Citation: Xifeng Lu, Pei Su. Design and application of metal-organic frameworks derivatives as 3-electron ORR electrocatalysts for ^•OH generation in wastewater treatment: A review[J]. Chinese Chemical Letters, ;2025, 36(11): 110909. doi: 10.1016/j.cclet.2025.110909 shu

Design and application of metal-organic frameworks derivatives as 3-electron ORR electrocatalysts for ^•OH generation in wastewater treatment: A review

Xifeng Lu ,
Pei Su ^*,

Hebei Key Laboratory of Applied Chemistry and Hebei Key Laboratory of Heavy Metal Deep−Remediation in Water and Resource Reuse, School of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao 066004, China

sup@ysu.edu.cn

Received Date: 16 October 2024
Revised Date: 20 November 2024
Accepted Date: 3 February 2025
Available Online: 4 February 2025

Figures(6)

Derivatives of metal−organic frameworks (MOFs) are a promising bifunctional electrocatalysts in electrochemical advanced oxidation processes (EAOPs). These metal/carbon materials overcome the limitations of individual components by creating synergistic effects. EAOPs is primarily constrained by the generation and activation of H₂O₂. This article examines the regulatory strategies employed in MOFs derivatives to enhance the production of H₂O₂ via 2e⁻ pathways and its activation to ^•OH, focusing on preparation techniques, structures, and compositions. The design of these derivatives involves methods such as metal dispersion on the surface of nanocarbons, embedding in carbon shells, and atomic dispersion of metals anchored in porous carbon. MOFs derivatives promote ^•OH production and enhance wastewater purification through mechanisms such as boosting the Fe(Ⅱ)/Fe(Ⅲ) cycle, facilitating direct 3e⁻ reactions of O₂, and interacting of O₂^•−. Moreover, the performance and durability of MOFs derivatives in wastewater treatment, particularly in influencing ^•OH generation within EAOPs, were investigated. This review addresses current challenges and future prospects, offering valuable insights for the development of MOFs derivatives as 3e⁻ ORR electrocatalysts and the advancement of sustainable water treatment technologies.
- Metal−organic frameworks,
- Derivatives,
- 3-Electron ORR,
- Hydroxyl radicals,
- Water purification
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Design and application of metal-organic frameworks derivatives as 3-electron ORR electrocatalysts for •OH generation in wastewater treatment: A review

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通讯作者: 陈斌, bchen63@163.com

Design and application of metal-organic frameworks derivatives as 3-electron ORR electrocatalysts for ^•OH generation in wastewater treatment: A review