Citation: Jing Liu, Fei Wang, Huijie Wei, Yong Liu, Xiaoliang Zhai, Sifan Wen, Qiaobao Zhang. Fabrication and application of binder-free cathodes in high-performance lithium-chalcogen (S, Se, Te) batteries: A review[J]. Chinese Chemical Letters, ;2025, 36(11): 110475. doi: 10.1016/j.cclet.2024.110475 shu

Fabrication and application of binder-free cathodes in high-performance lithium-chalcogen (S, Se, Te) batteries: A review

Jing Liu ^a ,
Fei Wang ^b ,
Huijie Wei ^a ,
Yong Liu ^{a, *,} ,
Xiaoliang Zhai ^a ,
Sifan Wen ^{a, c} ,
Qiaobao Zhang ^{c, d, *,}

a.
School of Materials Science and Engineering, Provincial and Ministerial Co-construction of Collaborative Innovation Center for Non-ferrous Metal new Materials and Advanced Processing Technology, Henan University of Science and Technology, Luoyang 471023, China
b.
Faculty of Engineering, Huanghe Science & Technology University, Zhengzhou 450063, China
c.
State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Materials, Xiamen University, Xiamen 361005, China
d.
Longmen Laboratory, Luoyang 471023, China

liuyong209@haust.edu.cn

zhangqiaobao@xmu.edu.cn

Received Date: 2 September 2024
Revised Date: 17 September 2024
Accepted Date: 19 September 2024
Available Online: 19 September 2024

Figures(13)

Advanced lithium-chalcogen (S, Se, Te) batteries (LCBs) are among the most promising candidates for next generation energy storage systems because of their high energy density and theoretical capacities. However, they are still facing many challenges, such as expansion of the volume problems of chalcogen elements, the shuttle effect of intermediate products, low Coulombic efficiency and inferior cycling stability, which seriously hinder their commercial applications. The presence of a binder in the cathode causes an uneven distribution of the active substances, and also occupies a part of the electrode's volume, resulting in the unsatisfactory energy density of LCBs. In this regard, binder-free electrodes which do not need binders, conductive materials and even collectors, can be used as electrodes for flexible batteries, effectively solving the above-mentioned problems. In this review, the main methods of fabricating binder-free cathodes and their advantages and disadvantages are discussed. Furthermore, a review of representative works on binder-free cathodes for high-performance LCBs over the last decade is presented. The main binder-free electrode materials include paper cloth (PC), graphene oxide (GO), carbon nanotubes (CNTs), carbon nanofibers (CNFs), carbon cloth (CC), polymers, metallic compounds, and their composites. In addition, we discuss these works from four aspects: Advanced structures, methods of fabrication, electrochemical performance and the potential mechanism of binder-free cathode materials, providing important guidance for further researches. Finally, we propose the current challenges of binder-free LCBs and look forward to breakthroughs in this field through the use of binder-free electrodes.
- Binder-free cathode,
- Flexible,
- Lithium-chalcogen batteries,
- Li-S batteries,
- Electrochemical performance
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