Citation:
CHEN Hui-chao, WU Wei, LIANG Cai. Effect of attapulgite on PM2.5 emission and agglomeration during coal combustion[J]. Journal of Fuel Chemistry and Technology,
;2015, 43(2): 177-184.
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Effect of attapulgite on PM2.5 emissions and agglomeration during coal combustion was investigated in a fixed bed system. The effects of addition amount, combustion temperature, mole ratio of calcium to sulfate and combustion atmosphere on mass and number concentration and collection efficiency of PM2.5 were analyzed. The results show that attapulgite added during coal combustion can effectively reduce PM2.5 emissions. The suitable amount of attapulgite is no more than 3%. PM2.5 emission during coal combustion in air is higher than that in O2/CO2 atmosphere. PM1 mass concentration decreases with increasing mole ratio of calcium to sulfate, while PM1~2.5 mass concentration increases, indicating an increasing trend in particle size. Increasing combustion temperature will increase PM2.5 emission and reduce its collection.
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Keywords:
- attapulgite,
- PM2.5,
- particle agglomeration
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[1]
[1] 吕建燚, 李定凯. 不同条件对煤粉燃烧后PM10、PM2.5、PM1排放影响的实验研究[J]. 中国电机工程学报, 2006, 26(20): 103-107. (LV Jian-yi, LI Ding-kai. Experimental study on PM10, PM2.5, PM1 emission features influenced by different conditions in pulverized coal combustion[J]. Chin Soc Electr Eng, 2006, 26(20): 103-107.)
-
[2]
[2] STRAND M, PAGELS J, SZPILA A, GUDMUNDSSON A, SWIETLICKI E, BOHGARD M, SANATI M. Fly ash penetration through electrostatic precipitator and flue gas condenser in a 6 MW biomass fired boiler[J]. Energy Fuels, 2002, 16(6): 1499-1506.
-
[3]
[3] 岳勇, 陈雷, 姚强, 李水清. 燃煤锅炉颗粒物粒径分布和痕量元素富集特性实验研究[J]. 中国电机工程学报, 2005, 25(18): 74-79. (YUE Yong, CHEN lei, CAO Qiang, LI Shui-qing. Experimental study on characteristics of particulate matter size distribution and trace elements enrichment in emissions from a pulverized coal-fired boiler[J]. Chin Soc Electr Eng, 2005, 25(18): 74-79.)
-
[4]
[4] SENIOR C L, BOOL L E, SRINIVASACHAR S, PEASEB B R, PORLE K. Pilot scale study of trace element vaporization and condensation during combustion of a pulverrized sub-bituminous coal[J]. Fuel Process Technol, 2000, 63(2/3): 149-165.
-
[5]
[5] SONDREAL E A, BENSON S A, PAVLISH J H, NICHOLAS V C R. An overview of air quality: Mercury, trace elements, and particulate matter[J]. Fuel Process Technol, 2004, 85(6/7): 425-440.
-
[6]
[6] 魏凤, 张军营, 王春梅, 郑楚光. 煤燃烧超细颗粒物团聚促进技术的研究进展[J]. 煤炭转化, 2004, 26(3): 27-31. (WEI Feng, ZHANG Jun-ying, WANG Chun-mei, ZHENG Chu-guang. Review of submicron particles agglomeration in coal combustion process[J]. Coal Convers, 2004, 26(3): 27-31.)
-
[7]
[7] 徐鸿, 骆仲泱, 王鹏, 王涛, 高翔, 岑可法. 石灰石对煤燃烧产生颗粒物及重金属影响实验研究[J]. 工程热物理学报, 2004, 25(5): 871-874. (XU Hong, LUO Zhong-yang, WANG Peng, WANG Tao, GAO Xiang, CEN Ke-fa. Experimental research of limestone effect on particulates and heavy metals emitted from coal combustion[J]. J Eng Thermophysics, 2004, 25(5): 871-874.)
-
[8]
[8] TAKUWA T, NARUSE I. Emission control of sodium compounds and their formation mechanisms during coal combustion[J]. Proc Combust Inst, 2007, 31(2): 2863-2870.
-
[9]
[9] 屈成瑞, 赵长遂, 段伦博, 周骛. O2 /CO2 气氛添加高岭石对燃煤PM2. 5 排放的影响[J]. 燃料化学学报, 2010, 38(4): 398-402. (QU Cheng-rui, ZHAO Chang-sui, DUAN Lun-bo, ZHOU Wu. Effect of kaolinite additive on formation of PM2.5 under O2 /CO2 atmosphere during coal combustion[J]. J Fuel Chem Technol, 2010, 38(4): 398-402.)
-
[10]
[10] BRADLEY W F. The structure scheme of attapulgite[J]. Am Mineral, 1940, 25: 405-410.
-
[11]
[11] 张玉. 凹凸棒粘土及其在印染行业中的应用. 上海: 东华大学硕士学位论文, 2013. (ZHANG Yu. Application of the attapulgite clay in dyeing and finishing industry. Shanghai: Donghua University, 2013.)
-
[12]
[12] HEIDENREICH S, EBERT F. Condensational droplet growth as a preconditioning technique for the separation of submicron particles from gases[J]. Chem Eng Process, 1995, 34(3): 235-244.
-
[13]
[13] HEIDENREICH S, VOGT U, BVTTNER H, EBERT F. A novel process to separate submicron particles from gases-a cascade of packed columns[J]. Chem Eng Sci, 2000, 55(15): 2895-2905.
-
[14]
[14] 屈成锐. O2/CO2气氛下CFB燃煤PM2.5形成机理及其控制的研究. 南京: 东南大学, 2010. (QU Cheng-rui. Investigation on formation mechanisms and control of PM2.5 under O2/CO2 atmosphere during coal combustion in the CFB. Nanjing: Southeast University, 2010.)
-
[15]
[15] 屈成锐, 徐斌, 王学涛, 刘建新. O2/CO2气氛燃烧温度对燃煤PM2.5形成的影响[J]. 燃料科学与技术, 2012, 18(5): 410-414. (QU Cheng-rui, XU Bin, WANG Xue-tao, LIU Jian-xin. Effect of combustion temperature on formation of PM2.5 under O2/CO2 atmosphere during coal combustion[J]. J Combust Sci Technol, 2012, 18(5): 410-414.)
-
[1]
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