Citation: Changjun You, Chunchun Wang, Mingjie Cai, Yanping Liu, Baikang Zhu, Shijie Li. Improved Photo-Carrier Transfer by an Internal Electric Field in BiOBr/N-rich C₃N₅ 3D/2D S-Scheme Heterojunction for Efficiently Photocatalytic Micropollutant Removal[J]. Acta Physico-Chimica Sinica, ;2024, 40(11): 240701. doi: 10.3866/PKU.WHXB202407014 shu

Improved Photo-Carrier Transfer by an Internal Electric Field in BiOBr/N-rich C₃N₅ 3D/2D S-Scheme Heterojunction for Efficiently Photocatalytic Micropollutant Removal

Changjun You ^{1, †} ,
Chunchun Wang ^{1, †} ,
Mingjie Cai ² ,
Yanping Liu ^1,, ,
Baikang Zhu ^1,, ,
Shijie Li ^1,,

1.
Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control, National Engineering Research Center for Marine Aquaculture, Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, Zhejiang Ocean University, Zhoushan 316022, Zhejiang Province, China
2.
College of Environmental Science and Engineering, State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China

Corresponding author: Yanping Liu, liuyp@zjou.edu.cn Baikang Zhu, zszbk@126.com Shijie Li, lishijie@zjou.edu.cn

^†

Received Date: 14 July 2024
Revised Date: 12 August 2024
Accepted Date: 13 August 2024
Available Online: 19 August 2024
Fund Project: National Natural Science Foundation of China U1809214the Natural Science Foundation of Zhejiang Province of China LY20E080014the Natural Science Foundation of Zhejiang Province of China LTGN23E080001the Open Research Subject of Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control 2021Y02the Science and Technology Project of Zhoushan 2022C41011

Photocatalytic wastewater decontamination techniques hold eminent promise in mitigating environmental deterioration, yet the lack of distinctive photocatalysts prevents their further large-scale application. Herein, an S-scheme heterojunction photocatalyst BiOBr/C₃N₅ (BBN) was fabricated for efficiently dislodging micropollutants under visible light. Among the BBN samples, the optimal BBN-2 demonstrated exceptional activity in photocatalytic TC removal with a rate constant of 0.0139 min^‒1, which surpassed that of pure BiOBr and C₃N₅ by 0.6 and 2.8 times, respectively. The spatially segregated photoredox sites and efficient photo-carrier separation propelled by an internal electric field are found to play a cardinal role in promoting photoreaction kinetics. Moreover, BBN-2 exhibited remarkable resistance to environmental interference and stability, retaining a high activity level after five runs. Through active radical detection, •O₂^‒, h⁺ and •OH were identified as the primary active species in the photocatalytic reaction process. This research would encourage the exploration of C₃N₅-based photocatalysts for environmental protection.
