Citation: YAO Xiao-Jiang, NG Ying-Tao, LI Hong-Li, YANG Fu-Mo. Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NO_x by NH₃[J]. Acta Physico-Chimica Sinica, ;2015, 31(5): 817-828. doi: 10.3866/PKU.WHXB201503253 shu

Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NO_x by NH₃

YAO Xiao-Jiang ^1, ,
NG Ying-Tao ^1,2 ,
LI Hong-Li ¹ ,
YANG Fu-Mo ^1,3,

1.
1 Key Laboratory of Reservoir Aquatic Environment of CAS, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714, P. R. China;
2 Chongqing Key Laboratory of Catalysis and Functional Organic Molecules, Chongqing Technology and Business University, Chongqing 400067, P. R. China;
3 Yangtze Normal University, Chongqing 408100, P. R. China

Received Date: 19 January 2015
Available Online: 25 March 2015
Fund Project: 重庆市科学技术委员会项目(cstc2013jcsf20001, cstc2014pt-gc20002) (cstc2013jcsf20001, cstc2014pt-gc20002)重庆文理学院环境材料与修复技术重庆市重点实验室开放课题基金(CEK1405)资助 (CEK1405)

Nitrogen oxides (NO_x), which are emitted from stationary sources (such as coal-fired power plant flue gases) and mobile sources (such as motor vehicle exhausts), cause serious atmospheric pollution. As a result, it is very important to control the emissions of NO_x. Some studies have suggested that NH₃-selective catalytic reduction (NH₃-SCR) of NO_x is one of the best techniques for this purpose. Ceria-based catalysts are widely used in the NH₃-SCR reaction because of their od redox ability, suitable surface acidity, high oxygen storage or release capacity, and rich resource reserves. Investigating the role of ceria component in this reaction is important to understand the nature of the related catalytic process, and provides a valuable scientific reference for the optimization of existing catalysts and the design of novel catalysts. Based on the different roles of ceria in NH₃-SCR catalysts, we have performed a systematic review of the latest research progress of ceria-based catalysts in the NH₃-SCR reaction for the following aspects: CeO₂ used as supports, ceria-based mixed oxides, surface loading components (additives and active species), and ceria-based catalysts with special structures. Finally, we discuss the future directions of this field.
- Ceria-based catalyst,
- Nitrogen oxide,
- Selective catalytic reduction by NH₃,
- Support,
- Mixed oxide,
- Surface loading component,
- Special structure
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Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NOx by NH3

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Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NO_x by NH₃