Citation: LU Ya, LÜ Tian-Xi, HU Wei-Ji, WU Xiao-Yong, ZHAO Guo-Liang. Syntheses, Structures, DNA Interaction of Ag(Ⅰ) and Cd(Ⅱ) Coordination Polymers Based on Biphenyl-2, 4, 4', 6-tetracarboxylic Acid and Imidazo-phenanthrolin-phenoxy Acetic Acid[J]. Chinese Journal of Inorganic Chemistry, ;2017, 33(10): 1869-1875. doi: 10.11862/CJIC.2017.215 shu

Syntheses, Structures, DNA Interaction of Ag(Ⅰ) and Cd(Ⅱ) Coordination Polymers Based on Biphenyl-2, 4, 4', 6-tetracarboxylic Acid and Imidazo-phenanthrolin-phenoxy Acetic Acid

LU Ya ¹ ,
LÜ Tian-Xi ² ,
HU Wei-Ji ² ,
WU Xiao-Yong ² ,
ZHAO Guo-Liang ^1,2,,

1.
Xingzhi College, Zhejiang Normal University, Jinhua, Zhejiang 321004, China
2.
College of Chemistry and Life Science, Zhejiang Normal University, Jinhua, Zhejiang 321004, China

Corresponding author: ZHAO Guo-Liang, sky53@zjnu.cn
Received Date: 11 May 2017
Revised Date: 19 July 2017

Figures(6)

