Citation: Xiaodong Zhao, Qian Liu, Xiaolei Li, Huiming Ji, Zhurui Shen. Two-dimensional g-C₃N₄ nanosheets-based photo-catalysts for typical sustainable processes[J]. Chinese Chemical Letters, ;2023, 34(11): 108306. doi: 10.1016/j.cclet.2023.108306 shu

Two-dimensional g-C₃N₄ nanosheets-based photo-catalysts for typical sustainable processes

Xiaodong Zhao ^a ,
Qian Liu ^b ,
Xiaolei Li ^{a, *,} ,
Huiming Ji ^a ,
Zhurui Shen ^{b, *,}

a.
Key Laboratory of Advanced Ceramics and Machining Technology, Ministry of Education, School of Materials Science and Engineering, Tianjin University, Tianjin 300072, China
b.
School of Materials Science and Engineering, Nankai University, Tianjin 300350, China

lxlei@tju.edu.cn

shenzhurui@nankai.edu.cn

Received Date: 29 October 2022
Revised Date: 6 February 2023
Accepted Date: 5 March 2023
Available Online: 11 March 2023

Figures(9)

Graphitic carbon nitride (g-C₃N₄) has been widely studied as a visible light responsive photocatalyst in recent years, due to its facile synthesis, low cost, high stability, and appropriate bandgap/band positions. In this review, we firstly introduce and compare various exfoliation approaches of bulk g-C₃N₄ into ultrathin g-C₃N₄ nanosheets. Then, many modification strategies of g-C₃N₄ nanosheets are also reviewed, including heterojunction construction, doping, defect control, and structure design. Thereafter, the charge transfer mechanism in g-C₃N₄ nanosheets based heterojunctions is present, e.g., Z-scheme, S-scheme and other forms. Besides, the photocatalytic applications of g-C₃N₄ nanosheets based photocatalysts are summarized including environmental remediation, energy generation and storage, organic synthesis, and disinfection. This review ends with a summary and some perspectives on the challenges and new directions in exploring g-C₃N₄ nanosheets-based photocatalysts.
- Graphitic carbon nitride (g-C₃N₄) nanosheets,
- Exfoliation approaches,
- Hetero-junction,
- Z-scheme mechanism,
- Photo-catalytic applications
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Two-dimensional g-C3N4 nanosheets-based photo-catalysts for typical sustainable processes

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通讯作者: 陈斌, bchen63@163.com

Two-dimensional g-C₃N₄ nanosheets-based photo-catalysts for typical sustainable processes