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Citation: SUN Ying, HUANG Yan, ZHAO Wei, SU qian, ZHANG Jun-feng, YANG Liu-chun. Research on catalytic performance of supported perovskite catalyst for NO oxidation and resistance to SO2 poisoning[J]. Journal of Fuel Chemistry and Technology, ;2014, 42(10): 1246-1252. shu

Research on catalytic performance of supported perovskite catalyst for NO oxidation and resistance to SO2 poisoning

  • 1.

    Department of Environmental Science and Engineering, Xiangtan University, Xiangtan 411105, China

  • Corresponding author: HUANG Yan, 
  • Received Date: 8 April 2014
    Available Online: 15 July 2014

    Fund Project: 湖南省自然科学基金(12JJ3020) (12JJ3020) 湖南省高校创新平台开放基金(14K094)。 (14K094)

  • Supported perovskite-type catalysts La1-xCexCoO3/CeO2 (x = 0~0.3) were synthesized through complexing impregnation with citric acid and characterized by X-ray diffraction (XRD), Fourier transformed infrared (FT-IR), nitrogen adsorption, H2 temperature-programmed reduction (H2-TPR), and O2 temperature-programmed desorption (O2-TPD). The performance of NO catalytic oxidation and SO2 resistance were investigated in the article. The results showed that the catalytic activity of La1-xCexCoO3/CeO2 was closely related to the surface area and redox properties. Especially La0.8Ce0.2CoO3/CeO2 achieved 78% NO conversion at 300 ℃.The introduction of CeO2 as support simultaneously enhanced the low temperature activity and SO2 resistance.
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    1. [1]

      [1] SHEN B, LIN X, ZHAO Y. Catalytic oxidation of NO with O2 over Pt/γ-Al2O3 and La0.8Sr0.2MnO3[J]. Chem Eng J, 2013, 222(1): 9-15.

    2. [2]

      [2] SKALSKA K, MILLER J S, LEDAKOWICZ S. Trends in NOx abatement: A review[J]. Sci Total Environ, 2010, 408(19): 3976-3989.

    3. [3]

      [3] LANDI G, LISI L, PIRONE R, TORTORELLI M, RUSSO G. NO decomposition over La-doped Cu-ZSM5 monolith under adsorption-reaction conditions[J]. Appl Catal A: Gen, 2013, 464(1): 61-67.

    4. [4]

      [4] ROY S, BAIKER A. NOx storage-reduction catalysis: From mechanism and materials properties to storage-reduction performance[J]. Chem Rev, 2009, 109(9): 4054-4091.

    5. [5]

      [5] HAUFF K, TUTTLIES U, EIGENBERGER G, NIEKEN U. Platinum oxide formation and reduction during NO oxidation on a diesel oxidation catalyst-Experimental results[J]. Appl Catal B: Environ, 2012, 123(2): 107-116.

    6. [6]

      [6] SHAN W, LIU F, HE H, SHI X, ZHANG C. An environmentally-benign CeO2-TiO2 catalyst for the selective catalytic reduction of NOx with NH3 in simulated diesel exhaust[J]. Catal Today, 2012, 184(1): 160-165.

    7. [7]

      [7] 寻洲, 童华, 黄妍, 童志权. Mn-Ce-Fe/TiO2低温催化还原NO的性能[J]. 环境科学学报, 2008, 28(9): 1733-1738. (XUN Zhou, TONG Hua, HUANG Yan, TONG Zhi-quan. Reduction of NO with Mn-Ce-Fe/TiO2 as catalyst at low temperature[J]. Acta Scientiae Circumstantiae, 2008, 28(9): 1733-1738.)

    8. [8]

      [8] WORCH D, SUPRUN W, GLÄSER R. Supported transition metal-oxide catalysts for HC-SCR DeNOx with propene[J]. Catal Today, 2011, 176(1): 309-313.

    9. [9]

      [9] CHEN J, SHEN M, WANG X, WANG J, SU Y, ZHAO Z. Catalytic performance of NO oxidation over LaMeO3(Me= Mn, Fe, Co) perovskite prepared by the sol-gel method[J]. Catal Commun, 2013, 37(1): 105-108.

    10. [10]

      [10] ZHU J, THOMAS A. Perovskite-type mixed oxides as catalytic material for NO removal[J]. Appl Catal B: Environ, 2009, 92(3): 225-233.

    11. [11]

      [11] BUENO-LÓPEZ A. Diesel soot combustion ceria catalysts[J]. Appl Catal B: Environ, 2014, 146(1): 1-11.

    12. [12]

      [12] WEN Y, ZHANG C, HE H, YU Y, TERAOKA Y. Catalytic oxidation of nitrogen monoxide over La1-xCexCoO3 perovskites[J]. Catal Today, 2007, 126(3): 400-405.

    13. [13]

      [13] ZHANG R, YANG W, LUO N, LI, P, LEI Z CHEN B. Low-temperature NH3-SCR of NO by lanthanum manganite perovskites: Effect of A/B-site substitution and TiO2/CeO2 support[J]. Appl Catal B: Environ, 2014, 146(1): 94-104.

    14. [14]

      [14] 罗娜. 负载型钙钛矿复合氧化物低温氨选择性催化还原NOx的研究[D]. 北京: 北京化工大学, 2012. (LUO Na. Research on low-temperature selective catalytic reduction of NO with NH3 over supported perovskite-typed oxides[D]. Beijing: Beijing University of Chemical Technology, 2012.)

    15. [15]

      [15] 徐海波, 吴晓东, 翁瑞, 潘吉庆. 过渡金属-铈基复合氧化物的制备与碳烟燃烧催化性能[J].中国稀土学报, 2010, 28(1):10-15. (XU Hai-bo, WU Xiao-dong, WENG Duan, PAN Ji-qing. Preparation and soot oxidation activity of transition metal cerium mixed oxides[J]. Journal of the Chinese Rare Earth Society, 2010, 28(1):10-15.)

    16. [16]

      [16] 张华民, 陈永英, 寺冈靖刚, 山添曻. 钴系钙钛矿型复合氧化物A,B位的部分置换对缺陷结构与催化活性的影响[J]. 催化学报, 1992, 13(6): 432-437. (ZHANG Hua-min, CHEN Yong-ying, TERAORA Yasutake, YAMAZOE Noboru. Effect of partial substitution for A, B sites of perovskite-type oxides containing cobalt on oxygen desorption and catalytic activity[J]. Chinese Journal of Catalysis, 1992, 13(6): 432-437.)

    17. [17]

      [17] 马爱静, 王绍增, 邹鸿鹄, 孟明, 李志军, 鲍骏, 李新刚. La0.7Sr0.3Co1-x FexO3催化剂氮氧化物储存及抗硫性能[J]. 物理化学学报, 2012, 28(6): 1474-1480. (MA Ai-jing, WANG Shao-zeng, ZOU Hong-hu, MENG Ming, LI Zhi-jun, BAO Jun, LI Xin-gang. The performance of the NOx storage capacity and sulfur tolerance of the La0.7Sr0.3Co1-xFexO3 Catalyst[J]. Acta Physico-Chimica Sinica, 2012, 28(6): 1474-1480.)

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