Two novel coordination polymers[Ag₄(BPTC)]_n (1) and[Cd(PIMPHC)₂]_n (2) were synthesized under hydrothermal reactions by using biphenyl-2, 4, 4', 6-tetracarboxylic acid (H₄BPTC, C₁₆H₁₀O₈) and 2-(4-(1H-imidazo-2-[4, 5-f] [1, 10]phenanthrolinyl)phenoxy) acetic acid (HPIMPHC, C₂₁H₁₄N₄O₃). They were characterized by elemental analysis, IR spectra, TGA, single crystal X-ray diffraction. Complex 1 crystallizes in triclinic system with space group P1, the coordination numbers of Ag(Ⅰ) are four, three and two, forming distorted tetrahedron, flat triangular and V-type coordination geometry. Complex 2 crystallizes in orthorhombic system with space group Pbcn, Each Cd(Ⅱ) is bridged by the PIMPHC^- anions, forming a distorted octahedral coordination geometry. The interaction of complexes, ligands and ct-DNA were studied by EtBr fluorescence probe.
- biphenyl-2, 4, 4', 6-tetracarboxylic acid,
- 2-(4-(1H-imidazo-2-[4, 5-f]-[1, 10]phen-anthrolinyl)phenoxy) acetic acid,
- Ag(Ⅰ),
- Cd(Ⅱ),
- DNA
1. [1]
  He Y B, Zhou W, Qian G D, et al. Chem. Soc. Rev., 2014, 43(16):5657-5678 doi: 10.1039/C4CS00032C
2. [2]
  Mason J A, Veenstra M, Long J R. Chem. Sci., 2014, 5(1):32-51 doi: 10.1039/C3SC52633J
3. [3]
  Li J R, Sculley J, Zhou H C. Chem. Rev., 2011, 112(2):869-932
4. [4]
  Herm Z R, Bloch E D, Long J R. Chem. Mater., 2014, 26(1):323-338 doi: 10.1021/cm402897c
5. [5]
  Wang Q, Bai J, Lu Z, et al. Chem. Commun., 2016, 52(3):443-452 doi: 10.1039/C5CC07751F
6. [6]
  Yoon M, Srirambalaji R, Kim K. Chem. Rev., 2011, 112(2):1196-1231
7. [7]
  Zhao M, Ou S, Wu C D. Acc. Chem. Res., 2014, 47(4):1199-1207 doi: 10.1021/ar400265x
8. [8]
  Kreno L E, Leong K, Farha O K, et al. Chem. Rev., 2011, 112(2):1105-1125
9. [9]
  Hu Z, Deibert B J, Li J. Chem. Soc. Rev., 2014, 43(16):5818-5840
10. [10]
  Hurd J A, Vaidhyanathan R, Thangadurai V, et al. Nat. Chem., 2009, 1(9):705-710 doi: 10.1038/nchem.402
11. [11]
  Sahoo S C, Kundu T, Banerjee R. J. Am. Chem. Soc., 2011, 133(44):17950-17958 doi: 10.1021/ja2078637
12. [12]
  Ma Z B, Moulton B. Coord. Chem. Rev., 2011, 255:1623-1641 doi: 10.1016/j.ccr.2011.01.031
13. [13]
  Efthimiadou E K, Karaliota A, Psomas G. J. Inorg. Biochem., 2010, 104:455-466 doi: 10.1016/j.jinorgbio.2009.12.019
14. [14]
  Cui Y, Yue Y, Qian G, et al. Chem. Rev., 2011, 112(2):1126-1162
15. [15]
  Zhao J, Wang X L, Shi X, et al. Inorg. Chem., 2011, 50(11):3198-3205
16. [16]
  Yu W H, Wang X Z, Ren X M, et al. Inorg. Chem. Commun., 2008, 11:799-801 doi: 10.1016/j.inoche.2008.03.036
17. [17]
  Shan X C, Zhou Y F, Zhang H B, et al. Inorg. Chem. Commun., 2012, 22:149-153 doi: 10.1016/j.inoche.2012.05.048
18. [18]
  Chen P K, Che Y X, Zheng J M, et al. CrystEngComm, 2010, 12:720-724 doi: 10.1039/B919676P
19. [19]
  Chang X H, Qin J H, Ma L F, et al. Cryst. Growth Des., 2012, 12(6):4649-4657
20. [20]
  Mereacre V, Baniodeh A, Powell A K, et al. J. Am. Chem. Soc., 2011, 133(6):15335-15337
21. [21]
  Li B, Zang S Q, Ji C, et al. Cryst. Growth Des., 2012, 12(3):1443-1451 doi: 10.1021/cg2015447
22. [22]
  Lin X, Jia J H, Zhao X B, et al. Angew. Chem. Int. Ed., 2006, 45(44):7358-7364 doi: 10.1002/(ISSN)1521-3773
23. [23]
  Liu T F, Lu J, Guo Z G, et al. Cryst. Growth Des., 2012, 10(4):1489-1491
24. [24]
  沈伟, 胡未极, 吴小勇, 等.无机化学学报, 2016, 32(6):1101-1110
25. [25]
  Sheldrick G M. SADABS, University of Göttingen, Germany, 1996.
26. [26]
  Sheldrick G M. SHELXS-97, Program for the Solution of Crystal Structure, University of Göttingen, Germany, 1997.
27. [27]
  Sheldrick G M. SHELXL-97, Program for the Refinement of Crystal Structure, University of Göttingen, Germany, 1997.
28. [28]
  王记江, 侯向阳, 曹培香, 等.无机化学学报, 2012, 28(4):829-832
29. [29]
  余玉叶, 石沛, 盛秀冬, 等.无机化学学报, 2014, 30(10):2332-2340
30. [30]
  Guo H D, Guo X M, Zhang H J, et al. Cryst. Growth Des., 2009, 9(3):1394-1401 doi: 10.1021/cg8006469
31. [31]
  Nakamoto K, Translated by HUANG De-Ru(黄德如), WANG Ren-Qing(汪仁庆). Infrared and Raman Spectra of Inorganic and Coordination Compounds(无机和配位化合物的红外和拉曼光谱). Beijing:Chemistry Industry Press, 1986.
32. [32]
  Lakowicz J R, Webber G. Biochemistry, 1973, 12(21):4161-4170 doi: 10.1021/bi00745a020
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