Citation: Liwei Hou, Xianyun Peng, Siliu Lyu, Zhongjian Li, Bin Yang, Qinghua Zhang, Qinggang He, Lecheng Lei, Yang Hou. Advancements in MXene-based nanohybrids for electrochemical water splitting[J]. Chinese Chemical Letters, ;2025, 36(6): 110392. doi: 10.1016/j.cclet.2024.110392 shu

Advancements in MXene-based nanohybrids for electrochemical water splitting

Liwei Hou ^{a, b} ,
Xianyun Peng ^{a, c, *,} ,
Siliu Lyu ^e ,
Zhongjian Li ^{a, c} ,
Bin Yang ^{a, c} ,
Qinghua Zhang ^a ,
Qinggang He ^a ,
Lecheng Lei ^{a, c} ,
Yang Hou ^{a, c, d, *,}

a.
Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China
b.
College of Ocean Science and Engineering, Shanghai Maritime University, Shanghai 201306, China
c.
Institute of Zhejiang University - Quzhou, Quzhou 324000, China
d.
Zhejiang University Hydrogen Energy Institute, Hangzhou 310027, China
e.
Hubei Key Laboratory of Automotive Power Train and Electronic Control, School of Automotive Engineering, Hubei University of Automotive Technology, Shiyan 442002, China

xianyunpeng@zju.edu.cn

yhou@zju.edu.cn

Received Date: 14 July 2024
Revised Date: 4 August 2024
Accepted Date: 29 August 2024
Available Online: 31 August 2024

Figures(16)

Electrochemical water splitting presents a promising, environmentally friendly alternative to fossil fuels for hydrogen production. However, the efficiency is constrained by the sluggish kinetics and high overpotentials associated with the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). While noble metal catalysts, such as Pt for HER and Ir for OER, currently offer superior performance, their widespread adoption is hindered by high cost and scarcity. This has spurred research into cost-effective alternatives, with a focus on understanding the underlying electrocatalytic mechanisms. MXenes, a class of two-dimensional materials, have emerged as promising candidates for electrocatalytic water splitting due to their unique physical and chemical properties. However, research in this field remains largely experimental, lacking a comprehensive understanding of fundamental mechanisms. This knowledge gap impedes the development of high-efficiency electrocatalysts and necessitates further investigation. This review systematically examines recent advancements in MXene-based nanohybrids for electrocatalytic water splitting, covering synthetic methods, structure-property relationships, and performance enhancement strategies. It encompasses both precious and non-noble metal-based systems for HER, OER, and overall water splitting applications. Additionally, this review addresses current challenges, opportunities, and future research directions for MXene-based nanohybrids. By providing comprehensive insights into the development of high-performance MXene-based electrocatalysts, this review aims to accelerate progress in the field of electrochemical water splitting. It serves as a valuable resource for researchers and engineers working towards more efficient and sustainable hydrogen production technologies, potentially contributing to the broader goal of transitioning away from fossil fuels towards cleaner energy sources.
- Two-dimensional MXene,
- Electrocatalytic,
- Water splitting,
- Hydrogen evolution reaction,
- Oxygen evolution reaction
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沈阳化工大学材料科学与工程学院沈阳 110142