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Citation: Yi YANG, Shuang WANG, Wendan WANG, Limiao CHEN. Photocatalytic CO2 reduction performance of Z-scheme Ag-Cu2O/BiVO4 photocatalyst[J]. Chinese Journal of Inorganic Chemistry, ;2024, 40(5): 895-906. doi: 10.11862/CJIC.20230434 shu

Photocatalytic CO2 reduction performance of Z-scheme Ag-Cu2O/BiVO4 photocatalyst

  • College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China

  • Corresponding author: Limiao CHEN, chenlimiao@csu.edu.cn
  • Received Date: 20 November 2023
    Revised Date: 21 March 2024

Figures(8)

  • A Z-scheme heterojunction photocatalyst Ag - Cu2 O/BiVO4 was successfully constructed with effective charge carrier separation/transfer by uniformly encapsulating Cu2O nanospheres and Ag nanoparticles on the surface of decahedral BiVO4 using a simple chemical reduction deposition strategy. The photo-reduction of carbon dioxide reaction result indicated that the as - prepared Ag - Cu2O/BiVO4 heterostructure exhibited excellent activity of photo-reduction CO2 with the CO yield of 5.37 μmol·g-1·h-1, about 35.8 times and 6.25 times of original BiVO4 and Cu2O, respectively. Ag-Cu2O/BiVO4 was characterized by X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), scanning electron microscope (SEM), energy dispersive X - ray spectroscopy (EDS), UV - Vis diffuse reflectance absorption spectra (UV - Vis DRS), photoluminescence (PL) spectra, transient photocurrent responses (TPC), and electrochemical impedance spectroscopy (EIS), and the possible reaction mechanism for the reduction of CO2 in the photocatalytic system was proposed.
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