- C₃N₅,
- S-scheme heterojunction,
- Micropollutant removal,
- Internal electric field,
- Photocatalysis
1. [1]
  Xu, H.; Jia, Y.; Sun, Z.; Su, J.; Liu, Q. S.; Zhou, Q.; Jiang, G. Eco-Environ. Health 2022, 1, 31. doi: 10.1016/j.eehl.2022.04.003 doi: 10.1016/j.eehl.2022.04.003
2. [2]
  Li, X.; He, F.; Wang, Z.; Xing, B. Eco-Environ. Health 2022, 1, 181. doi: 10.1016/j.eehl.2022.10.001 doi: 10.1016/j.eehl.2022.10.001
3. [3]
  Li, S.; Liu, Y.; Wu, Y.; Hu, J.; Zhang, Y.; Sun, Q.; Sun, W.; Geng, J.; Liu, X.; Jia, D.; et al. Natl. Sci. Open 2022, 1, 20220029. doi: 10.1360/nso/20220029 doi: 10.1360/nso/20220029
4. [4]
  Mangla, D.; Annu; Sharma, A.; Ikram, S. J. Hazard Mater. 2022, 425, 127946. doi: 10.1016/j.jhazmat.2021.127946 doi: 10.1016/j.jhazmat.2021.127946
5. [5]
  Loffler, P.; Escher, B. I.; Baduel, C.; Virta, M. P.; Lai, F. Y. Environ. Sci. Technol. 2023, 57, 9474. doi: 10.1021/acs.est.2c09854 doi: 10.1021/acs.est.2c09854
6. [6]
  Leonel, A. G.; Mansur, H. S. Water Res. 2021, 190, 116693. doi: 10.1016/j.watres.2020.116693 doi: 10.1016/j.watres.2020.116693
7. [7]
  Pulizzi, F.; Sun, W. Nat. Nanotechnol. 2018, 13, 633. doi: 10.1038/s41565-018-0238-4 doi: 10.1038/s41565-018-0238-4
8. [8]
  Jassby, D.; Cath, T. Y.; Buisson, H. Nat. Nanotechnol. 2018, 13, 670. doi: 10.1038/s41565-018-0234-8 doi: 10.1038/s41565-018-0234-8
9. [9]
  Hodges, B. C.; Cates, E. L.; Kim, J.-H. Nat. Nanotech. 2018, 13, 642. doi: 10.1038/s41565-018-0216-x doi: 10.1038/s41565-018-0216-x
10. [10]
  Long T.; Wang Z.; He Y.; Fang J.; Feng J.; Sun Q. J. Liaocheng Univ. (Nat. Sci. Ed. ) 2023, 36, 48. doi: 10.19728/j.issn1672-6634.2023030005 doi: 10.19728/j.issn1672-6634.2023030005
11. [11]
  Šuligoj, A.; Korošec, R. C.; Žerjav, G.; Tušar, N. N.; Štangar, U. L. Topics Curr. Chem. 2022, 380, 51. doi: 10.1007/s41061-022-00409-2 doi: 10.1007/s41061-022-00409-2
12. [12]
  Wang, T.; Wang, H. J.; Lin, J. S.; Yang, J. L.; Zhang, F. L.; Lin, X. M.; Zhang, Y. J.; Jin, S. Z.; Li, J. F. Chin. J. Struct. Chem. 2023, 42, 100066. doi: 10.1016/j.cjsc.2023.100066 doi: 10.1016/j.cjsc.2023.100066
13. [13]
  Chen, L.; A. Maigbay, M.; Li, M.; Qiu, X. Q. Adv. Powder Mater. 2024, 3, 100150. doi: 10.1016/j.apmate.2023.100150 doi: 10.1016/j.apmate.2023.100150
14. [14]
  Lee, J. H.; Hansora, D. P.; Lee, J. S. Chem 2023, 9, 1632. doi: 10.1016/j.chempr.2023.05.040 doi: 10.1016/j.chempr.2023.05.040
