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Citation: FU Qing-Bin, GAO Bo, SU Ling-Hao, YUAN Chang-Zhou, LU Xiang-Jun, ZHANG Xiao-Gang. Preparation of Polypyrrole/Benzenesulfonic Functionalized Multi-Walled Carbon Nanotubes Induced by Hydrogen Bonding and Their Electrochemical Behavior[J]. Acta Physico-Chimica Sinica, ;2009, 25(11): 2199-2204. doi: 10.3866/PKU.WHXB20091023 shu

Preparation of Polypyrrole/Benzenesulfonic Functionalized Multi-Walled Carbon Nanotubes Induced by Hydrogen Bonding and Their Electrochemical Behavior

1.
College of Material Science and Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, P. R. China

Received Date: 17 April 2009
Available Online: 2 September 2009

Multi-walled carbon nanotubes were functionalized using in situ generated aryl diazonium and were then used to synthesize polypyrrole/benzenesulfonic functionalized multi-walled carbon nanotube composites (PPy/f-MWCNTs). Transmission electron microscopy (TEM) and scanning electron microscopy (SEM) results indicated that a uniform PPy was successfully coated onto the sidewall of the f-MWCNTs, which was induced by hydrogen bonding. Cyclic voltammetry and galvanostatic charge/discharge measurements results showed that the composite possessed od electrochemical capacitive performance. The composite with m(PPy):m(MWCNTs) of 1:1 had a capacity of 266 F·g-1 at a current density of 1.0 A·g-1, and the utilization of PPy was more than one time higher than polypyrrole/un-functionalized multi-walled carbon nanotube composites (PPy/p-MWCNTs) and pure PPy.
- Supercapacitor,
- Polypyrrole,
- Carbon nanotube,
- Benzenesulfonic functionalization
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沈阳化工大学材料科学与工程学院沈阳 110142

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