Citation: GUO Shuai-Long, CHAO Yun-Xiu, YANG Hong-Wei, YANG Yu-Wen, LI Yu-Xiu, FANG Wei. Preparation and Catalytic Activity of Three-Dimensional Highly Branched Snowflake-like Silver[J]. Chinese Journal of Inorganic Chemistry, ;2018, 34(3): 421-426. doi: 10.11862/CJIC.2018.040 shu

Preparation and Catalytic Activity of Three-Dimensional Highly Branched Snowflake-like Silver

State Key Laboratory of Advanced Technologies for Comprehensive Utilization of Platinum Metals, Kunming Institute of Precious Metals, Kunming 650106, China

Corresponding author: FANG Wei, yhw@ipm.com.cn
Received Date: 16 August 2017
Revised Date: 25 October 2017

Figures(6)

Three-dimensional highly branched snowflake-like silver powder (3DHBS) has been one-step synthesized by reducing silver nitrate with ascorbic acid under the protection of polyvinyl alcohol in aqueous solution at room temperature. The microstructure of 3DHBS was investigated in details through different characteristic methods including X-ray diffraction (XRD) and scanning electron microscopy (SEM), and the possible formation mechanism was proposed based upon it. Additionally, 3DHBS exhibits superior catalytic activity for the hydrogenation reduction of p-nitrophenol.
- silver powder,
- polyvinyl alcohol,
- ascorbic acid,
- 4-nitrophenol,
- hydrogenation reduction
1. [1]
  Chia M Y, Chiu W S, Daud S N H, et al. Mater. Charact., 2015, 106:185-194 doi: 10.1016/j.matchar.2015.05.031
2. [2]
  Park S K, Choi K, Lee S H, et al. Carbon, 2017, 116:500-509 doi: 10.1016/j.carbon.2017.02.024
3. [3]
  Zhao R, Fu G, Zhou T, et al. Nanoscale, 2014, 6(5):2776-2781 doi: 10.1039/c3nr05718f
4. [4]
  Lu H, Zhang H, Yu X, et al. Plasmonics, 2012, 7(1):167-173 doi: 10.1007/s11468-011-9290-8
5. [5]
  HUANG Fu-Chun, LI Wen-Lin, XIONG Qing-Feng, et al. Precious Met., 2012, 33(2):30-35
6. [6]
  Yang J, Lu L, Wang H, et al. Cryst. Growth Des., 2006, 6(9):2155-2158 doi: 10.1021/cg060143i
7. [7]
  WANG Jing, WANG Hui, JING Xiao-Lian, et al. China Sciencepaper, 2015, 10(6):629-632
8. [8]
  SHI Chang-Kuai, LIANG Shi-Yu, ZHU Xiao-Yun. Rare Met., 2015, 39(6):533-539
9. [9]
  Zhai A X, Cai X H, Bin D U. Trans. Nonferrous Met. Soc. China, 2014, 24(5):1452-1457 doi: 10.1016/S1003-6326(14)63212-X
10. [10]
  SONG Yong-Hui, LIANG Gong-Ying, ZHANG Qiu-Li, et al. Rare Met. Mater. Eng., 2007, 36(4):709-712
11. [11]
  Song Y H, Zhou J T, Lan X Z, et al. Adv. Mater. Res., 2011, 233-235:1911-1915 doi: 10.4028/www.scientific.net/AMR.233-235
12. [12]
  Hild M, Mohammed F A R, Aibibu D, et al. Autex Res. J., 2015, 15(1):54-59
13. [13]
  Bleken F L, Chavan S, Olsbye U, et al. Appl. Catal. A, 2012, 447-448(24):178-185
14. [14]
  Burgin J, Florea I, Majimel J, et al. Nanoscale, 2012, 4(4):1299-1303 doi: 10.1039/c2nr11454b
15. [15]
  He Y, Su S, Xu T, et al. Nano Today, 2011, 6(2):122-130 doi: 10.1016/j.nantod.2011.02.004
16. [16]
  Ma X, Guo Q, Xie Y, et al. Chem. Phys. Lett., 2016, 652:148-151 doi: 10.1016/j.cplett.2016.04.004
17. [17]
  Yang C, Cui X, Zhang Z, et al. Nat. Commun., 2015, 6(8150):10-19
18. [18]
  Saha S, Pal A, Kundu S, et al. Langmuir, 2010, 26(4):2885-2893 doi: 10.1021/la902950x
19. [19]
  Liu W, Sun D, Fu J, et al. RSC Adv., 2014, 4(21):11003-11011 doi: 10.1039/C3RA47829G
20. [20]