15. [15]
  Andrei, V.; Roh, I.; Yang, P. Sci. Adv. 2023, 9, eade9044. doi: 10.1126/sciadv.ade9044 doi: 10.1126/sciadv.ade9044
16. [16]
  Stanley, P. M.; Haimerl, J.; Shustova, N. B.; Fischer, R. A.; Warnan, J. Nat. Chem. 2022, 14, 1342. doi: 10.1038/s41557-022-01093-x doi: 10.1038/s41557-022-01093-x
17. [17]
  Nikoloudakis, E.; Loxpez-Duarte, I.; Georgios Charalambidis; Ladomenou, K.; Ince, M.; Coutsolelos, A. G. Chem. Soc. Rev. 2022, 51, 6965. doi: 10.1039/d2cs00183g doi: 10.1039/d2cs00183g
18. [18]
  Mateo, D.; Cerrillo, J. L.; Durini, S.; Gascon, J. Chem. Soc. Rev. 2021, 50, 2173. doi: 10.1039/d0cs00357c doi: 10.1039/d0cs00357c
19. [19]
  Koya, A. N.; Zhu, X.; Ohannesian, N.; Yanik, A. A.; Alabastri, A.; Proietti Zaccaria, R.; Krahne, R.; Shih, W.-C.; Garoli, D. ACS Nano 2021, 15, 6038. doi: 10.1021/acsnano.0c10945 doi: 10.1021/acsnano.0c10945
20. [20]
  Moss, B.; Wang, Q.; Butler, K. T.; Grau-Crespo, R.; Selim, S.; Regoutz, A.; Hisatomi, T.; Godin, R.; Payne, D. J.; Kafizas, A.; et al. Nat. Mater. 2021, 20, 511. doi: 10.1038/s41563-020-00868-2 doi: 10.1038/s41563-020-00868-2
21. [21]
  Goto, Y.; Hisatomi, T.; Wang, Q.; Higashi, T.; Ishikiriyama, K.; Maeda, T.; Sakata, Y.; Okunaka, S.; Tokudome, H.; Katayama, M.; et al. Joule 2017, 2, 509. doi: 10.1016/j.joule.2017.12.009 doi: 10.1016/j.joule.2017.12.009
22. [22]
  Kosco, J.; Bidwell, M.; Cha, H.; Martin, T.; Howells, C. T.; Sachs, M.; Anjum, D. H.; Lopez, S. G.; Zou, L.; Wadsworth, A.; et al. Nat. Mater. 2020, 19, 559. doi: 10.1038/s41563-019-0591-1 doi: 10.1038/s41563-019-0591-1
23. [23]
  Lu Y.; Zou X; Wang L.; Geng Y. J. Liaocheng Univ. (Nat. Sci. Ed. ) 2023, 36, 57. doi: 10.19728/j.issn1672-6634.2023040004 doi: 10.19728/j.issn1672-6634.2023040004
24. [24]
  Jiao, L.; Jiang, H.-L. Chin. J. Catal. 2023, 45, 1. doi: 10.1016/S1872-2067(22)64193-7 doi: 10.1016/S1872-2067(22)64193-7
25. [25]
  Jing, L. Q.; Xu, Y. G.; Xie, M.; Wu, C. C.; Zhao, H.; Wang, J.; Wang, H.; Yan, Y. B.; Zhong, N.; Li, H. M.; et al. J. Mater. Sci. Technol. 2024, 177, 10. doi: 10.1016/j.jmst.2023.07.064 doi: 10.1016/j.jmst.2023.07.064
26. [26]
  Niu J.; Wang L.; Meng X.; Li C. J. Liaocheng Univ. (Nat. Sci. Ed. ) 2024, 37, 36. doi: 10.19728/j.issn1672-6634.2023050002 doi: 10.19728/j.issn1672-6634.2023050002
27. [27]
  Zhang, L. X.; Qi, M. Y.; Tang, Z. R.; Xu, Y. J. Research 2023, 6, 0073. doi: 10.34133/research.0073 doi: 10.34133/research.0073
28. [28]
  Li, B.; Wang, T.; Le, Q.; Qin, R.; Zhang, Y.; Zeng, H. C. Nano Mater. Sci. 2023, 5, 293. doi: 10.1016/j.nanoms.2022.05.001 doi: 10.1016/j.nanoms.2022.05.001
