Citation: CHEN Ke, SUN Zhenhua, FANG Ruopian, LI Feng, CHENG Huiming. Development of Graphene-based Materials for Lithium-Sulfur Batteries[J]. Acta Physico-Chimica Sinica, ;2018, 34(4): 377-390. doi: 10.3866/PKU.WHXB201709001 shu

Development of Graphene-based Materials for Lithium-Sulfur Batteries

CHEN Ke ^1,2 ,
SUN Zhenhua ¹ ,
FANG Ruopian ¹ ,
LI Feng ^1,, ,
CHENG Huiming ^1,3,,

1.
Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, P. R. China
2.
School of Physical Science and Technology, Shanghai Tech University, Shanghai 201210, P. R. China
3.
Tsinghua-Berkeley Shenzhen Institute, Tsinghua University, Shenzhen 518055, Guangdong Province, P. R. China

Corresponding author: LI Feng, fli@imr.ac.cn CHENG Huiming, cheng@imr.ac.cn
Received Date: 24 July 2017
Revised Date: 21 August 2017
Accepted Date: 22 August 2017
Available Online: 1 April 2017
Fund Project: the National Key R & D Program of China 2014CB932402the "Strategic Priority Research Program" of the Chinese Academy of Sciences XDA09010104the National Natural Science Foundation of China 51525206the Youth Innovation Promotion Association of the Chinese Academy of Sciences 2015150the Key Research Program of the Chinese Academy of Sciences KGZD-EW-T06the National Natural Science Foundation of China 51521091The project was supported by the National Key R & D Program of China (2016YFA0200102, 2016YFB0100100, 2014CB932402), the National Natural Science Foundation of China (51525206, 51521091, 51372253, U1401243), the "Strategic Priority Research Program" of the Chinese Academy of Sciences (XDA09010104), the Key Research Program of the Chinese Academy of Sciences (KGZD-EW-T06), the Youth Innovation Promotion Association of the Chinese Academy of Sciences (2015150), the Natural Science Foundation of Liaoning Province, China (2015021012), the Institute of Metal Research (2015-PY03), and the CAS/SAFEA International Partnership Program for Creative Research Teamsthe National Natural Science Foundation of China U1401243the National Natural Science Foundation of China 51372253the Institute of Metal Research 2015-PY03the National Key R & D Program of China 2016YFA0200102the Natural Science Foundation of Liaoning Province, China 2015021012the National Key R & D Program of China 2016YFB0100100

Lithium-sulfur (Li-S) batteries are promising electrochemical energy storage systems because of their high theoretical energy density, natural abundance, and environmental benignity. However, several problems such as the insulating nature of sulfur, high solubility of polysulfides, large volume variation of the sulfur cathode, and safety concerns regarding the lithium anode hinder the commercialization of Li-S batteries. Graphene-based materials, with advantages such as high conductivity and good flexibility, have shown effectiveness in realizing Li-S batteries with high energy density and high stability. These materials can be used as the cathode matrix, separator coating layer, and anode protection layer. In this review, the recent progress of graphene-based materials used in Li-S batteries, including graphene, functionalized graphene, heteroatom-doped graphene, and graphene-based composites, has been summarized. And perspectives regarding the development trend of graphene-based materials for Li-S batteries have been discussed.
- Lithium sulfur battery,
- Graphene,
- Doping,
- Functionalization,
- Composites
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