Citation: Jiayu Li, Binli Wang, Yu Luo, Hongyu Wang, Lei Zhang. The double-sided roles of difluorooxalatoborate contained electrolyte salts in electrochemical energy storage devices: A review[J]. Chinese Chemical Letters, ;2025, 36(8): 110220. doi: 10.1016/j.cclet.2024.110220 shu

The double-sided roles of difluorooxalatoborate contained electrolyte salts in electrochemical energy storage devices: A review

Jiayu Li ^a ,
Binli Wang ^b ,
Yu Luo ^b ,
Hongyu Wang ^{c, *,} ,
Lei Zhang ^{b, *,}

a.
School of Chemical Engineering and Energy Technology, Dongguan University of Technology, Dongguan 523808, China
b.
Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences, Shenzhen 518055, China
c.
Key Laboratory of UV Light Emitting Materials and Technology under Ministry of Education, Northeast Normal University, Changchun 130024, China

hongyuwang@aliyun.com

ZL199302@mail.ustc.edu.cn

Received Date: 28 May 2024
Revised Date: 17 June 2024
Accepted Date: 4 July 2024
Available Online: 5 July 2024

Figures(8)

In the realm of advanced electrochemical energy storage, the study of diverse electrolyte salts as integral components of electrolyte engineering has garnered immense attention. Notably, lithium di(fluoro)oxalateborate (LiDFOB) as the representative DFOB⁻ contained electrolyte salts, which possesses structural attributes resembling both lithium bis(oxalate)borate (LiBOB) and lithium tetrafluoroborate (LiBF₄), has garnered significant attention initially as a classical additive for the formation of solid electrolyte interface (SEI) films in graphite anodes. However, its unique properties have also piqued interest in other battery components, encompassing current collectors, capacity-enhanced cathodes or anodes, polymer solid-state electrolytes, and the full batteries. The introduction of LiDFOB or NaDFOB into these batteries exhibits a dual-faceted effect, with the beneficial aspect outweighing the potential drawbacks. Herein, we present a comprehensive overview of the research advancements surrounding LiDFOB, including the synthesis techniques of LiDFOB, the inherent properties of LiDFOB and LiDFOB-based electrolyte solutions, and the impact of LiDFOB on the performance of traditional graphite anodes, capacity-enlarged anodes, various classic cathodes, and the full batteries. And sectional content is about the usage of NaDFOB in Na-ion batteries. This review aims to aid readers in understanding the pivotal role of LiDFOB and NaDFOB as a constituent of electrolytes and how its utilization can influence electrode materials and other components, ultimately altering the electrochemical energy storage device's performance.
- Lithium difluorooxalatoborate,
- Sodium difluorooxalatoborate,
- Electrolyte,
- Electrode,
- Rechargeable batteries
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沈阳化工大学材料科学与工程学院沈阳 110142