Citation: Ming Yue, Yi-Rong Wang, Jia-Yong Weng, Jia-Li Zhang, Da-Yu Chi, Mingjin Shi, Xiao-Gang Hu, Yifa Chen, Shun-Li Li, Ya-Qian Lan. Multi-metal porous crystalline materials for electrocatalysis applications[J]. Chinese Chemical Letters, ;2025, 36(6): 110049. doi: 10.1016/j.cclet.2024.110049 shu

Multi-metal porous crystalline materials for electrocatalysis applications

School of Chemistry, Guangzhou Key Laboratory of Analytical Chemistry for Biomedicine, South China Normal University, Guangzhou 510006, China

Author Bio: Ming Yue received her B. Eng. degree at East China University of Science and Technology in 2021, and is now studying for a postgraduate degree at South China Normal University under the supervision of Prof. Ya-Qian Lan and Prof. Yifa Chen. Her research interest focuses on the design and synthesis of crystalline porous materials (MOF- and COF-based composites) for energy conversion
Yi-Rong Wang received her M.S. degree (2019) and Ph.D. degrees (2022) from Nanjing Normal University under the supervision of Prof. Ya-Qian Lan. Since 2022, she has carried out postdoctoral research at South China Normal University with Prof. Ya-Qian Lan. Her current research focuses on the synthesis of crystalline porous materials (MOF- and COF-based composites) and their applications in energy storage and conversion

Xiao-Gang Hu received his Ph.D. degree (2008) from the School of Chemistry and Chemical Engineering, Sun Yat-sen University. He joined the Analytical Chemistry Committee of Guangdong Chemical Society and the Chromatography Committee of Guangdong Analytical Testing Association. He joined South China Normal University (SCNU, China) in 2001, and is now a professor of chemistry. His-current research interest focuses on the fields of sample pretreatment, separation and enrichment materials, solid phase extraction, chromatographic analysis, nucleic acid aptamer, etc
Yifa Chen was born in 1989 in Fujian, China. He received his B.S. degree from School of Chemistry, Beijing Institute of Technology. He subsequently obtained his Ph.D. degree from School of Chemistry and Chemical Engineering, Beijing Institute of Technology under the supervision of Prof. Bo Wang. In 2018, he became an associate professor at Nanjing Normal University (NNU, China). In 2022, he joined South China Normal University (SCNU, China) as a professor of chemistry. His-research interest focuses on the fabrication of porous crystalline material based devices like membranes, foams and fibers that can be applicable in energy storage, environment treatment or photo-/electro-catalysis

yirongwang@m.scnu.edu.cn

huxg@scnu.edu.cn

chyf927821@163.com

Received Date: 7 February 2024
Revised Date: 4 May 2024
Accepted Date: 24 May 2024
Available Online: 24 May 2024

Figures(25)

Multi-metal porous crystalline materials (MPCM), integrating the functions of both multi-metal centres and porous crystalline materials (e.g., metal-organic frameworks (MOFs) and covalent organic frameworks (COFs)), are an extended class of porous materials that have attracted much attention for a broad range of applications. Owing to the advantages of these materials, they generally display high porosity, multi-metal active sites, well-tuned functions, and pre-designable structures, etc., serving as desired platforms for the study of structure-property relationships. In view of the clean and sustainable target, a series of MPCM have been explored as electrocatalysts for electrocatalytic reactions like hydrogen evolution reaction, oxygen evolution reaction and electrocatalytic CO₂ reduction reaction. Concerning the progress achieved for MPCM in electrocatalytic field during past years, this review will provide a brief introduction on the recent breakthrough of MPCM based electrocatalysts including their synthesis methods, structure design, component/morphology tuning, electrocatalytic property and structure-property relationship, etc. Besides, it will also conclude the current challenges and present perspectives for the MPCM based electrocatalysts, which might promote the development of porous crystalline materials in electrocatalysis and hope to provide new insights for scientists in related fields.
- Porous crystalline materials,
- Multi-metal,
- Metal-organic frameworks,
- Covalent organic frameworks,
- Electrocatalysis
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