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Citation: Asif Hassan Raza, Shumail Farhan, Zhixian Yu, Yan Wu. Double S-Scheme ZnS/ZnO/CdS Heterostructure Photocatalyst for Efficient Hydrogen Production[J]. Acta Physico-Chimica Sinica, ;2024, 40(11): 240602. doi: 10.3866/PKU.WHXB202406020 shu

Double S-Scheme ZnS/ZnO/CdS Heterostructure Photocatalyst for Efficient Hydrogen Production

  • Faculty of Materials Science and Chemistry, China University of Geosciences, Wuhan 430078, China

  • Corresponding author: Yan Wu, wuyan@cug.edu.cn
  • Received Date: 17 June 2024
    Revised Date: 24 July 2024
    Accepted Date: 29 July 2024
    Available Online: 12 August 2024

    Fund Project: the National Natural Science Foundation of China 22378372

  • This work illustrates the novelty of double S-scheme ZnS/ZnO/CdS ternary heterojunction photocatalyst with efficient photocatalytic activity. The sample with optimal CdS content, ZnS/ZnO/CdS-14% (ZZC14%), displayed the maximum H2 evolution rate of 4.1 mmol·g‒1·h‒1. The maximum photocatalytic performance was approximately 2 and 13 times higher than their corresponding counterparts, ZnS/CdS and ZnO/ZnS, respectively. A high AQE of 19.8% under 420 nm was obtained. Additionally, the slight changes in H2 evolution activities and retentions of crystal structures after six successive cycles indicate the stability of the photocatalyst. In accordance with the theoretical calculations and experimental results, the remarkable enhancement in photocatalytic activity is attributed to fast electron transfer and separation as well as the intimate contact due to mutual interaction between S-scheme. This work highlights an innovative approach to constructing a dual S-scheme photocatalytic system with high separation and fast migration capabilities of photogenerated charge carriers for splitting water to produce hydrogen.
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