  Xiong R, Lu C, Wang Y, et al. J. Mater. Chem. A, 2013, 1(47):14910-14918 doi: 10.1039/c3ta13314a
21. [21]
  MENG Xian-Wei, YANG Hong-Wei, HU Chang-Yi, et al. Chinese J. Inorg. Chem., 2016, 32(11):1981-1986
22. [22]
  Choi I H, Kim Y, Lee D N, et al. Polyhedron, 2016, 105:96-103 doi: 10.1016/j.poly.2015.12.022
23. [23]
  Zhang G, Deng C, Shi H, et al. Appl. Surf. Sci., 2017, 402:154-160 doi: 10.1016/j.apsusc.2017.01.042
24. [24]
  Mao Y, Wei J, Wang C, et al. Mater. Lett., 2015, 154(S01):47-50
25. [25]
  And M H R, Mandal T K. J. Phys. Chem. C, 2007, 111(45):16750-16760 doi: 10.1021/jp074963x
26. [26]
  Chi Y, Tu J, Wang M, et al. J. Colloid Interface Sci., 2014, 423(3):54-59
27. [27]
  Chi Y, Yuan Q, Li Y, et al. J. Colloid Interface Sci., 2012, 383(1):96-102 doi: 10.1016/j.jcis.2012.06.027
28. [28]
  Tang S, Vongehr S, Meng X. J. Phys. Chem. C, 2010, 114(2):977-982 doi: 10.1021/jp9102492
29. [29]
  Shin K S, Cho Y K, Chol J Y, et al. Appl. Catal. A, 2012, 413(1):170-175
30. [30]
  Gu S, Wang W, Tan F, et al. Mater. Res. Bull., 2014, 49(1):138-143
1. [1]
  Guimin ZHANG , Wenjuan MA , Wenqiang DING , Zhengyi FU . Synthesis and catalytic properties of hollow AgPd bimetallic nanospheres. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 963-971. doi: 10.11862/CJIC.20230293
2. [2]
  Jie ZHANG , Xin LIU , Zhixin LI , Yuting PEI , Yuqi YANG , Huimin LI , Zhiqiang LIU . Assembling a luminescence silencing system based on post-synthetic modification strategy: A highly sensitive and selective turn-on metal-organic framework probe for ascorbic acid detection. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 823-833. doi: 10.11862/CJIC.20230310
3. [3]
  Li'na ZHONG , Jingling CHEN , Qinghua ZHAO . Synthesis of multi-responsive carbon quantum dots from green carbon sources for detection of iron ions and L-ascorbic acid. Chinese Journal of Inorganic Chemistry, 2025, 41(4): 709-718. doi: 10.11862/CJIC.20240280
4. [4]
  Hailian Tang , Siyuan Chen , Qiaoyun Liu , Guoyi Bai , Botao Qiao , Fei Liu . Stabilized Rh/hydroxyapatite Catalyst for Furfuryl Alcohol Hydrogenation: Application of Oxidative Strong Metal-Support Interactions in Reducing Conditions. Acta Physico-Chimica Sinica, 2025, 41(4): 100036-. doi: 10.3866/PKU.WHXB202408004
5. [5]
  Yi DING , Peiyu LIAO , Jianhua JIA , Mingliang TONG . Structure and photoluminescence modulation of silver(Ⅰ)-tetra(pyridin-4-yl)ethene metal-organic frameworks by substituted benzoates. Chinese Journal of Inorganic Chemistry, 2025, 41(1): 141-148. doi: 10.11862/CJIC.20240393
6. [6]
  Xinhao Yan , Guoliang Hu , Ruixi Chen , Hongyu Liu , Qizhi Yao , Jiao Li , Lingling Li . Polyethylene Glycol-Ammonium Sulfate-Nitroso R Salt System for the Separation of Cobalt (II). University Chemistry, 2024, 39(6): 287-294. doi: 10.3866/PKU.DXHX202310073
7. [7]
  Yanan Liu , Yufei He , Dianqing Li . Preparation of Highly Dispersed LDHs-based Catalysts and Testing of Nitro Compound Reduction Performance: A Comprehensive Chemical Experiment for Research Transformation. University Chemistry, 2024, 39(8): 306-313. doi: 10.3866/PKU.DXHX202401081
8. [8]
  Xuejiao Wang , Suiying Dong , Kezhen Qi , Vadim Popkov , Xianglin Xiang . Photocatalytic CO₂ Reduction by Modified g-C₃N₄. Acta Physico-Chimica Sinica, 2024, 40(12): 2408005-. doi: 10.3866/PKU.WHXB202408005