29. [29]
  Huang, W.; Bo, T.; Zuo, S.; Wang, Y.; Chen, J.; Ould-Chikh, S.; Li, Y.; Zhou, W.; Zhang, J.; Zhang, H. SusMat 2022, 2, 466. doi: 10.1002/sus2.76 doi: 10.1002/sus2.76
30. [30]
  Wang, Z.; Sun, Z.; Yin, H.; Wei, H.; Peng, Z.; Pang, Y. X.; Jia, G.; Zhao, H.; Pang, C. H.; Yin, Z. eScience 2023, 3, 100136. doi: 10.1016/j.esci.2023.100136 doi: 10.1016/j.esci.2023.100136
31. [31]
  Zhou, W.; Jing, Q.; Li, J.; Chen, Y.; Hao, G.; Wang, L.-N. Acta Phys.-Chim.Sin. 2023, 39, 2211010. doi: 10.3866/PKU.WHXB202211010 doi: 10.3866/PKU.WHXB202211010
32. [32]
  Chong, W.; Meng, R.; Liu, Z.; Liu, Q.; Hu, J.; Zhu, B.; Macharia, D. K.; Chen, Z.; Zhang, L. Adv. Fiber Mater. 2023, 5, 1063. doi: 10.1007/s42765-023-00276-6 doi: 10.1007/s42765-023-00276-6
33. [33]
  Han, Z.; Lv, M.; Shi, X.; Li, G.; Zhao, J.; Zhao, X. Adv. Fiber Mater. 2023, 5, 266. doi: 10.1007/s42765-022-00220-0 doi: 10.1007/s42765-022-00220-0
34. [34]
  Banoo, M.; Kaur, J.; Sah, A. K.; Roy, R. S.; Bhakar, M.; Kommula, B.; Sheet, G.; Gautam, U. K. ACS Appl. Mater. Interfaces 2023, 15, 32425. doi: 10.1021/acsami.3c04959 doi: 10.1021/acsami.3c04959
35. [35]
  Kumar, A.; Rana, A.; Sharma, G.; Naushad, M.; Sillanpää, M.; Guo, C.; Katubi, K. M. M.; Alzahrani, F. M.; Dhiman, P.; Stadler, F. J. Chem. Eng. J. 2021, 423, 130173. doi: 10.1016/j.cej.2021.130173 doi: 10.1016/j.cej.2021.130173
36. [36]
  Bera, S.; Ghosh, S.; Maiyalagan, T.; Basu, R. N. ACS Appl. Energy Mater. 2022, 5, 3821. doi: 10.1021/acsaem.2c00296 doi: 10.1021/acsaem.2c00296
37. [37]
  Ahmadi, Y.; Kim, K. H. Renew. Sustain. Energy Rev. 2024, 189, 113948. doi: 10.1016/j.rser.2023.113948 doi: 10.1016/j.rser.2023.113948
38. [38]
  Luo, C.; Long, Q.; Cheng, B.; Zhu, B.; Wang, L. Acta Phys.-Chim.Sin. 2023, 39, 2212026. doi: 10.3866/PKU.WHXB202212026 doi: 10.3866/PKU.WHXB202212026
39. [39]
  Zu, X.; Zhao, Y.; Li, X.; Chen, R.; Shao, W.; Wang, Z.; Hu, J.; Zhu, J.; Pan, Y.; Sun, Y.; Xie, Y. Angew. Chem. Int. Ed. 2021, 60, 13840. doi: 10.1002/anie.202101894 doi: 10.1002/anie.202101894
40. [40]
  Rahaman, M.; Andrei, V.; Wright, D.; Lam, E.; Pornrungroj, C.; Bhattacharjee, S.; Pichler, C. M.; Greer, H. F.; Baumberg, J. J.; Reisner, E. Nat. Energy 2022, 8, 629. doi: 10.1038/s41560-023-01262-3 doi: 10.1038/s41560-023-01262-3
41. [41]
  Estrada-Pomares, J.; Ramos-Terrón, S.; Lasarte-Aragonés, G.; Lucena, R.; Cárdenas, S.; Rodríguez-Padrón, D.; Luque, R.; Miguel, G. d. J. Mater. Chem. A 2022, 10, 11298. doi: 10.1039/D1TA10323G doi: 10.1039/D1TA10323G
42. [42]
