Citation: Rui Li, Huan Liu, Yinan Jiao, Shengjian Qin, Jie Meng, Jiayu Song, Rongrong Yan, Hang Su, Hengbin Chen, Zixuan Shang, Jinjin Zhao. Emerging Irreversible and Reversible Ion Migrations in Perovskites[J]. Acta Physico-Chimica Sinica, ;2024, 40(11): 231101. doi: 10.3866/PKU.WHXB202311011 shu

Emerging Irreversible and Reversible Ion Migrations in Perovskites

Rui Li ^{1, 2, †} ,
Huan Liu ^{1, 2, †} ,
Yinan Jiao ^{2, †} ,
Shengjian Qin ² ,
Jie Meng ^{1, 2} ,
Jiayu Song ^{1, 2} ,
Rongrong Yan ^{1, 2} ,
Hang Su ^{1, 2} ,
Hengbin Chen ^{1, 2} ,
Zixuan Shang ¹ ,
Jinjin Zhao ^1,,

1.
Hebei Technology Innovation Center for Energy Conversion Materials and Devices, Hebei Key Laboratory of Inorganic Nanomaterials, Engineering Research Center of Thin Film Solar Cell Materials and Devices, Hebei Province, College of Chemistry and Materials Science, Hebei Normal University, Shijiazhuang 050024, China
2.
School of Materials Science and Engineering, Shijiazhuang Tiedao University, Shijiazhuang 050043, China

Corresponding author: Jinjin Zhao, jinjinzhao2012@163.com; jinjinzhao2023@hebtu.edu.cn

^†

Received Date: 8 November 2023
Revised Date: 17 December 2023
Accepted Date: 8 January 2024
Available Online: 12 January 2024
Fund Project: the National Natural Science Foundation of China U2130128Yanzhao Young Scientist Project from Natural Science Foundation of Hebei Province B2023205040Basic Research Cooperation Special Foundation of Beijing-Tianjin-Hebei Region H2022205047Basic Research Cooperation Special Foundation of Beijing-Tianjin-Hebei Region 22JCZXJC00060Basic Research Cooperation Special Foundation of Beijing-Tianjin-Hebei Region E3B33911DFCentral Government Guiding Local Science and Technology Development Project 216Z4302GHebei Administration for Market Supervision Science and Technology Project List 2023ZC03Innovation Capability Improvement Plan Project of Hebei Province 22567604HPh.D Scientific Research Start-up Fund of Hebei Normal University L2023B18

Metal halide perovskite (MHP) materials show great prospects in applications such as solar cells, luminescent displays, and biomedicines, owing to their outstanding visible light absorption, photoelectric conversion, adjustable energy level structure, and low energy consumption. Their exceptional properties, such as high visible light absorption, efficient photoelectric conversion, adjustable energy level structure, and low energy consumption, have attracted significant attention. However, the presence of ion migration in MHPs has been identified as a critical challenge, leading to reduced energy conversion efficiency and device instability. Overcoming this obstacle is crucial for the commercialization of perovskite-based technologies. In recent years, extensive research has been conducted to understand the conditions and mechanisms of ion migration in perovskite materials, as well as develop strategies to mitigate its adverse effects. This paper adopts a dialectical perspective on ion migration, with a specific focus on energy barriers. A comprehensive review is provided, covering the fundamental concepts and formation mechanisms of both irreversible unidirectional and reversible bidirectional ion migrations. This paper begins by presenting a detailed summary of the degradation processes caused by irreversible unidirectional ion migrations phenomena induced by external fields, including illumination, stress/strain, thermal and electrical fields. Understanding the underlying mechanisms of such degradation is essential to address the stability concerns associated with perovskite devices. Moreover, the overview of bidirectional reversible ion migration phenomena in perovskite is presented. The cyclic formation and restoration of Schottky barriers at the interface can significantly influence the photoelectrical properties and impact the overall performance of perovskite devices. Various strategies for regulating ion migrations under external fields are discussed, aiming to enhance device stability and performance. By understanding the energy landscape and migration pathways, researchers can develop effective strategies to control and optimize ion migrations, ultimately improving the photoelectric conversion performance of perovskite devices. This paper provides comprehensive analysis of ion migration in perovskite materials, addressing fundamental concepts, ion migration mechanisms, and strategies for regulating ion migrations. By providing a clear understanding of the challenges associated with ion migration, this work contributes to the advancement of perovskite-based technologies and facilitates their commercialization. Ultimately, the optimization of ion migration control will lead to improved performance and stability of perovskite devices, enabling their widespread adoption in various applications.
- Halide perovskite,
- Solar cells,
- Ion migration,
- Irreversible unidirectional ion migration,
- Reversible bidirectional ion migration
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