Citation: Bofeng Li, Yuxian Wang, Ya Liu, Zhe Han, Tiantian Xing, Yumin Zhang, Chunmao Chen. Design and engineering strategies of porous carbonaceous catalysts toward activation of peroxides for aqueous organic pollutants oxidation[J]. Chinese Chemical Letters, ;2025, 36(6): 110374. doi: 10.1016/j.cclet.2024.110374 shu

Design and engineering strategies of porous carbonaceous catalysts toward activation of peroxides for aqueous organic pollutants oxidation

Bofeng Li ^a ,
Yuxian Wang ^{a, *,} ,
Ya Liu ^b ,
Zhe Han ^a ,
Tiantian Xing ^a ,
Yumin Zhang ^a ,
Chunmao Chen ^{a, *,}

a.
State Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing 102249, China
b.
School of Chemical Engineering, The University of Adelaide, Adelaide, SA 5005, Australia

yuxian.wang@cup.edu.cn

c.chen@cup.edu.cn

Received Date: 13 May 2024
Revised Date: 22 July 2024
Accepted Date: 25 August 2024
Available Online: 26 August 2024

Figures(8)

Advanced oxidation processes (AOPs) governed by peroxide activation to produce highly oxidative active species have been extensively explored for environmental remediation. Nevertheless, the low diffusion rates, inadequate interactions of the reactants, and limited active site exposure hinder treatment efficiency. Porous carbocatalysts with high specific surface area, tunable pore size, and programmable active sites demonstrate outstanding performance in activating diverse types of peroxides to generate active species for treatment of aqueous organic pollutants. The pore-rich structures enhance reaction kinetics for peroxide activation by facilitating diffusion of the reactants and their interactions. Additionally, the structural flexibility of porous structures favors the accommodation of highly dispersed metal species and allows for precise tuning of the microenvironment around the active sites, which further enhances the catalytic activity. This review critically summarizes the recent research progress in the applications of engineered porous carbocatalysts for peroxide activation and outlines the prevailing pore construction methods in carbocatalysts. Moreover, engineering strategies to regulate the mass transfer efficiency and fine-tune the microenvironment around the active sites are systematically addressed to enhance their catalytic peroxide activation performances. Challenges and future research opportunities pertaining to the design, optimization, mechanistic investigation, and practical application of porous carbocatalysts in peroxide activation are also proposed.
- Porous carbocatalysts,
- Advanced oxidation processes (AOPs),
- Peroxide activation,
- Pore construction,
- Activity tuning
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沈阳化工大学材料科学与工程学院沈阳 110142