9. [9]
  Jianyu Qin , Yuejiao An , Yanfeng Zhang . In Situ Assembled ZnWO₄/g-C₃N₄ S-Scheme Heterojunction with Nitrogen Defect for CO₂ Photoreduction. Acta Physico-Chimica Sinica, 2024, 40(12): 2408002-. doi: 10.3866/PKU.WHXB202408002
10. [10]
  Wenlong LI , Xinyu JIA , Jie LING , Mengdan MA , Anning ZHOU . Photothermal catalytic CO₂ hydrogenation over a Mg-doped In₂O_3-x catalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 919-929. doi: 10.11862/CJIC.20230421
11. [11]
  Weihan Zhang , Menglu Wang , Ankang Jia , Wei Deng , Shuxing Bai . 表面硫物种对钯-硫纳米片加氢性能的影响. Acta Physico-Chimica Sinica, 2024, 40(11): 2309043-. doi: 10.3866/PKU.WHXB202309043
12. [12]
  Yi YANG , Shuang WANG , Wendan WANG , Limiao CHEN . Photocatalytic CO₂ reduction performance of Z-scheme Ag-Cu₂O/BiVO₄ photocatalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 895-906. doi: 10.11862/CJIC.20230434
13. [13]
  Hailang JIA , Hongcheng LI , Pengcheng JI , Yang TENG , Mingyun GUAN . Preparation and performance of N-doped carbon nanotubes composite Co₃O₄ as oxygen reduction reaction electrocatalysts. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 693-700. doi: 10.11862/CJIC.20230402
14. [14]
  Tong Zhou , Xue Liu , Liang Zhao , Mingtao Qiao , Wanying Lei . Efficient Photocatalytic H₂O₂ Production and Cr(VI) Reduction over a Hierarchical Ti₃C₂/In₄SnS₈ Schottky Junction. Acta Physico-Chimica Sinica, 2024, 40(10): 2309020-. doi: 10.3866/PKU.WHXB202309020
15. [15]
  Hao XU , Ruopeng LI , Peixia YANG , Anmin LIU , Jie BAI . Regulation mechanism of halogen axial coordination atoms on the oxygen reduction activity of Fe-N₄ site: A density functional theory study. Chinese Journal of Inorganic Chemistry, 2025, 41(4): 695-701. doi: 10.11862/CJIC.20240302
16. [16]
  Shiyi WANG , Chaolong CHEN , Xiangjian KONG , Lansun ZHENG , Lasheng LONG . Polynuclear lanthanide compound [Ce₄^ⅢCe₆^Ⅳ(μ₃-O)₄(μ₄-O)₄(acac)₁₄(CH₃O)₆]·2CH₃OH for the hydroboration of amides to amine. Chinese Journal of Inorganic Chemistry, 2025, 41(1): 88-96. doi: 10.11862/CJIC.20240342
17. [17]
  Gaofeng WANG , Shuwen SUN , Yanfei ZHAO , Lixin MENG , Bohui WEI . Structural diversity and luminescence properties of three zinc coordination polymers based on bis(4-(1H-imidazol-1-yl)phenyl)methanone. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 849-856. doi: 10.11862/CJIC.20230479
18. [18]
  Yongqing Kuang , Jie Liu , Jianjun Feng , Wen Yang , Shuanglian Cai , Ling Shi . Experimental Design for the Two-Step Synthesis of Paracetamol from 4-Hydroxyacetophenone. University Chemistry, 2024, 39(8): 331-337. doi: 10.12461/PKU.DXHX202403012
19. [19]
  Liuyun Chen , Wenju Wang , Tairong Lu , Xuan Luo , Xinling Xie , Kelin Huang , Shanli Qin , Tongming Su , Zuzeng Qin , Hongbing Ji . 软模板法诱导Cu/Al₂O₃深孔道结构促进等离子催化CO₂加氢制二甲醚. Acta Physico-Chimica Sinica, 2025, 41(6): 100054-. doi: 10.1016/j.actphy.2025.100054
20. [20]
  Yunting Shang , Yue Dai , Jianxin Zhang , Nan Zhu , Yan Su . Something about RGO (Reduced Graphene Oxide). University Chemistry, 2024, 39(9): 273-278. doi: 10.3866/PKU.DXHX202306050

Get Citation

PDF

XML

Metrics

PDF Downloads(6)
Abstract views(1788)
HTML views(256)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142