Citation: Yuan Zhang, Shenghao Gong, A.R. Mahammed Shaheer, Rong Cao, Tianfu Liu. Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH₂-UiO-66 core-shell nanostructures[J]. Chinese Chemical Letters, ;2024, 35(4): 108587. doi: 10.1016/j.cclet.2023.108587 shu

Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH₂-UiO-66 core-shell nanostructures

Yuan Zhang ^{a, b, c, 1} ,
Shenghao Gong ^{a, b, c, 1} ,
A.R. Mahammed Shaheer ^{a, c} ,
Rong Cao ^{a, b, c, *,} ,
Tianfu Liu ^{a, b, c, *,}

a.
Fujian Science Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou 350108, China
b.
College of Chemistry and Materials Science, Fujian Normal University, Fuzhou 350007, China
c.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China

rcao@fjirsm.ac.cn

tfliu@fjirsm.ac.cn

Received Date: 12 April 2023
Revised Date: 4 May 2023
Accepted Date: 17 May 2023
Available Online: 20 May 2023

Figures(5)

MOF-based core-shell structures with high surface area, abundant active sites, and broad absorption bands are viable alternatives to traditional single-component photocatalysts. In this report, we describe the design and construction of delicate Ag nanowires@NH₂-UiO-66 with a core-shell structure for use as photocatalysts in imine synthesis under light. The optimized composites exhibited 80% imine production, which was higher than both MOF and Ag NWs. The significant improvement in photocatalytic activity under light may be attributed to the plasmonic effect of silver nanowires and their core-shell structure, which promotes the separation of electron-hole pairs. Moreover, the photocatalytic activity of the core-shell nanostructure may provide valuable insight into the design and construction of MOF-based composite photocatalysts for oxidative coupling of amines.
- Metal-organic frameworks,
- Plasmonic silver nanowires,
- Photocatalyst,
- Core-shell nanostructure,
- Oxidative coupling of amines
1. [1]
  S. Kobayashi, Y. Mori, J.S. Fossey, M.M. Salter, Chem. Rev. 111 (2011) 2626–2704. doi: 10.1021/cr100204f
2. [2]
  S. Kobayashi, H. Ishitani, Chem. Rev. 99 (1999) 1069–1094. doi: 10.1021/cr980414z
3. [3]
  B.S.Holla M.Ashok, B. Poojary, Eur. J. Med. Chem. 46 (2007) 1095.
4. [4]
  B. Ohtani, H. Osaki, S.I. Nishimoto, T. Kagia, Chem. Lett. 21 (1985) 1075. doi: 10.1246/cl.1985.1075
5. [5]
  F.Z. Su, S.C. Mathew, L. Mohlmann, et al., Angew. Chem. Int. Ed. 123 (2011) 683–686. doi: 10.1002/ange.201004365
6. [6]
  H.L. Chen, C. Liu, W. Guo, et al., Catal. Sci. Technol. 12 (2022) 1812. doi: 10.1039/d1cy02344f
7. [7]
  W. Phasayavan, M. Japa, S. Pornsuwan, et al., J. Colloid Interf. Sci. 581 (2021) 719–728. doi: 10.1016/j.jcis.2020.07.140
8. [8]
  K. Gao, H.J. Li, W J.H.W. Hou, ACS Appl. Mater. Interfaces. 13 (2021) 2779–2787. doi: 10.1021/acsami.0c21007
9. [9]
  Y. Xiao, Y. Huang, S. Xue, J. Zhao, Appl. Catal. B 265 (2020) 118596. doi: 10.1016/j.apcatb.2020.118596
10. [10]
  Z.Y. Zhai, X.N. Guo, G.Q. Jin, X.Y. Guo, Catal. Sci. Technol. 5 (2015) 4202–4207. doi: 10.1039/C5CY00395D
11. [11]
  Y. Xu, Y. Chen, W.F. Fu, Appl. Catal. B236 (2018) 176–183. doi: 10.1016/j.apcatb.2018.03.098
12. [12]
  L. Jiao, Y. Wang, H.L. Jiang, Q. Xu, Adv. Mater. 30 (2018) 1703663. doi: 10.1002/adma.201703663
13. [13]
  A. Dhakshinamoorthy, Z. Li, H. Garcia, Chem. Soc. Rev. 47 (2018) 8134–8172. doi: 10.1039/c8cs00256h
14. [14]
  Y. Song, R. Wang, X.Y. Li, et al., Chin. Chem. Lett. 33 (2021) 1283–1287.
15. [15]
  J. Perezjuste, I. Pastorizasantos, L. Lizmarzan, P. Mulvaney, Coord. Chem. Rev. 249 (2005) 1870–1901. doi: 10.1016/j.ccr.2005.01.030
16. [16]
  Q.Q. Huang, Z.B. Fang, K. Pang, et al., Adv. Funct. Mater. 32 (2022) 2205147. doi: 10.1002/adfm.202205147
17. [17]
  C. Liu, Y.Y. Liu, Y.Z. Shi, J. Colloid Interf. Sci. 631 (2023) 154–163. doi: 10.1016/j.jcis.2022.11.042
18. [18]
  D. Bellet, M. Lagrange, T. Sannicolo, et al., Materials 10 (2017) 570. doi: 10.3390/ma10060570
19. [19]
  Y. Bai, Y. Dou, L.H. Xie, et al., Chem. Soc. Rev. 45 (2016) 2327–2367. doi: 10.1039/C5CS00837A
20. [20]
  L. Shi, X. Zou, T. Wang, et al., Chin. Chem. Lett. 33 (2022) 442–446. doi: 10.1016/j.cclet.2021.06.048
21. [21]
  T. Xia, Y.C. Lin, W.Z. Li, et al., Chin. Chem. Lett. 32 (2021) 2975–2984. doi: 10.1016/j.cclet.2021.02.058
22. [22]
  S. Choi, J. Park, W. Hyun, et al., ACS Nano 9 (2015) 6626. doi: 10.1021/acsnano.5b02790
23. [23]
  A.H. Ibrahim, W.A. Eimehalmey, R.R. Haikal, et al., Inorg. Chem. 58 (2019) 15078–15087. doi: 10.1021/acs.inorgchem.9b01611
24. [24]
  X. Fang, S.B. Wu, Y.H. Wu, et al., Appl. Surf. Sci. 518 (2020) 146226. doi: 10.1016/j.apsusc.2020.146226
25. [25]
  R. Chandra, M. Nath, Appl. Organoment. Chem. 34 (2020) e5951. doi: 10.1002/aoc.5951
26. [26]
  C.X. Zhang, C.F. Xie, Y.Y. Gao, et al., Angew. Chem. Int. Ed. 61 (2022) e202204108. doi: 10.1002/anie.202204108
27. [27]
  C. Sönnichsen, T. Franzl, T. Wilk, et al., Phys. Rev. Lett. 88 (2002) 077402. doi: 10.1103/PhysRevLett.88.077402
28. [28]
  R.B. Jiang, B.X. Li, C.H. Fang, J.F. Wang, Adv. Mater. 26 (2014) 5274–5309. doi: 10.1002/adma.201400203
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沈阳化工大学材料科学与工程学院沈阳 110142

Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH2-UiO-66 core-shell nanostructures

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通讯作者: 陈斌, bchen63@163.com

Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH₂-UiO-66 core-shell nanostructures