Citation: Qi Li, Pingan Li, Zetong Liu, Jiahui Zhang, Hao Zhang, Weilai Yu, Xianluo Hu. Fabricating Micro/Nanostructured Separators and Electrode Materials by Coaxial Electrospinning for Lithium-Ion Batteries: From Fundamentals to Applications[J]. Acta Physico-Chimica Sinica, ;2024, 40(10): 231103. doi: 10.3866/PKU.WHXB202311030 shu

Fabricating Micro/Nanostructured Separators and Electrode Materials by Coaxial Electrospinning for Lithium-Ion Batteries: From Fundamentals to Applications

Qi Li ¹ ,
Pingan Li ¹ ,
Zetong Liu ¹ ,
Jiahui Zhang ¹ ,
Hao Zhang ¹ ,
Weilai Yu ^2,, ,
Xianluo Hu ^1,,

1.
State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China;
2.
Department of Chemical Engineering, Stanford University, Stanford CA 94305, USA

Corresponding author: Weilai Yu, Xianluo Hu,
Received Date: 23 November 2023
Revised Date: 12 December 2023
Accepted Date: 14 December 2023

Fund Project: This project was supported by the National Natural Foundation Science of China (52272206, 51972132).

Highly coveted for their exceptional energy density, extended cycle life, impressive rate capability, and thermal stability, lithium-ion batteries (LIBs) stand out as the optimal power sources for real-world applications, ranging from portable electronics to electric vehicles (EVs). In this context, coaxial electrospinning has emerged as a compelling technique for fabricating nanofiber materials endowed with properties ideally suited for LIBs. These properties include a high specific surface area, exceptional porosity, a substantial aspect ratio, and facile surface modification. This comprehensive review encapsulates the fundamental principles, practical applications, and recent strides in coaxial electrospinning, particularly in the preparation of crucial LIB components such as cathodes, anodes, and separators. The intricate relationships between the micro/nanostructures of coaxially electrospun fiber materials and their resultant battery performances are meticulously examined. Additionally, the review outlines future directions and underscores the challenges inherent in advancing the field of coaxial electrospinning for LIBs.
- Lithium-ion batteries,
- Coaxial electrospinning,
- Micro/nanostructured materials,
- Core-shell structures,
- Electrochemical performance
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