Citation: Li Yan, Hu Xingsheng, Huang Jingwei, Wang Lei, She Houde, Wang Qizhao. Development of Iron-Based Heterogeneous Cocatalysts for Photoelectrochemical Water Oxidation[J]. Acta Physico-Chimica Sinica, ;2021, 37(8): 200902. doi: 10.3866/PKU.WHXB202009022 shu

Development of Iron-Based Heterogeneous Cocatalysts for Photoelectrochemical Water Oxidation

College of Chemistry and Chemical Engineering, Gansu International Scientific and Technological Cooperation Base of Water-Retention Chemical Functional Materials, Research Center of Gansu Military and Civilian Integration Advanced Structural Materials, Northwest Normal University, Lanzhou 730070, China

Author Bio:

Jingwei Huang is currently an associate professor in the school of chemistry and chemical engineering of Northwest Normal University. He obtained Ph.D. degree from Lanzhou University in 2017. Now he is mainly engaged in photoelectrocatalytic and electrocatalytic water splitting to produce hydrogen, and CO₂ reduction

Prof. Qizhao Wang obtained his Ph.D. degree in engineering from Shanghai Jiaotong University. Now he is mainly engaged in the research of new energy materials (hydrogen production by photolysis of water, photoelectric conversion, electrocatalysis, CO₂ photoelectric catalytic reduction), environmental catalysis and water treatment
Corresponding author: Huang Jingwei, huangjingwei2009@163.com Wang Qizhao, wangqizhao@163.com; qizhaosjtu@gmail.com
Received Date: 7 September 2020
Revised Date: 30 September 2020
Accepted Date: 22 October 2020
Available Online: 28 October 2020
Fund Project: the National Natural Science Foundation of China 21808189This work was financially supported by the National Natural Science Foundation of China (21663027, 21808189, 21962018), and the Young Teachers'Research Ability Improvement Project of Northwest Normal University (NWNU-LKQN2020-01)the Young Teachers'Research Ability Improvement Project of Northwest Normal University NWNU-LKQN2020-0the National Natural Science Foundation of China 21962018the National Natural Science Foundation of China 21663027

The use of fossil fuels has caused serious environmental problems such as air pollution and the greenhouse effect. Moreover, because fossil fuels are a non-renewable energy source, they cannot meet the continuously increasing demand for energy. Therefore, the development of clean and renewable energy sources is necessitated. Hydrogen energy is a clean, non-polluting renewable energy source that can ease the energy pressure of the whole society. The sunlight received by the Earth is 1.7× 10¹⁴ J in 1 s, which far exceeds the total energy consumption of humans in one year. Therefore, conversion of solar energy to valuable hydrogen energy is of significance for reducing the dependence on fossil fuels. Since Fujishima and Honda first reported on TiO₂ in 1972, it has been discovered that semiconductors can generate clean, pollution-free hydrogen through water splitting driven by electricity or light. Hydrogen generated through this approach can not only replace fossil fuels but also provide environmentally friendly renewable hydrogen energy, which has attracted considerable attention. Photoelectrochemical (PEC) water splitting can use solar energy to produce clean, sustainable hydrogen energy. Because the oxygen evolution reaction (OER) over a photoanode is sluggish, the overall energy conversion efficiency is considerably low, limiting the practical application of PEC water splitting. A cocatalyst is, thus, necessary to improve PEC water splitting performance. So far, the synthesis of first-row transition-metal-based (e.g., Fe, Co, Ni, and Mn) cocatalysts has been intensively studied. Iron is earth-abundant and less toxic than other transition metals, making it a good cocatalyst. In addition, iron-based compounds exhibit the properties of a semiconductor/metal and have unique electronic structures, which can improve electrical conductivity and water adsorption. Various iron-based catalysts with high activity have been designed to improve the efficiency of PEC water oxidation. This article briefly summarizes the research progress related to the structure, synthesis, and application of iron oxyhydroxides, iron-based layered double hydroxides, and iron-based perovskites and discusses the evaluation of the performance of these cocatalysts toward photoelectrochemical water oxidation.
- Photoelectrochemical water splitting,
- Oxygen evolution reaction,
- Ferric hydroxide,
- Iron-based layered double hydroxide,
- Iron-based perovskites
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