  Kumar, R.; Raizada, P.; Verma, N.; Hosseini-Bandegharaei, A.; Vijay Kumar Thakur; Le, Q. V.; Nguyen, V.-H.; Selvasembian, R.; Singh, P. J. Clean. Prod. 2021, 297, 126617. doi: 10.1016/j.jclepro.2021.126617 doi: 10.1016/j.jclepro.2021.126617
43. [43]
  Jin, X.; Ye, L.; Xie, H.; Chen, G. Coordin. Chem. Rev. 2017, 349, 84. doi: 10.1016/j.ccr.2017.08.010 doi: 10.1016/j.ccr.2017.08.010
44. [44]
  Shi, Y.; Yang, Z.; Shi, L.; Li, H.; Liu, X.; Zhang, X.; Cheng, J.; Liang, C.; Cao, S.; Guo, F.; et al. Environ. Sci. Technol. 2022, 56, 14478. doi: 10.1021/acs.est.2c03769 doi: 10.1021/acs.est.2c03769
45. [45]
  Wu, J.; Li, X.; Shi, W.; Ling, P.; Sun, Y.; Jiao, X.; Gao, S.; Liang, L.; Xu, J.; Yan, W.; et al. Angew. Chem. Int. Ed. 2018, 130, 8855. doi: 10.1002/ange.201803514 doi: 10.1002/ange.201803514
46. [46]
  Huo, Y.; Zhang, J.; Miao, M.; Jin, Y. Appl. Catal. B 2012, 111–112, 334. doi: 10.1016/j.apcatb.2011.10.016 doi: 10.1016/j.apcatb.2011.10.016
47. [47]
  Imam, S. S.; Adnan, R.; Kaus, N. H. M. J. Environ. Chem. Eng. 2021, 9, 105404. doi: 10.1016/j.jece.2021.105404 doi: 10.1016/j.jece.2021.105404
48. [48]
  Wang, C.; Rong, K.; Liu, Y.; Yang, F.; Li, S. Sci. China Mater. 2024, 67, 562. doi: 10.1007/s40843-023-2764-8 doi: 10.1007/s40843-023-2764-8
49. [49]
  Yu, Q.; Chen, J.; Li, Y.; Wen, M.; Liu, H.; Li, G.; An, T. Chin. J. Catal. 2020, 41, 1603. doi: 10.1016/S1872-2067(19)63496-0 doi: 10.1016/S1872-2067(19)63496-0
50. [50]
  Bi, J.; Zhang, Z.; Tian, J.; Huang, G. J. Colloid Interface Sci. 2024, 661, 761. doi: 10.1016/j.jcis.2024.01.213 doi: 10.1016/j.jcis.2024.01.213
51. [51]
  Lee, D. E.; Mameda, N.; Reddy, K. P.; Abraham, B. M.; Jo, W. K.; Tonda, S. J. Mater. Sci. Technol. 2023, 161, 74. doi: 10.1016/j.jmst.2023.03.024 doi: 10.1016/j.jmst.2023.03.024
52. [52]
  Zhu, B.; Sun, J.; Zhao, Y.; Zhang, L.; Yu, J. Adv. Mater. 2024, 36, 2310600. doi: 10.1002/adma.202310600 doi: 10.1002/adma.202310600
53. [53]
  Yu J.; Yao X.; Su P.; Wang S.; Zhang D.; Ge B.; Pu X. J. Liaocheng Univ. (Nat. Sci. Ed. ) 2024, 37, 52. doi: 10.19728/j.issn1672-6634.2023090011 doi: 10.19728/j.issn1672-6634.2023090011
54. [54]
  Wang, L.; Bie, C.; Yu, J. Trends Chem. 2022, 4, 973. doi: 10.1016/j.trechm.2022.08.008 doi: 10.1016/j.trechm.2022.08.008
55. [55]
  Dong, K.; Shen, C.; Yan, R.; Liu, Y.; Zhuang, C.; Li, S. Acta Phys.-Chim.Sin. 2024, 40, 2310013. doi: 10.3866/PKU.WHXB202310013 doi: 10.3866/PKU.WHXB202310013
56. [56]
  Yousefi, S. R.; Ghanbari, M.; Amiri, O.; Marzhoseyni, Z.; Mehdizadeh, P.; Hajizadeh-Oghaz, M.; Salavati-Niasari, M. J. Am. Ceram. Soc. 2021, 104, 2952. doi: 10.1111/jace.17696 doi: 10.1111/jace.17696
