Citation: Gu Shilei, Wang Lin, Zhao Jishou, Li Jing. Diketopyrrolopyrrole Contained Platinum Polyyne for Organic Field Effect Transistors[J]. Chemistry, ;2016, 79(9): 817-821. shu

Diketopyrrolopyrrole Contained Platinum Polyyne for Organic Field Effect Transistors

Gu Shilei ¹ ,
Wang Lin ^1,, ,
Zhao Jishou ¹ ,
Li Jing ^2,,

1.
1. Department of Chemistry and Environment, Yunnan Minzu University, Kunming 650504;
2.
2. Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714

Corresponding author: Wang Lin, Li Jing,
Received Date: 9 May 2016
Available Online: 2 June 2016
Fund Project:

A platinum polyyne PtDPP with 2,5-bis(2-octyl-dodecyl)-3,6-di(thiophen-2-yl)pyrrolo[3,4-c]pyrrole-1,4(2H,5H)-dione as co-unit was synthesized and characterized. The LUMO and HOMO energy of PtDPP was estimated to be -3.4 eV and -5.3 eV by cyclic voltammogram and UV-Vis spectrum. Bottom gate bottom contact OFET devices of PtDPP were fabricated via spin coating. After annealing at 160℃, the OFET devices show highest performance with hole mobility up to 1.0×10^-3cm²·V^-1·s^-1, on/off ratio of 10⁵ and threshold voltage of -15 V. Further investigation on XRD and AFM suggested that the crytalline order enhanced along the annealing process.
- Diketopyrrolopyrrole,
- Metal-organic polymer,
- Field-effect transistors
1. [1]
  [1] (a) I Manners. Angew. Chem. Int. Ed., 1996, 35(15):1602~1621; (b) P Nguyen, P Gómez-Elipe, I Manners. Chem. Rev., 1999, 99(6):1515~1548; (c) D A Foucher, B Z Tang, I Manners. J. Am. Chem. Soc., 1992, 114(15):6246~6248; d) K Kulbaba, I Manners. Macromol. Rapid Commun, 2001, 22(10):711~724; (e) Y Ni, R Rulkens, I Manners. J. Am. Chem. Soc., 1996, 118(17):4102~4114; (f) J A Massey, K N Power, I Manners et al. J. Am. Chem. Soc., 2000, 122(47):11577~11584.
2. [2]
  [2] R D Archer, D Wohrle. Angew. Chem.Ger. Ed., 2001, 113(23):4644.
3. [3]
  [3] D J Caruana, A Heller. J. Am. Chem. Soc., 1999, 121(4):769~774.
4. [4]
  [4] R Yoshida, T Takahashi, T Yamaguchi et al. Adv. Mater., 1997, 9(2):175~178.
5. [5]
  [5] R P Kingsborough, T M Swager. Prog. Inorg. Chem., 2009, 48:123~231.
6. [6]
  [6] M J MacLachlan, M Ginzburg, N Coombs et al. Science, 2000, 287(5457):1460~1463.
7. [7]
  [7] J A Massey, M A Winnik, I Manners et al. J. Am. Chem. Soc., 2001, 123(13):3147~3148.
8. [8]
  [8] J Y Cheng, C A Ross, V Z H Chan et al. Adv. Mater., 2001, 13(15):1174~178.
9. [9]
  [9] C L Fraser, A P Smith, X Wu. J. Am. Chem. Soc., 2000, 122(37):9026~9027.
10. [10]
  [10] S J Hou, W K Chan. Macromol. Rapid. Commun., 1999, 20(8):440~443.
11. [11]
  [11] R Tassoni, R R Schrock. Chem. Mater., 1994, 6(6):744~749.
12. [12]
  [12] W Steffen, B Köhler, M Altmann et al. Chem. Eur. J., 2001, 7(1):117~126.
13. [13]
  [13] M Enomoto, A Kishimura, T Aida. J. Am. Chem. Soc., 2001, 123(23):5608~5609.
14. [14]
  [14] J Massey, K N Power, I Manners et al. J. Am. Chem. Soc., 1998, 120(37):9533~9540.
15. [15]
  [15] A Köhler, H F Wittmann, R H Friend et al. Synth. Met. 1996, 77(1):147~150.
16. [16]
  [16] F Guo, Y G Kim, J R Reynolds et al. Chem. Commun., 2006,(17):1887~1889.
17. [17]
  [17] W Y Wong, X Z Wang, Z He et al. Nat. Mater., 2007, 6(7):521~527.
18. [18]
  [18] W Y Wong, X Z Wang, Z He et al. J. Am. Chem. Soc., 2007, 129(46):14372~14380.
19. [19]
  [19] K Sonogashira, S Takahashi, N Hagihara et al. Macromolecules, 1977, 10(4):879~880.
20. [20]
  [20] I L Kang, H J Yun, D S Chung et al. J. Am. Soc. Chem., 2013, 135(40):14896~14899.
21. [21]
  [21] Y Li, P Sonar, S P Singh et al. J. Am. Chem. Soc., 2011, 133(7):2198~2204.
22. [22]
  [22] (a) A J Bard, R Memming, B Miller. Pure Appl. Chem., 1991, 63(4):569~596; (b) S Trasatti. Pure Appl. Chem., 1986, 58(7):955~966; (c) H Usta, A Facchetti, T J Marks. J. Am. Chem. Soc., 2008, 130(27):8580~8581.
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沈阳化工大学材料科学与工程学院沈阳 110142

Diketopyrrolopyrrole Contained Platinum Polyyne for Organic Field Effect Transistors

南开大学师唯/华北电力大学（保定）刘景维：二维配位聚合物中有序的亲锂冠醚位点用于无枝晶锂沉积

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通讯作者: 陈斌, bchen63@163.com