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Citation: WANG Mei, ZHANG Li-qi, LIU Hao, ZHANG Jun-ying, ZHENG Chu-guang. Studies on CO2 absorption performance by imidazole-based ionic liquid mixtures[J]. Journal of Fuel Chemistry and Technology, ;2012, 40(10): 1264-1268. shu

Studies on CO2 absorption performance by imidazole-based ionic liquid mixtures

  • 1.

    1. State Key Laboratory of Coal Combustion, Huazhong University of Science and Technology, Wuhan 430074, China;

  • Corresponding author: ZHANG Li-qi, 
  • Received Date: 28 April 2012
    Available Online: 14 July 2012

    Fund Project: 国家自然科学基金(51076056, 51021065) (51076056, 51021065) 国家重点基础研究发展规划(973计划, 2011CB707301) (973计划, 2011CB707301) 煤燃烧国家重点实验室开放基金(FSKLCC1111)。 (FSKLCC1111)

  • Conventional and functional imidazole-based ionic liquids (abbr. ILs) were mixed based on their advantage and disadvantage on CO2 reduction. Additionally, CO2 absorption effect and regeneration performance of imidazole-based IL mixtures were discussed. It was showed that imidazole-based IL mixtures had good fluidity and smooth of transferring CO2. It had better absorption capacity of CO2 for the mixtures of [bmim][BF4] (or [bmim][Tf2N]) and [NH2e-mim][BF4] than the single IL, and lower absorption capacity for the mixtures of [bmim][CH3CO2] and [NH2e-mim][BF4] than [bmim][CH3CO2]. While the cation of conventional imidazolium ILs became longer and the mixtures could absorb CO2 more obviously, more strong effect was shown on CO2 absorption with the anion [Tf2N] than the anion [BF4] for the conventional imidazolium IL. CO2 absorption capacity of the imidazole-based IL mixtures had maintained 75%~85% of the initial capacity during 10 times of the absorption/regeneration cycles, while the quality of the regeneration was unchanged.
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