Citation: Qin Hu, Liuyun Chen, Xinling Xie, Zuzeng Qin, Hongbing Ji, Tongming Su. Construction of Electron Bridge and Activation of MoS₂ Inert Basal Planes by Ni Doping for Enhancing Photocatalytic Hydrogen Evolution[J]. Acta Physico-Chimica Sinica, ;2024, 40(11): 240602. doi: 10.3866/PKU.WHXB202406024 shu

Construction of Electron Bridge and Activation of MoS₂ Inert Basal Planes by Ni Doping for Enhancing Photocatalytic Hydrogen Evolution

Qin Hu ¹ ,
Liuyun Chen ¹ ,
Xinling Xie ¹ ,
Zuzeng Qin ¹ ,
Hongbing Ji ^{1, 2} ,
Tongming Su ^1,,

1.
Guangxi Key Laboratory of Petrochemical Resource Processing and Process Intensification Technology, School of Chemistry and Chemical Engineering, Guangxi University, Nanning 530004, China
2.
Institute of Green Petroleum Processing and Light Hydrocarbon Conversion, College of Chemical Engineering, Zhejiang University of Technology, Hangzhou 310014, China

Corresponding author: Tongming Su, sutm@gxu.edu.cn
Received Date: 20 June 2024
Revised Date: 20 July 2024
Accepted Date: 22 July 2024
Available Online: 12 August 2024
Fund Project: the National Natural Science Foundation of China 22208065Guangxi Natural Science Foundation 2022GXNSFBA035483Opening Project of Guangxi Key Laboratory of Petrochemical Resource Processing and Process Intensification Technology 2023K012

Photocatalytic hydrogen production is one of the effective ways to address environmental pollution and energy crises. Herein, Ni_x-MoS₂/ZnIn₂S₄ heterojunctions were constructed to improve the separation efficiency of photogenerated electrons and holes and increase the number of active sites for hydrogen evolution. According to the catalyst characterization and theoretical calculations, the Ni at the interface between Ni_x-MoS₂ and ZnIn₂S₄ can act as a bridge for charge transfer, the Ni―S bond is the active site for H₂O dissociation, and the S site near the S vacancy on the Ni_x-MoS₂ surface enhances the hydrogen evolution reaction. Benefiting from the synergistic effect of the S vacancy and the Ni-doped MoS₂ cocatalyst, the optimal Ni_0.08-MoS₂/ZnIn₂S₄ exhibited the best hydrogen production rate of 7.13 mmol∙h⁻¹∙g⁻¹, which is 12.08 times than that of ZnIn₂S₄. This work provides a new strategy for enhancing photocatalytic efficiency through the synergistic effect of surface vacancies and doping and the optimization of heterojunctions.
- Photocatalytic,
- Hydrogen,
- ZnIn₂S₄,
- MoS₂,
- Doping
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Construction of Electron Bridge and Activation of MoS2 Inert Basal Planes by Ni Doping for Enhancing Photocatalytic Hydrogen Evolution

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通讯作者: 陈斌, bchen63@163.com

Construction of Electron Bridge and Activation of MoS₂ Inert Basal Planes by Ni Doping for Enhancing Photocatalytic Hydrogen Evolution