Citation: Jizhou Liu, Chenbin Ai, Chenrui Hu, Bei Cheng, Jianjun Zhang. Accelerated Interfacial Electron Transfer in Perovskite Solar Cell by Ammonium Hexachlorostannate Modification and fs-TAS Investigation[J]. Acta Physico-Chimica Sinica, ;2024, 40(11): 240200. doi: 10.3866/PKU.WHXB202402006 shu

Accelerated Interfacial Electron Transfer in Perovskite Solar Cell by Ammonium Hexachlorostannate Modification and fs-TAS Investigation

1.
State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China
2.
Laboratory of Solar Fuel, Faculty of Materials Science and Chemistry, China University of Geosciences, Wuhan 430078, China

Corresponding author: Jianjun Zhang, zhangjianjun@cug.edu.cn
Received Date: 5 February 2024
Revised Date: 28 February 2024
Accepted Date: 28 February 2024
Available Online: 4 March 2024
Fund Project: the National Natural Science Foundation of China 52073223the National Natural Science Foundation of China 22278324the National Natural Science Foundation of China 52202375Natural Science Foundation of Hubei Province of China 2022CFA001

Organic-inorganic halide perovskite solar cells (PSCs) have received widespread attention due to their outstanding photovoltaic performance and straightforward preparation process. However, charge recombination at the interface is a crucial factor limiting further enhancement of the power conversion efficiency (PCE) of the PSCs. In this study, we report the interfacial modification between the electron transport layer and the perovskite film (PSK) using ammonium hexachlorostannate (AH) crystals synthesized via the room temperature spin-coating method. AH as an inorganic tin-based perovskite material, can passivate defects in the PSK and establish a better lattice match, thereby enhancing the quality and crystallinity of the PSK. Kelvin probe force microscopy results confirm that AH promotes the directional migration of photogenerated electrons. Femtosecond transient absorption spectroscopy results verify that AH effectively shortens the lifetime of electron extraction and facilitates interfacial electron transfer. Based on the benefits of AH modification, AH-based PSCs exhibit higher PCE and reduced hysteresis effect.
- Interface modification,
- Lattice matching,
- Femtosecond transient absorption spectra,
- Electron transfer kinetics,
- Electron dynamics
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