57. [57]
  Kumar, A.; Khosla, A.; Sharma, S. K.; Dhiman, P.; Sharma, G.; Gnanasekaran, L.; Naushad, M.; Stadler, F. J. Fuel 2023, 333, 126267. doi: 10.1016/j.fuel.2022.126267 doi: 10.1016/j.fuel.2022.126267
58. [58]
  Chen, Y.; Wang, Z.; Zhang, Y.; Wei, P.; Xu, W.; Wang, H.; Yu, H.; Jia, J.; Zhang, K.; Peng, C. ACS Appl. Mater. Interfaces 2023, 15, 20027. doi: 10.1021/acsami.2c21049 doi: 10.1021/acsami.2c21049
59. [59]
  Yu, W.; Bie, C. Acta Phys.-Chim.Sin. 2024, 40, 2307022. doi: 10.3866/PKU.WHXB202307022 doi: 10.3866/PKU.WHXB202307022
60. [60]
  Deng, X.; Zhang, J.; Qi, K.; Liang, G.; Xu, F.; Yu, J. Nat. Commun. 2024, 15, 4807. doi: 10.1038/s41467-024-49004-7 doi: 10.1038/s41467-024-49004-7
61. [61]
  Kim, I. Y.; Kim, S.; Jin, X.; Premkumar, S.; Chandra, G.; Lee, N.-S.; Mane, G. P.; Hwang, S.-J.; Umapathy, S.; Vinu, A. Angew. Chem. Int. Ed. 2018, 57, 17135. doi: 10.1002/ange.201811061 doi: 10.1002/ange.201811061
62. [62]
  Kumar, P.; Vahidzadeh, E.; Thakur, U. K.; Kar, P.; Alam, K. M.; Goswami, A.; Mahdi, N.; Cui, K.; Bernard, G. M.; Michaelis, V. K.; et al. J. Am. Chem. Soc. 2019, 141, 5415. doi: 10.1021/jacs.9b00144 doi: 10.1021/jacs.9b00144
63. [63]
  Monga, D.; Basu, S. J. Environ. Manage. 2023, 336, 117570. doi: 10.1016/j.jenvman.2023.117570 doi: 10.1016/j.jenvman.2023.117570
64. [64]
  Wu, B.; Sun, T.; Liu, N.; Lu, L.; Zhang, R.; Shi, W.; Cheng, P. ACS Appl. Mater. Interfaces 2022, 14, 26742. doi: 10.1021/acsami.2c04729 doi: 10.1021/acsami.2c04729
65. [65]
  Ng, S.-F.; Chen, X.; Foo, J. J.; Xiong, M.; Ong, W.-J. Chin. J. Catal. 2023, 47, 150. doi: 10.1016/S1872-2067(23)64417-1 doi: 10.1016/S1872-2067(23)64417-1
66. [66]
  Huang, H.; Verhaeghe, D.; Weng, B.; Ghosh, B.; Zhang, H.; Hofkens, J.; Steele, J. A.; Roeffaers, M. B. J. Angew. Chem. Int. Ed. 2022, 134, e202203261. doi: 10.1002/ange.202203261 doi: 10.1002/ange.202203261
67. [67]
  Li, H.; Zhou, Y.; Tu, W.; Ye, J.; Zou, Z. Adv. Funct. Mater. 2015, 25, 998. doi: 10.1002/adfm.201401636 doi: 10.1002/adfm.201401636
68. [68]
  Afroz, K.; Moniruddin, M.; Bakranov, N.; Kudaibergenovbc, S.; Nuraje, N. J. Mater. Chem. A 2018, 6, 21696. doi: 10.1039/C8TA04165B doi: 10.1039/C8TA04165B
69. [69]
  Marschall, R. Adv. Funct. Mater. 2014, 24, 2421. doi: 10.1002/adfm.201303214. doi: 10.1002/adfm.201303214
70. [70]
  Kumar, A.; Krishnan, V. Adv. Funct. Mater. 2021, 31, 2009807. doi: 10.1002/adfm.202009807 doi: 10.1002/adfm.202009807
71. [71]
