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Citation: KANG Min, ZHANG Jun, ZHAO Ning, WEI Wei, SUN Yu-han. CO production via thermochemical CO2 splitting over Ni ferrite-based catalysts[J]. Journal of Fuel Chemistry and Technology, ;2014, 42(1): 68-73. shu

CO production via thermochemical CO2 splitting over Ni ferrite-based catalysts

  • 1.

    1. State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China;

  • Corresponding author: ZHAO Ning, 
  • Received Date: 11 July 2013
    Available Online: 3 September 2013

    Fund Project: 科技部国家科技支撑计划(2013BAC11B02) (2013BAC11B02)国家自然科学基金(21301186)。 (21301186)

  • The thermochemical CO2 splitting activity of NiFe2O4 and NiFe2O4/ZrO2 prepared by the conventional co-precipitation method was investigated with thermogravimetric analysis (TGA) technique. Significant sintering was observed over the two samples during cyclic reactions because of the high reaction temperature. This would lead to an incomplete re-oxidation of the reduced sample in the CO2 splitting reaction. Introduction of ZrO2 could greatly enhance the thermal stability of NiFe2O4, and hence, the cycling behavior in repeated cycles. The catalytic results of NiFe2O4/ZrO2 for cyclic splitting of CO2 in a high-temperature furnace indicate that CO productivity increased with the thermal reduction temperature, while the cycling stability severely decreased with the cyclic number.
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