Citation: Liying Ou, Zhenluan Xue, Bo Li, Zhiwei Jin, Jiaochan Zhong, Lixia Yang, Penghui Shao, Shenglian Luo. Nitrogen-containing linkage-bonds in covalent organic frameworks: Synthesis and applications[J]. Chinese Chemical Letters, ;2025, 36(6): 110294. doi: 10.1016/j.cclet.2024.110294 shu

Nitrogen-containing linkage-bonds in covalent organic frameworks: Synthesis and applications

Liying Ou ^a ,
Zhenluan Xue ^a ,
Bo Li ^{a, *,} ,
Zhiwei Jin ^a ,
Jiaochan Zhong ^b ,
Lixia Yang ^b ,
Penghui Shao ^{b, *,} ,
Shenglian Luo ^b

a.
School of Materials Science and Engineering, Nanchang Hangkong University, Nanchang 330063, China
b.
Key Laboratory of Jiangxi Province for Persistent Pollutants Prevention Control and Resource Reuse, Nanchang Hangkong University, Nanchang 330063, China

Received Date: 27 February 2024
Revised Date: 25 June 2024
Accepted Date: 24 July 2024
Available Online: 25 July 2024

Figures(8)

Covalent organic frameworks (COFs) are crystalline porous polymeric materials composed of organic monomers connected by strong covalent bonds and offer high stability, good crystallinity, a large specific surface area, and controllable structures. COFs are widely used in the fields of adsorption and separation, catalysis, photovoltaics, and drug-delivery. The structural regulation and performance optimization of COFs can be realized through the modification of ligands and the selection of linkage methods. In which, the types of linkage are closely related to the stability and performance of COFs. In this review, nitrogen-containing linkage-bonds (NCLBs) in COFs are divided into N-containing double bonds, N-containing conjugated rings and N-containing unconjugated rings. The association between structure and performance of COFs is elaborated and the synthesis methods of COFs are systematically summarized. Moreover, the structural design, theoretical prediction and machinable application of COFs are prospected
- Covalent organic frameworks,
- Nitrogen-containing linkage-bonds,
- Structure and properties,
- Synthesis strategy and application,
- Porous materials
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