  Han, T.; Cao, X.; Chen, H.-C.; Ma, J.; Yu, Y.; Li, Y.; Xu, W.; Sun, K.; Huang, A.; Chen, Z.; et al. Angew. Chem. Int. Ed. 2023, 62, e202313325. doi: 10.1002/anie.202313325 doi: 10.1002/anie.202313325
72. [72]
  Dutta, V.; Sudhaik, A.; Raizada, P.; Singh, A.; Ahamad, T.; Thakur, S.; Le, Q. V.; Nguyen, V.-H.; Singh, P. J. Mater. Sci. Technol. 2024, 162, 11. doi: 10.1016/j.jmst.2023.03.037 doi: 10.1016/j.jmst.2023.03.037
73. [73]
  Liu, C.; Mao, S.; Shi, M.; Wang, F.; Xia, M.; Chen, Q.; Ju, X. J. Hazard. Mater. 2021, 420, 126613. doi: 10.1016/j.jhazmat.2021.126613 doi: 10.1016/j.jhazmat.2021.126613
74. [74]
  Zhang, L.; Wu, Y.; Tsubaki, N.; Jin, Z. Acta Phys.-Chim.Sin. 2023, 39, 2302051. doi: 10.3866/PKU.WHXB202302051 doi: 10.3866/PKU.WHXB202302051
75. [75]
  Shang, W.; Liu, W.; Cai, X.; Hu, J.; Guo, J.; Xin, C.; Li, Y.; Zhang, N.; Wang, N.; Hao, C.; Shi, Y. Adv. Powder Mater. 2023, 2, 100094. doi: 10.1016/j.apmate.2022.100094 doi: 10.1016/j.apmate.2022.100094
76. [76]
  Zhuang, C.; Chang, Y.; Li, W.; Li, S.; Xu, P.; Zhang, H.; Zhang, Y.; Zhang, C.; Gao, J.; Chen, G.; Zhang, T.; Kang, Z.; Han, X. ACS Nano 2024, 18, 5206. doi: 10.1021/acsnano.4c00217 doi: 10.1021/acsnano.4c00217
77. [77]
  Selvaraj, V.; Ong, W.-J.; Pandikumar, A. Coordin. Chem. Rev. 2022, 464, 214541. doi: 10.1016/j.ccr.2022.214541 doi: 10.1016/j.ccr.2022.214541
78. [78]
  Li, Y.; Li, Z.; Liu, E. J. J. Liaocheng Univ. (Nat. Sci. Ed. ) 2023, 36, 1. doi: 10.19728/j.issn1672-6634.2022090001. doi: 10.19728/j.issn1672-6634.2022090001
79. [79]
  Bariki, R.; Pradhan, S. K.; Panda, S.; Nayak, S. K.; Pati, A. R.; Mishra, B. G. Langmuir 2023, 39, 7707. doi: 10.1021/acs.langmuir.3c00519 doi: 10.1021/acs.langmuir.3c00519
80. [80]
  Wadsworth, A.; Hamid, Z.; Kosco, J.; Gasparini, N.; McCulloch, I. Adv. Mater. 2020, 32, 2001763. doi: 10.1002/adma.202001763 doi: 10.1002/adma.202001763
81. [81]
  Mandal, S.; Adhikari, S.; Choi, S.; Lee, Y.; Kim, D.-H. Chem. Eng. J. 2022, 444, 136609. doi: 10.1016/j.cej.2022.136609 doi: 10.1016/j.cej.2022.136609
82. [82]
  Sun, T.; Li, C.; Bao, Y.; Fan, J.; Liu, E. Acta Phys.-Chim.Sin. 2023, 39, 2212009. doi: 10.3866/PKU.WHXB202212009 doi: 10.3866/PKU.WHXB202212009
1. [1]
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Improved Photo-Carrier Transfer by an Internal Electric Field in BiOBr/N-rich C3N5 3D/2D S-Scheme Heterojunction for Efficiently Photocatalytic Micropollutant Removal

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通讯作者: 陈斌, bchen63@163.com

Improved Photo-Carrier Transfer by an Internal Electric Field in BiOBr/N-rich C₃N₅ 3D/2D S-Scheme Heterojunction for Efficiently Photocatalytic Micropollutant Removal