]
  [17] R T K Baker, P S Harris, R B Thomas et al. J. Catal., 1973, 30(1): 86~95.
18. [18]
  [18] 董鹏, 吴惠真. 石油化工, 1997, 26(1): 17~21.
19. [19]
  [19] P Wang, E Tanabe, K Ito et al. Appl. Catal. A: Gen., 2002, 231(1): 35~44.
20. [20]
  [20] 刘红梅.中国科学院大连化学物理研究所学位论文, 2001,46~60.
1. [1]
  Guojie Xu , Fang Yu , Yunxia Wang , Meng Sun . Introduction to Metal-Catalyzed β-Carbon Elimination Reaction of Cyclopropenones. University Chemistry, 2024, 39(8): 169-173. doi: 10.3866/PKU.DXHX202401060
2. [2]
  Zhuoyan Lv , Yangming Ding , Leilei Kang , Lin Li , Xiao Yan Liu , Aiqin Wang , Tao Zhang . Light-Enhanced Direct Epoxidation of Propylene by Molecular Oxygen over CuO_x/TiO₂ Catalyst. Acta Physico-Chimica Sinica, 2025, 41(4): 2408015-0. doi: 10.3866/PKU.WHXB202408015
3. [3]
  Xingyang LI , Tianju LIU , Yang GAO , Dandan ZHANG , Yong ZHOU , Meng PAN . A superior methanol-to-propylene catalyst: Construction via synergistic regulation of pore structure and acidic property of high-silica ZSM-5 zeolite. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1279-1289. doi: 10.11862/CJIC.20240026
4. [4]
  Wenxiu Yang , Jinfeng Zhang , Quanlong Xu , Yun Yang , Lijie Zhang . Bimetallic AuCu Alloy Decorated Covalent Organic Frameworks for Efficient Photocatalytic Hydrogen Production. Acta Physico-Chimica Sinica, 2024, 40(10): 2312014-0. doi: 10.3866/PKU.WHXB202312014
5. [5]
  Zijian Zhao , Yanxin Shi , Shicheng Li , Wenhong Ruan , Fang Zhu , Jijun Jiang . A New Exploration of the Preparation of Polyacrylic Acid by Free Radical Polymerization Based on the Concept of Green Chemistry. University Chemistry, 2024, 39(5): 315-324. doi: 10.3866/PKU.DXHX202311094
6. [6]
  Huiwei Ding , Bo Peng , Zhihao Wang , Qiaofeng Han . Advances in Metal or Nonmetal Modification of Bismuth-Based Photocatalysts. Acta Physico-Chimica Sinica, 2024, 40(4): 2305048-0. doi: 10.3866/PKU.WHXB202305048
7. [7]
  Junke LIU , Kungui ZHENG , Wenjing SUN , Gaoyang BAI , Guodong BAI , Zuwei YIN , Yao ZHOU , Juntao LI . Preparation of modified high-nickel layered cathode with LiAlO₂/cyclopolyacrylonitrile dual-functional coating. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1461-1473. doi: 10.11862/CJIC.20240189
8. [8]
  Guimin ZHANG , Wenjuan MA , Wenqiang DING , Zhengyi FU . Synthesis and catalytic properties of hollow AgPd bimetallic nanospheres. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 963-971. doi: 10.11862/CJIC.20230293
9. [9]
  Ping ZHANG , Chenchen ZHAO , Xiaoyun CUI , Bing XIE , Yihan LIU , Haiyu LIN , Jiale ZHANG , Yu'nan CHEN . Preparation and adsorption-photocatalytic performance of ZnAl@layered double oxides. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1965-1974. doi: 10.11862/CJIC.20240014
10. [10]
  Peng XU , Shasha WANG , Nannan CHEN , Ao WANG , Dongmei YU . Preparation of three-layer magnetic composite Fe₃O₄@polyacrylic acid@ZiF-8 for efficient removal of malachite green in water. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 544-554. doi: 10.11862/CJIC.20230239
11. [11]
  Geyang Song , Dong Xue , Gang Li . Recent Advances in Transition Metal-Catalyzed Synthesis of Anilines from Aryl Halides. University Chemistry, 2024, 39(2): 321-329. doi: 10.3866/PKU.DXHX202308030
12. [12]
  Jiaming Xu , Yu Xiang , Weisheng Lin , Zhiwei Miao . Research Progress in the Synthesis of Cyclic Organic Compounds Using Bimetallic Relay Catalytic Strategies. University Chemistry, 2024, 39(3): 239-257. doi: 10.3866/PKU.DXHX202309093
13. [13]
  Lutian Zhao , Yangge Guo , Liuxuan Luo , Xiaohui Yan , Shuiyun Shen , Junliang Zhang . Electrochemical Synthesis for Metallic Nanocrystal Electrocatalysts: Principle, Application and Challenge. Acta Physico-Chimica Sinica, 2024, 40(7): 2306029-0. doi: 10.3866/PKU.WHXB202306029
14. [14]
  Ye Wang , Ruixiang Ge , Xiang Liu , Jing Li , Haohong Duan . An Anion Leaching Strategy towards Metal Oxyhydroxides Synthesis for Electrocatalytic Oxidation of Glycerol. Acta Physico-Chimica Sinica, 2024, 40(7): 2307019-0. doi: 10.3866/PKU.WHXB202307019
15. [15]
  Lu Zhuoran , Li Shengkai , Lu Yuxuan , Wang Shuangyin , Zou Yuqin . Cleavage of C―C Bonds for Biomass Upgrading on Transition Metal Electrocatalysts. Acta Physico-Chimica Sinica, 2024, 40(4): 2306003-0. doi: 10.3866/PKU.WHXB202306003
16. [16]
  Zhengyu Zhou , Huiqin Yao , Youlin Wu , Teng Li , Noritatsu Tsubaki , Zhiliang Jin . Synergistic Effect of Cu-Graphdiyne/Transition Bimetallic Tungstate Formed S-Scheme Heterojunction for Enhanced Photocatalytic Hydrogen Evolution. Acta Physico-Chimica Sinica, 2024, 40(10): 2312010-0. doi: 10.3866/PKU.WHXB202312010
17. [17]
  Zelong LIANG , Shijia QIN , Pengfei GUO , Hang XU , Bin ZHAO . Synthesis and electrocatalytic CO₂ reduction performance of metal-organic framework catalysts loaded with silver particles. Chinese Journal of Inorganic Chemistry, 2025, 41(1): 165-173. doi: 10.11862/CJIC.20240409
18. [18]
  Bing WEI , Jianfan ZHANG , Zhe CHEN . Research progress in fine tuning of bimetallic nanocatalysts for electrocatalytic carbon dioxide reduction. Chinese Journal of Inorganic Chemistry, 2025, 41(3): 425-439. doi: 10.11862/CJIC.20240201
19. [19]
  Xuexia He , Zhibin Lei , Pei Chen , Qi Li , Weiyu Deng , Peng Hu . 以“溶度积规则”指导电荷转移共晶沉淀析出——材料类专业无机化学教学改革案例. University Chemistry, 2025, 40(8): 1-10. doi: 10.12461/PKU.DXHX202410099
20. [20]
  Xinyu Miao , Hao Yang , Jie He , Jing Wang , Zhiliang Jin . Adjusting the electronic structure of Keggin-type polyoxometalates to construct S-scheme heterojunction for photocatalytic hydrogen evolution. Acta Physico-Chimica Sinica, 2025, 41(6): 100051-0. doi: 10.1016/j.actphy.2025.100051

Get Citation

PDF

XML

Metrics

PDF Downloads(0)
Abstract views(257)
HTML views(19)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142