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Citation: Sha Guohe, Zhong Xian, Zhao Shen, Zhang Cunhao. AN OODR-MPI STUDY OF CARBON MONOXIDE[J]. Acta Physico-Chimica Sinica, ;1985, 1(01): 66-75. doi: 10.3866/PKU.WHXB19850109 shu

AN OODR-MPI STUDY OF CARBON MONOXIDE

1.
Dalian Institute of Chemical Physics; Academia Sinica

Received Date: 17 June 1984
Available Online: 15 February 1985

Optical-optical double resonance multiphoton ionization(OODR-MPI)spectroscopy is a rapidly developing, versatile technique which should find wide applications in both molecular spectroscopy and molecular dynamics.
In an OODR-MPI study of CO, we irradiate the static sample cell by 2 pulsed dye laser beams. The first UV laser light (“pump beam”) resonantly pumps ground state CO to A~1∏ state via a 2-photon process. Then a second visible laser light (“probe beam”) excites CO A~1∏ to B~1∑~+. The excited B~1∑~. The excited B~1∑~+ molecule further under es ionization by absorbing one more UV photon, so the whole process follows a 2+1+1 photon scheme.
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